Abstract
EARLY in 1920 Harkins and Broeker reported a separation of chlorine into isotopes, which amounted at that time to an increase in density equal to 1550 parts per million. About six months later Brønsted and von Hevesy reported a separation of mercury, which was, however, only about one-thirtieth as great, or 50 parts per million. On account of the slightness of the density change reported for mercury, the evidence, that it had been separated did not appear to be conclusive, so it seemed worth while to attempt a confirmation by the same method—that is, a vaporisation at low pressures. As a result of 4 cuts of 2 on the heavy fraction or residue the density has been increased by 69 parts per million, and by the same number of cuts on the light fraction it has been decreased 62 parts, or the total density change obtained is 133 parts pet million, or 0.027 units of atomic weight.
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HARKINS, W., MULLIKEN, R. The Separation of Mercury into Isotopes. Nature 108, 146 (1921). https://doi.org/10.1038/108146a0
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DOI: https://doi.org/10.1038/108146a0