Table 1 Performance of quasi-2D PeLEDs (from NIR to blue)
From: High-performance quasi-2D perovskite light-emitting diodes: from materials to devices
Year | Perovskite materials | Device architecture | EL [nm] | FWHM [nm] | Peak EQE [%] | Lmax [cd m−2]/ Rmax [Wsr−1 m−2] | T50 stability | Refs. |
|---|---|---|---|---|---|---|---|---|
Near-infrared (NIR) quasi-2D PeLEDs | ||||||||
2016 | (PEA)2MA4Pb5I16 | ITO/TiO2/perov/F8/MoO3/Au | 750 | – | 8.8 | 80R | – | |
2016 | (NMA)2FAPb2I6Br | ITO/ZnO/PEIE/perov/TFB/MoOx/Au | 786 | – | 11.7 | 82R | 2 h @10 mA cm−2 | |
2017 | MAPbI3·20%FPMAI | ITO/Poly-TPD/perov/TPBi/LiF/Al | 749 | – | 7.9 | 72R | >10 h@3 mA cm−2 | |
2017 | MAPbI3·20%BAI | ITO/Poly-TPD/perov/TPBi/LiF/Al | 748 | – | 10.4 | 30 | 90 s@5 v | |
2018 | Cs0.2FA0.8PbI2.8Br0.2·20%BAI | ITO/Poly-TPD/perov/TPBi/LiF/Al | 752 | – | 17.6 | 199R | 50 min@10 mA cm−2 | |
2018 | (NMA)2(FA)n−1PbnI3n+1·poly-HEMA | ITO/MZO/PEIE/PPBH/TFB-PFO/MoOx/Au | ~780 | ~49 | 20.1 | <10R | 46 h@0.1 mA cm−2 | |
2018 | MAPbI3·FPMAI | AgNW/Poly-TPD/perov/TPBi/LiF/Al | 740 | – | 13 | – | – | |
2018 | (NMA)2FAn−1PbnI3n+1 | ITO/PEIE-ZnO/perov/TFB/MoOx/Al | ~790 | – | 12.7 | 254R | 30 min@100 mA cm−2 | |
2019 | MAPbI3·20%PMAI | ITO/Poly-TPD/perov/TPBi/LiF/Al | 750 | – | 15 | – | – | |
2019 | (EDBE)FAn−1PbnI3n+1 | ITO/ZnMgO/perov/TFB/MoOx/Al | 804 | – | 11.4 | 60R | 1.3 h@10 mA cm−2 20 h@2 mA cm−2 | |
2019 | (BAB)FAn−1PbnI3n+1 | ITO/PEIE-ZnO/perov/TFB/MoOx/Al | 776 | 50 | 5.2 | 88.5R | >100 h@25 mA cm−2 | |
2020 | PbS QDs in (PEA)2Cs2Pb3Br10 | ITO/PEDOT:PSS/QDLP/TPBi/LiF/Al | 980 | – | 8.1 | 7.4R | >1 h@10 mA cm−2 | |
2020 | (NMA)2FAn−1PbnI3n+1 | Glass/Au/ZnO/PEIE/perov/TFB/MoO3/Au | 800 | 35.4 | 20.2 | 114.9R | – | |
Red quasi-2D PeLEDs | ||||||||
2017 | (NMA)2Csn−1Pbn(I/Cl)3n+1 | ITO/ZnO/PEIE/perov/TFB/MoOx/Au | 688 | – | 3.7 | ~440 | 5 h@10 mA cm−2 | |
2017 | (PBA)2Csn−1PbnI3n+1 | ITO/NiO/Poly-TPD/PVK/perov/TPBi/Ca/Al | 683 | ~34 | 7.3 | ~130 | – | |
2018 | (NMA)2Csn−1PbnI3n+1 | ITO/ZnO/PEIE/perov/TFB/MoOx/Au | 694 | 7.3 | 732 | – | ||
2018 | (BA)2Csn−1PbnI3n+1·PEO | ITO/PEDOT:PSS/Poly-TPD/perov/BCP/LiF/Al | 638 | 61 | 0.41 | 390 | >4 h@3.5 v | |
664 | 50 | 2.81 | 1231 | |||||
680 | 39 | 6.23 | 1392 | |||||
690 | 36 | 4.73 | 186 | |||||
2019 | (PBA)2Csn−1PbnI3n+1 | ITO/PEDOT:PSS/Poly-TPD/PVK/perov/TPBi/LiF/Al | 664 | (0.72, 0.27) | 13.3 | 968 | – | |
2020 | (PEA)2SnI4 | ITO/PEDOT:PSS/perov/TPBi/LiF/Al. | 633 | 24/(0.706,0.294) | 0.3 | 70 | ||
2020 | (PEA)2SnI4 | ITO/PEDOT:PSS/perov/TPBi/LiF/Al | 632 | 21/(0.708,0.292) | 5 | ~100 | >15 h@20 cd m−2 | |
Green quasi-2D PeLEDs | ||||||||
2016 | (PEA)2MAn−1PbnBr3n+1 | ITO/Buf-HIL/perov/TPBi/LiF/Al | 525 | – | 4.9(CE) | 2935 | – | |
2017 | (PEA)2MAn−1PbnBr3n+1 | ITO/PEDOT:PSS/perov/TPBi/LiF/Al | 526 | – | 7.4 | 8400 | – | |
2017 | (PBA)2Csn−1PbnBr3n+1 | ITO/NiO/TFB/PVK/perov/TPBi/Ca/Al | 514 | 17 | 10.4 | 14,000 | – | |
2018 | (C8H17NH3)2FAn−1PbnBr3n+1 | ITO/LiF/perov/PO-T2T/Ca/Al | 540 | – | 5 | ~3000 | – | |
2018 | (OA)2FAn−1PbnBr3n+1 FAPbBr3 NCs | ITO/PEDOT:PSS/perov/PO-T2T/Ca/Al | 528–532 | 25–26 | 13 | 56,143 | – | |
2018 | (BA)2FA2Pb3Br10 | ITO/NiOx/perov/TPBi/LiF/Al | 530–540 | – | 14.6 | 24,100 | 102 min@100 cd m−2 | |
2018 | (PEA)2FA2Pb3Br10 | ITO/m-PEDOT:PSS/perov/TOPO/TPBi/LiF/Al | 532 | 23 | 14.36 | 9120 | 70 min@280 cd m−2 | |
2018 | (BA)2Csn−1PbnBr3n+1·PEO | ITO/PEDOT:PSS/perov/TPBi/Ca/Al | 514 | 19–21 | 8.42 | 33,533 | 45 min@100 cd m−2 | |
2018 | (PEA)2Csn−1PbnBr3n+1/Cs4PbBr6 | ITO/PEDOT:PSS:PFI/perov/TPBi/LiF/Al | 500 | 24 | 4.51 | 3259 | 72 min@10 mA cm−2 | |
2018 | (PEA)2CsnPbnBr3n+1 | ITO/Poly-TPD/PFN/perov/TPBi/LiF/Al | 512 | 22 | 14.4 | 23,380 | >25 min@3.5 v | |
2018 | (BIZ)2FA2PbnBr3n+1 | ITO/PVK/perov/TmPyPB/LiF/Al | 537 | – | 7.7 | 30,000 | 63 min@1330 cd m−2 | |
2018 | (PEA)2Csn−1PbnBr3n+1 | ITO/Poly-TPD/perov/TPBi/LiF/Al | 514 | – | 15.5 | ~20,000 | 90 min@2 mA cm−2 | |
2018 | FAPbBr3·DPPABr | ITO/PEDOT:PSS/TFB/perov/TPBi/LiF/Al | 526 | 22 | 16.3 | 13,970 | – | |
2019 | (PBA/PA)2FAn−1PbnBr3n+1 | ITO/PVK:TPD-DDAB/perov/TPBi/CsF/Al | 534 | 25 | 15.1 | 8052 | – | |
2019 | (PEA)2FAn−1PbnBr3n+1 | ITO/PEDOT:PSS-Na/perov/TOPO/TPBi/LiF/Al | 532 | – | 15.4 | 15,765 | – | |
2019 | (PEA)2FA2Pb3Br10 | ITO/PEDOT:PSS/perov/TPBi/LiF/Al | 525 | – | 10.6 | 41,500 | 9.2 h@10 mA cm−2 | |
2019 | CsPbBr3·NaBr | ITO/TFB/PVK/perov/TPBi/LiF/Al | 518 | 21.7 | 15.9 | 11,560 | ~2.5 h@150 cd m−2 | |
2019 | BA2CsnPbnBr3n+1 | ITO/PEDOT:PSS/PVK/perov/TPBi/Al | 506 | – | 10.1 | 3810 | – | |
513 | 7.2 | 11,200 | ||||||
2019 | (PEA)2Csn−1PbnBr3n+1·NaBr | ITO/NiOx/PVK/perov/TPBi/LiF/Al | 512 | – | 17.4 | 8353 | 40 min@100 cd m−2 | |
2020 | PEA2Cs2.4MA0.6Pb4Br13 | ITO/PEDOT:PSS:PFI/perov/TPBi/LiF/Al | 517 | – | 14 | 45,230 | 3.5 h@4000 cd m−2 | |
2020 | (PEA)2FAn−1PbnBr3n+1 | ITO/PVK/perov/TPBi/LiF/Al | 529 | 23 | 14.7 | 37,477 | <1 h@0.25 mA cm−2 | |
2020 | (PEA)2(FA/Cs)n−1PbnBr3n+1 | ITO/PEDOT:PSS/perov/TPBi/LiF/Al | 528 | 24 | 4.5 | 10,000 | 42 s@5 V | |
2020 | (PEA)2FAn−1PbnBr3n+1 | ITO/PVK/perov/TPBi/LiF/Al | 527 | 21 | 12.4 | ~6500 | 1.5 h@1 mA cm−2 | |
2020 | (PEA)2Csn−1PbnBr3n+1 | ITO/TFB/LiF/perov/TPBi/LiF/Al | ~520 | ~18 | 19.1 | ~50,000 | – | |
2021 | (p-FPEA)2MAn−1PbnBr3n+1 | ITO/PEDOT:PSS/PFNBr/perov/PMMA/TmPyPB/LiF/Al | 525 | 21.2 | 20.36 | 82,480 | 6.5 min@10000 cd m−2 | |
Blue quasi-2D PeLEDs | ||||||||
2016 | (PEA)2PbBr4 | ITO/PEDOT: PSS/perov/TPBi/Al/Ca | 410 | – | 0.04 | – | – | |
2016 | (OLA)2MAn−1PbnBr3n+1 | ITO/PEDOT: PSS/CBP/perov/TPBi/LiF/Al | 492 | 24 | 0.23 | 8.5 | ||
456 | 18 | 0.024 | 1 | |||||
432 | 40 | 0.004 | 1 | |||||
2017 | (PEOA)2MAn−1PbnBr3n+1 | ITO/PEDOT: PSS/perov/TPBi/Ba/Al | 494 | – | 1.1 | 19.5 | – | |
462 | 0.06 | 1.26 | ||||||
2017 | (4-PBA)2PbBr4 | ITO/PEIE-ZnO/perov/TFB/MoOx/Al | 491 | – | 0.015 | 186 | – | |
2017 | (EA)2MAn−1PbnBr3n+1 | ITO/PEDOT:PSS/perov/TmPyPB/CsF/Al | 473 | – | 2.6 | 200 | – | |
2018 | (PEA/IPA)2(MA/Cs)n−1PbnBr3n+1 | ITO/PEDOT:PSS/NiOx/PVK/perov/TPBi/LiF/Al | 490 | 28 | 1.5 | 2480 | 10 min@10 cd m−2 4 min@20 cd m−2 0.5 min@210 cd m−2 | |
2018 | PA2Csn−1PbnBr3n+1 | ITO/PEDOT:PSS/perov/TmPyPB/Cs2CO3/Al | 505 | 26 | 3.6 | 7320 | 30 min@4.8 v | |
2019 | (BA)2Csn−1Pbn(Br/Cl)3n+1 | ITO/PEDOT:PSS/PVK/perov/TPBi/Al | 465 | 23 | 2.4 | 962 | 1 min@500 cd m−2 | |
487 | 25 | 6.2 | 3340 | 10 min@800 cd m−2 | ||||
2019 | (PBA)2Csn−1Pbn(Br/Cl)3n+1 | ITO/NiOx/LiF/perov/TPBi/LiF/Al | 490 | 21 | 0.52 | 1446 | – | |
2019 | (PA)2Csn−1PbnBr3n+1 | ITO/NiOx-PSSNa/perov/TPBi/LiF/Al | 492 | 26 | 1.45 | 4359 | 220 min@150 cd m−2 120 min@415 cd m−2 | |
2019 | (PEA)2Csn−1Pbn(Br/Cl)3n+1 | ITO/PEDOT:PSS/perov/TPBi/LiF/Al | 485 | – | 11.0 | 9040 | 100 min@100 cd m−2 | |
2019 | (PEA)2Csn−1Pbn(Br/Cl)3n+1 | ITO/PEDOT:PSS/perov/TPBi/LiF/Al | 480 | 21 | 5.7 | 3780 | 10 min@1500 cd m−2 | |
2019 | (PEA/P-PDABr2)2Csn−1PbnBr3n+1 | ITO/PVK/PFI/perov/3TPYMB/Liq/Al | 465 | 25 | 2.6 | 211 | 13.5 min@0.35 mA cm−2 | |
2019 | (PEA)2(Rb/Cs)n−1PbnBr3n+1 | ITO/PEDOT:PSS/perov/TmPyPB/LiF/Al | 475 | 20 | 1.35 | 100.6 | 14.5 min@15 cd m−2 | |
2019 | (PEA/NPA)2Csn−1PbnBr3n+1 | ITO/PVK/perov/PO-T2T/Liq/Al | 485 | 23 | 2.62 | 1200 | 4.3 min@100 cd m−2 | |
2019 | PBABr2(Cs0.7FA0.3PbBr3) | ITO/NiOx/TFB/PVK/perov/TPBi/LiF/Al | 483 | – | 9.5 | 700 | 4 min@100 cd m−2 | |
2020 | PEA2Cs1.6MA0.4Pb3Br10·DPPOCl | ITO/PEDOT:PSS:PFI or Poly-TPD/perov/TPBi/LiF/Al | 489 | 18 | 1.3 | 5141 | 51 min@1500 cd m−2 | |
479 | 18 | 5.2 | 468 | 90 min@100 cd m−2 | ||||
2020 | (PBA)2Csn−1PbnBr3n+1 | ITO/PEDOT:PSS/perov/POT2T/LiF/Al | 465 | – | 2.34 | 150 | 232 s@12 cd m−2 | |
493 | 5.08 | 1000 | ||||||
2020 | CsPbBr3·GABA | ITO/PEDOT:PSS:PFI/PVK/CsPbBr3 QW/TPBi/LiF/Al | 478 | (0.12, 0.14) | 6.3 | 200 | 150 s@200 cd m−2 | |
2020 | PEA2(Cs1−xEAxPbBr3)2PbBr4 | ITO/m-PEDOT:PSS/perov/TPBi/LiF/Al | 495 | 23 | 13.3 | 2790 | 200s@100 cd m−2 | |
488 | 25 | 12.1 | 2191 | |||||
480 | 25 | 4.19 | 83 | |||||
2020 | (PEA)2Csn−1Pbn(Br/Cl)3n+1·NaBr | ITO/NiOx/PTAA/PVK/perov/TPBi/LiF/Al | 488 | 18.8 | 11.7 | 1511 | 970 s@100 cd m−2 | |
2020 | (PEA/PA)2Csn−1PbnBr3n+1 | ITO/PVK/perov/TPBi/LiF/Al | 486 | 25 | 10.11 | ~600 | 81.3 min@0.3 mA cm−2 | |
2020 | (Cs/FA/p-F-PEA)Pb(Cl/Br)3 | ITO/PEDOT:PSS/perov/TPBi/LiF/Al | 469 | (0.125, 0.076) | 4.14 | 451 | 14.0 min@1 mA cm−2 | |