Fig. 3 | Nature Communications

Fig. 3

From: All-optical control of long-lived nuclear spins in rare-earth doped nanoparticles

Fig. 3

All-optical dynamical decoupling. a CPMG sequence with optical 2-color excitation and rephasing π pulses. The initial excitation pulse has a Y phase and the π pulses an X phase. This is obtained by varying the relative phase between the two frequency components of the optical pulses. b Echo decays (circles) for different initial phases and exponential fits (lines). A much lower T2DD is observed for an X initial phase (~1.0 ms) than for an Y one (~3.0 ms). This is due to the accumulation of pulse errors and confirms that our DD sequence behaves as a CPMG one. c Spin-echo decays (circles) obtained for τDD = 150, 200 and 300 µs with n ≤ 60, and exponential fits (lines). d Experimental (circles) and modelled (line) T2DD evolution as a function of τDD. (see Supplementary Fig. 5). The data point represented by the black circle was discarded for the fit. e Spin-echo decays (circles) with and without a weak magnetic field. Solid line: exponential fits. Error bars and uncertainties correspond to ±1 standard error

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