Fig. 3: Comparison between experiment and theory.

a Interfacial nuclear-spin current and thermal equilibration of nuclear spins in MnCO3. An interfacial spin current, Jne, is mediated by the Korringa process through the hyperfine interaction between nuclear spins of 55Mn and electron spins in the metal at the Pt/MnCO3 interface. Jne arises in proportion to the effective temperature difference between the electrons in Pt (Te) and nuclei in MnCO3 (Tn): \({J}_{{\rm{ne}}}={\Gamma }_{{\rm{ne}}}{k}_{\mathrm{B}}({T}_{\mathrm{e}}-{T}_{\mathrm{n}})\). Here, the difference Te − Tn may be triggered by the interfacial temperature drop Te − Tp between the Pt and MnCO3 (Tp: phonon temperature in MnCO3 close to the interface) and the thermalization between nuclei and phonons in MnCO3, whose rate is given by \({J}_{{\rm{np}}}={\Gamma }_{{\rm{np}}}{k}_{\mathrm{B}}({T}_{\mathrm{n}}-{T}_{\mathrm{p}})\). b B dependence of the calculated temperature difference \({T}_{\mathrm{e}}-{T}_{\mathrm{n}}\) normalized by the interfacial temperature drop \({T}_{\mathrm{e}}-{T}_{\mathrm{p}}\) at T = 100 mK and 1 K. In the steady state, \({J}_{{\rm{ne}}}={J}_{{\rm{np}}}\)31, which gives \(({T}_{\mathrm{e}}-{T}_{\mathrm{n}})/({T}_{\mathrm{e}}-{T}_{\mathrm{p}})={\Gamma }_{{\rm{np}}}/({\Gamma }_{{\rm{np}}}+{\Gamma }_{{\rm{ne}}})\). Bc indicates the crossover field, where \({\Gamma }_{{\rm{ne}}}={\Gamma }_{{\rm{np}}}\). c Comparison between the B dependence of the experimental V/I2rms (blue plots) for the Pt/MnCO3 Device 2 and the calculated V/I2rms for the nuclear SSE \({{\mathscr{S}}}_{{\rm{n}}}\) (red solid curve) and for the electronic SSE \({{\mathscr{S}}}_{{\rm{m}}}\) (gray solid curve) at T = 101 mK (see Supplementary Note 9 for details). The inset shows a blowup of the calculated V/I2rms for the electronic SSE \({{\mathscr{S}}}_{{\rm{m}}}\) (multiplied by 103). d Comparison between the B dependence of the experimental V/I2rms (blue plots) and the calculated V/I2rms for the nuclear SSE \({{\mathscr{S}}}_{{\rm{n}}}\) (red solid line) at 100 mK < T < 1 K. e Comparison between the T dependence of the experimental V/I2rms (green rhombus) and the calculated V/I2rms for the nuclear SSE \({{\mathscr{S}}}_{{\rm{n}}}\) (red solid curve). The error bar represents the SD.