Fig. 1: Sample architecture and principle of SOI.

a Schematic diagram of the microcavity CP-OLED device structure. The bottom Ag (200 nm) and the top Ag (35 nm)/CsF (10 nm) films serve as the hole and electron injection layers for the OLED and meanwhile function as two mirrors forming a Fabry-Pérot planar microcavity. The 6M-DSB OSCs serve as the emitting layer of the OLED and as birefringent optical medium necessary for the realization of SOI in the microcavity. Right panel: the top-view bright-field of patterned microcavity CP-OLEDs. b Left: Molecular structure of 6M-DSB from single-crystal data, showing the enhanced planarity. Right: brickwork molecular packing arrangement within the (001) crystal plane, viewed perpendicular to the microribbon top-facet. The nearest intermolecular distance is around 3.6 Å. c Left: two orthogonally linearly polarized modes with the same parity in an isotropic microcavity. Middle: the dispersion of two orthogonally linearly polarized modes in an anisotropic microcavity. Right: RD SOI emerges when two orthogonally linearly polarized modes with opposite parity are resonant. d The resonant X- and Y-polarized cavity modes of opposite polarity. The 6M-DSB crystal in the microcavity hence acts as a half-wave plate, and the intrinsic mode polarization of the light-emitting side of the mirror turns into a circle, corresponding to left-handed and right-handed circular polarizations, respectively.