Extended Data Fig. 3: Angle-resolved RABBIT traces and the extracted RABBIT phases of SB12 from the TDSE simulation based on the p− and p0 ground-state orbitals.
From: Attosecond circular-dichroism chronoscopy of electron vortices
(a-c), Results from the p− orbital. In this case the m of the main peaks created by the XUV photoionization is zero and thus the continuum electron wave packet has no chirality. Therefore, both the sideband yield and phase don’t depend on the helicity of the probe IR. (d-f), Results from the p0 orbital. In this case the m of the main peaks created by the XUV photoionization is 1, and thus the degree of chirality is less than that from the p+ ground-state orbital. Therefore, the CD effects on the sideband yield and phase are decreased compared to those from the p+ orbital shown in Fig. 2g-i, but the basic structures are not changed.
