Figure 2

(a–d) Time-domain P-polarized THz waveforms radiated from the (111) surface of n-type Cu0.02Bi2Se3 and p-type Bi2Te3 by P- and S-polarized optical pulse excitation. In (a), the thin-red line represents the 0.015-times smaller P-polarized THz wave that is generated from an n-type InAs under the same conditions. In both POpt-PTHz and SOpt-PTHz configurations, the polarities of the P-polarized THz waveforms from p-type Bi2Te3 (c,d) are in the reverse of that from n-type Cu0.02Bi2Se3 (a,b). ATHz is the peak-to-peak value of the THz waveform. (e–h): the plots of ATHz for the P-polarized THz waveforms as a function of azimuthal angles (
-scan) of Cu0.02Bi2Se3 (a,b) and Bi2Te3 (c,d) single crystals (black). The corresponding XRD
-scans for the (1 1 15) peak for both single crystals are also shown in (e–h) (green).