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Showing 1–2 of 2 results
Advanced filters: Author: Andrea Ruiz-Ferrando Clear advanced filters

  • The restructuring of carbon-based supports under reaction conditions limits catalyst stability for vinyl chloride synthesis. Here, the authors report that hydrogen chloride generates defect sites on carbon nitride supports, promoting acetylene polymerization and accelerating catalyst deactivation.

    • Vera Giulimondi
    • Mikhail Agrachev
    • Javier Pérez-Ramírez
    ResearchOpen Access
    Nature Communications
    Volume: 16, P: 1-12

  • Carbon is a key support for metal-catalyzed acetylene hydrochlorination to vinyl chloride but its role remains elusive. Here, the authors, by means of operando spectroscopy, demonstrate the co-catalytic function of neighboring carbon and isolated metal atoms, constituting the active ensemble.

    • Vera Giulimondi
    • Andrea Ruiz-Ferrando
    • Javier Pérez-Ramírez
    ResearchOpen Access
    Nature Communications
    Volume: 14, P: 1-12