Over the past few decades, two techniques in particular have opened up new avenues for probing molecular processes: ultrafast spectroscopy and single-molecule detection. The two approaches have now been combined, enabling not only the observation but also the manipulation of vibrational wave-packet interference at ambient conditions. The technique could help to unravel details of molecular function and dynamics in systems as diverse as light-harvesting complexes, photoactive proteins and conjugated polymers.
- Daan Brinks
- Fernando D. Stefani
- Niek F. van Hulst
