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Showing 1–4 of 4 results
Advanced filters: Author: Jürgen Senker Clear advanced filters

  • Zirconium-based metal–organic frameworks have defective structures that are useful in catalysis and gas storage. Here, the authors study the interplay between cluster disorder and linker vacancies in PCN-221 and propose a new structure model with tilted Zr6O4(OH)4 clusters rather than Zr8O6 clusters.

    • Charlotte Koschnick
    • Robert Stäglich
    • Bettina V. Lotsch
    ResearchOpen Access
    Nature Communications
    Volume: 12, P: 1-9

  • The applicability of metal-organic frameworks (MOFs) — in spite of their obvious potential — is hindered by stability issues, in particular towards water. Now, a ‘crumple zone’ concept has been proposed in which the presence of sacrificial bonds protects a MOF without significantly altering its structure or functionality.

    • Jürgen Senker
    News & Views
    Nature Chemistry
    Volume: 10, P: 1079-1081

  • Graphitic carbon nitride is a promising hydrogen evolution photocatalyst, although there is limited understanding of its mechanistic operation. Here, the authors employ molecular heptazine-based model catalysts to identify catalytically relevant defects and to rationally design a highly active carbon nitride photocatalyst.

    • Vincent Wing-hei Lau
    • Igor Moudrakovski
    • Bettina V. Lotsch
    ResearchOpen Access
    Nature Communications
    Volume: 7, P: 1-10

  • Spin-ice physics in frustrated magnets is constrained by the energy scale of magnetic interactions, which typically translates to temperatures of a few Kelvin. Here, the authors demonstrate that similar physics can be observed in the system of frustrated electric dipoles in Cd(CN)2 even at room temperature.

    • Chloe S. Coates
    • Mia Baise
    • Andrew L. Goodwin
    ResearchOpen Access
    Nature Communications
    Volume: 12, P: 1-8