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Showing 1–2 of 2 results
Advanced filters: Author: Jiamei Quan Clear advanced filters

  • Electronic spin influences chemistry profoundly, but its role in surface chemistry is poorly established. Now the spin-dependent reaction probabilities of oxygen atoms with a graphite surface have been studied. Molecular dynamics simulations help elucidate the mechanism for spin-flipping, which is observed to occur with low probability in surface scattering experiments.

    • Zibo Zhao
    • Yingqi Wang
    • G. Barratt Park
    ResearchOpen Access
    Nature Chemistry
    Volume: 15, P: 1006-1011

  • Vibrational and translational energies have previously been observed to promote reactions at surfaces occurring via dissociative mechanisms. Now, it has been shown that the reaction of CO2 with surface-adsorbed atomic hydrogen—which occurs via an associative (Eley–Rideal-type) mechanism—can be driven by vibrationally exciting CO2.

    • Jiamei Quan
    • Fahdzi Muttaqien
    • Junji Nakamura
    Research
    Nature Chemistry
    Volume: 11, P: 722-729