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Showing 1–35 of 35 results
Advanced filters: Author: Matthias F. Kling Clear advanced filters
  • Understanding light-matter interaction is important for the control of energy and charge transfer at the fundamental level. Here the authors spatially resolve proton generation in laser-induced dissociative ionization of ethanol and water on SiO2 nanoparticles and discuss the role of surface charge distribution.

    • Philipp Rupp
    • Christian Burger
    • Matthias F. Kling
    ResearchOpen Access
    Nature Communications
    Volume: 10, P: 1-7
  • Ionization delays from ethyl iodide around a giant dipole resonance are measured by attosecond streaking spectroscopy. Using theoretical knowledge of the iodine atom as a reference, the contribution of the functional ethyl group can be obtained.

    • Shubhadeep Biswas
    • Benjamin Förg
    • Matthias F. Kling
    Research
    Nature Physics
    Volume: 16, P: 778-783
  • Strong lasing effects similar to those in the optical regime can occur at 1.5–2.1 Å wavelengths during high-intensity XFEL-driven Kα1 lasing of copper and manganese.

    • Thomas M. Linker
    • Aliaksei Halavanau
    • Uwe Bergmann
    Research
    Nature
    Volume: 642, P: 934-940
  • A continuum spanning from 300 and 3000 nm is used to synthesize a single-cycle field transient and measure its waveform through electro-optic sampling, speeding up this sensitive technique so that it can access the electric field of visible light.

    • Enrico Ridente
    • Mikhail Mamaikin
    • Nicholas Karpowicz
    ResearchOpen Access
    Nature Communications
    Volume: 13, P: 1-7
  • Studying the dynamics of electrons is important for understanding fundamental processes in materials. Here the ionization of a pair of electrons in argon atoms is explored on attosecond timescales, offering insight into their correlated emission and the double ionization mechanism.

    • Boris Bergues
    • Matthias Kübel
    • Matthias F. Kling
    ResearchOpen Access
    Nature Communications
    Volume: 3, P: 1-6
  • Accelerating electrons to high energy and controlling their properties on ultrafast timescales is challenging. Here the authors show controlled acceleration of electron bunches using forward scattering in the resonantly enhanced polarization field of silver clusters driven by a phase-tuned two-color laser field.

    • Johannes Passig
    • Sergey Zherebtsov
    • Thomas Fennel
    ResearchOpen Access
    Nature Communications
    Volume: 8, P: 1-7
  • We introduce strong tailored light-wave-driven time-reversal symmetry breaking in monolayer hexagonal boron nitride, realizing a sub-laser-cycle controllable analogue of the topological model of Haldane and inducing non-resonant valley polarization.

    • Sambit Mitra
    • Álvaro Jiménez-Galán
    • Shubhadeep Biswas
    ResearchOpen Access
    Nature
    Volume: 628, P: 752-757
  • Photoconductive sampling of optical fields is a powerful measurement technique, but existing models fail to connect single-electron dynamics to measured signals. Here, the authors report a model that identifies the roles of electron-neutral scattering and mean-field charge interaction in photoconductive sampling.

    • Johannes Schötz
    • Ancyline Maliakkal
    • Matthias F. Kling
    ResearchOpen Access
    Nature Communications
    Volume: 13, P: 1-10
  • Time-resolved measurements of the X-ray photoemission delay of core-level electrons using attosecond soft X-ray pulses from a free-electron laser can be used to determine the complex correlated dynamics of photoionization.

    • Taran Driver
    • Miles Mountney
    • James P. Cryan
    Research
    Nature
    Volume: 632, P: 762-767
  • Bone marrow-derived cells can rapidly enter the systemic circulation, but how this is achieved is unclear. Grüneboom et al. identify tiny capillaries, termed trans-cortical vessels (TCVs), that connect the bone marrow cavity to the systemic vasculature, and show that the majority of blood in long bones passes through TCVs.

    • Anika Grüneboom
    • Ibrahim Hawwari
    • Matthias Gunzer
    Research
    Nature Metabolism
    Volume: 1, P: 236-250
  • The localized enhancement of laser light in optical near-fields of nanostructures enables the steering of ultrafast electronic motion. Here, the authors employ field propagation in nanospheres to obtain directional tunability and attosecond control of near-field-induced strong-field photoemission.

    • F. Süßmann
    • L. Seiffert
    • T. Fennel
    ResearchOpen Access
    Nature Communications
    Volume: 6, P: 1-9
  • Photoemission from nanometre-scale structures offer a route toward ultrafast light-field-driven electronic nanocircuits. Here, the authors use attosecond streaking spectroscopy for nanoscale characterization of near-fields in the vicinity of tapered gold nanowires.

    • B. Förg
    • J. Schötz
    • M. F. Kling
    ResearchOpen Access
    Nature Communications
    Volume: 7, P: 1-7
  • Researchers use plasmonic nanofocusing of near-infrared pulses in metallic tapered gap waveguides to generate ultrashort extreme-ultraviolet pulses. They calculate that the electromagnetic field intensity is around 350 times higher than that of a reference untapered waveguide, allowing harmonics up to the 43rd to be realized at a modest incident intensity of ∼1011 W cm−2.

    • In-Yong Park
    • Seungchul Kim
    • Seung-Woo Kim
    Research
    Nature Photonics
    Volume: 5, P: 677-681
  • Attosecond streaking is used to study the dynamics of electron scattering in dielectric nanoparticles in real time. Revealing the mechanisms involved is the first step towards understanding electron scattering in more complex dielectrics.

    • L. Seiffert
    • Q. Liu
    • M. F. Kling
    Research
    Nature Physics
    Volume: 13, P: 766-770
  • The H3+ ion plays a key role in interstellar chemistry and can be formed from organic compounds upon interaction with charged particles or radiation. Here the authors demonstrate that H3+ can also be formed from water adsorbed on silica nanoparticles exposed to intense laser pulses, conditions that mimic the impact of charged particles on dust in astrophysical settings.

    • M. Said Alghabra
    • Rami Ali
    • Ali S. Alnaser
    ResearchOpen Access
    Nature Communications
    Volume: 12, P: 1-8
  • A time-resolved observation of electron tunnelling and the short-lived electronic states that subsequently appear is useful as a new approach to obtain insights in multi-electron dynamics inside atoms and molecules. This technique of 'attosecond tunnelling' is applied to study the cascade of electronic transitions that occur in xenon atoms as a result of their ionization.

    • M. Uiberacker
    • Th. Uphues
    • F. Krausz
    Research
    Nature
    Volume: 446, P: 627-632
  • Conical intersections, a hallmark of polyatomic molecules, can be induced with light, leading to new reaction pathways. Here, the authors show that intense fields can create complex, beyond-conical intersections even in diatomics, resulting in an unexpected angular distribution of fragment ions.

    • M. Kübel
    • M. Spanner
    • A. Staudte
    ResearchOpen Access
    Nature Communications
    Volume: 11, P: 1-8
  • Even for simple systems, the interpretations of new attosecond measurements are complicated and provide only a glimpse of their potential. Nonetheless, the lasting impact will be the revelation of how short-time dynamics can determine the electronic properties of more complex systems.

    • Stephen R. Leone
    • C. William McCurdy
    • Marc J. J. Vrakking
    Comments & Opinion
    Nature Photonics
    Volume: 8, P: 162-166
  •   Petahertz electronics uses sub-cycle currents from tailored optical waveforms for high-speed signal processing. This Review discusses progress towards the analogue age of petahertz electronics for optical waveform analysis and communication and provides an outlook toward digital petahertz electronics for classical and quantum computing.

    • Christian Heide
    • Phillip D. Keathley
    • Matthias F. Kling
    Reviews
    Nature Reviews Physics
    Volume: 6, P: 648-662
  • Attosecond technology (1 as = 10−18 S) promises the tools needed to directly probe electron motion in real time. These authors report attosecond pump–probe measurements that track the movement of valence electrons in krypton ions. This first proof-of-principle demonstration uses a simple system, but the expectation is that attosecond transient absorption spectroscopy will ultimately also reveal the elementary electron motions that underlie the properties of molecules and solid-state materials.

    • Eleftherios Goulielmakis
    • Zhi-Heng Loh
    • Ferenc Krausz
    Research
    Nature
    Volume: 466, P: 739-743
  • Advanced X-ray-based, magnetic resonance and optical imaging technologies are capable of visualizing the complex architecture of bone and its blood supply. Clinical and experimental applications of these technologies and novel analytical methods are providing new insights into the structure and function of bone in health and disease.

    • Anika Grüneboom
    • Lasse Kling
    • Matthias Gunzer
    Reviews
    Nature Reviews Rheumatology
    Volume: 15, P: 533-549