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Showing 1–3 of 3 results
Advanced filters: Author: Xiangdi Zeng Clear advanced filters

  • The partial oxidation of CH4 to CH3OH is challenging to perform in artificial systems due to ready over-oxidation to CO and CO2. Here by confining mono-iron hydroxyl sites in a metal–organic framework, photo-oxidation of CH4 to CH3OH is achieved with high selectivity and time yield.

    • Bing An
    • Zhe Li
    • Martin Schröder
    Research
    Nature Materials
    Volume: 21, P: 932-938

  • Porous sorbents capable of high ammonia (NH3) uptake capacities are of great interest for ammonia storage for industry, as well as for the environmental remediation of this toxic and corrosive gas. Here, NH3 adsorption is investigated in four robust aluminium-based metal–organic frameworks, and in situ neutron powder diffraction, synchrotron IR micro-spectroscopy and 27Al solid-state NMR studies show that the pore geometries, framework rigidity, and nature of the host–guest binding sites together dictate the high NH3 capture and storage capacity.

    • Lixia Guo
    • Joseph Hurd
    • Sihai Yang
    ResearchOpen Access
    Communications Chemistry
    Volume: 6, P: 1-9