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Direct observation of magnetic monopole defects in an artificial spin-ice system

Abstract

Free monopoles have fascinated and eluded researchers since their prediction by Dirac1 in 1931. In spin ice, the bulk frustrated magnet, local ordering principles known as ice rules—two-in/two-out for four spins arranged in a tetrahedron—minimize magnetic charge. Remarkably, recent work2,3,4,5 shows that mobile excitations, termed ‘monopole defects’, emerge when the ice rules break down2. Using a cobalt honeycomb nanostructure we study the two-dimensional planar analogue called kagome or artificial spin ice. Here we show direct images of kagome monopole defects and the flow of magnetic charge using magnetic force microscopy. We find the local magnetic charge distribution at each vertex of the honeycomb pins the magnetic charge carriers, and opposite charges hop in opposite directions in an applied field. The parameters that enter the problem of creating and imaging monopole defects can be mapped onto a simple model that requires only the ice-rule violation energy and distribution of switching fields of the individual bars of a cobalt honeycomb lattice. As we demonstrate, it is the exquisite interplay between these energy scales in the cobalt nanostructure that leads to our experimental observations.

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Figure 1: Schematic of magnetic charge order and monopolar defect formation in artificial kagome spin ice.
Figure 2: Characterization of a honeycomb array.
Figure 3: The creation of monopole defects.
Figure 4: The movement of magnetic charge.
Figure 5: Simulation of data with a model of the normal distribution of bar coercive fields (HC: mean HC=60 mT,σ=10 mT) plus a tunable ice-rule modification to the coercive field (HI).

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Acknowledgements

This work was financially supported under grants from the EPSRC (EP/G004765/1) (W.R.B.) and the Leverhulme Trust (F/07058/AW) (L.F.C.).

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W.R.B. and L.F.C. are jointly responsible for all aspects of the work. S.L. carried out the MFM imaging and analysis and contributed to the preparation of the manuscript. D.E.R grew and processed the films and contributed to discussions. G.K.P. carried out the simulations.

Corresponding author

Correspondence to W. R. Branford.

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The authors declare no competing financial interests.

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Ladak, S., Read, D., Perkins, G. et al. Direct observation of magnetic monopole defects in an artificial spin-ice system. Nature Phys 6, 359–363 (2010). https://doi.org/10.1038/nphys1628

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