Abstract
The quantum spin Hall effect is characterized by spin-polarized counter-propagating edge states1,2,3. It has been predicted that this edge state configuration could occur in graphene when spin-split electron- and hole-like Landau levels are forced to cross at the edge of the sample4,5,6. In particular, a quantum-spin-Hall analogue has been predicted in bilayer graphene with a Landau level filling factor ν = 0 if the ground state is a spin ferromagnet7. Previous studies have demonstrated that the bilayer ν = 0 state is an insulator in a perpendicular magnetic field8,9,10,11,12,13,14, although the exact nature of this state has not been identified. Here we present measurements of the ν = 0 state in a dual-gated bilayer graphene device in a tilted magnetic field. We map out a full phase diagram of the ν = 0 state as a function of experimentally tunable in-plane magnetic field and perpendicular electric field. At large in-plane magnetic field we observe a quantum phase transition to a metallic state with conductance of the order of 4e2/h, consistent with predictions for the ferromagnet.
This is a preview of subscription content, access via your institution
Access options
Subscribe to this journal
Receive 12 print issues and online access
$259.00 per year
only $21.58 per issue
Buy this article
- Purchase on SpringerLink
- Instant access to the full article PDF.
USD 39.95
Prices may be subject to local taxes which are calculated during checkout




Similar content being viewed by others
References
Kane, C. L. & Mele, E. J. Z2 topological order and the quantum spin Hall effect. Phys. Rev. Lett. 95, 146802 (2005).
Bernevig, B. A., Hughes, T. L. & Zhang, S-C. Quantum spin Hall effect and topological phase transition in HgTe quantum wells. Science 314, 1757–1761 (2006).
König, M. et al. Quantum spin Hall insulator state in HgTe quantum wells. Science 318, 766–770 (2007).
Abanin, D. A., Lee, P. A. & Levitov, L. S. Spin-filtered edge states and quantum Hall effect in graphene. Phys. Rev. Lett. 96, 176803 (2006).
Fertig, H. A. & Brey, L. Luttinger liquid at the edge of undoped graphene in a strong magnetic field. Phys. Rev. Lett. 97, 116805 (2006).
Kharitonov, M. Edge excitations of the canted antiferromagnetic phase of the ν = 0 quantum Hall state in graphene: A simplified analysis. Phys. Rev. B 86, 075450 (2012).
Kharitonov, M. Canted antiferromagnetic phase of the ν = 0 quantum Hall state in bilayer graphene. Phys. Rev. Lett. 109, 046803 (2012).
Feldman, B. E., Martin, J. & Yacoby, A. Broken-symmetry states and divergent resistance in suspended bilayer graphene. Nature Phys. 5, 889–893 (2009).
Zhao, Y., Cadden-Zimansky, P., Jiang, Z. & Kim, P. Symmetry breaking in the zero-energy Landau level in bilayer graphene. Phys. Rev. Lett. 104, 066801 (2010).
Weitz, R. T., Allen, M. T., Feldman, B. E., Martin, J. & Yacoby, A. Broken-symmetry states in doubly gated suspended bilayer graphene. Science 330, 812–816 (2010).
Kim, S., Lee, K. & Tutuc, E. Spin-polarized to valley-polarized transition in graphene bilayers at ν = 0 in high magnetic fields. Phys. Rev. Lett. 107, 016803 (2011).
Velasco, J. Jr et al. Transport spectroscopy of symmetry-broken insulating states in bilayer graphene. Nature Nanotech. 7, 156–160 (2012).
Veligura, A. et al. Transport gap in suspended bilayer graphene at zero magnetic field. Phys. Rev. B 85, 155412 (2012).
Freitag, F., Trbovic, J., Weiss, M. & Schenberger, C. Spontaneously gapped ground state in suspended bilayer graphene. Phys. Rev. Lett. 108, 076602 (2012).
Gorbar, E. V., Gusynin, V. P. & Miransky, V. A. Dynamics and phase diagram of the ν = 0 quantum Hall state in bilayer graphene. Phys. Rev. B 81, 155451 (2010).
Lemonik, Y., Aleiner, I. L. & Falko, V. I. Competing nematic, antiferromagnetic, and spin-flux orders in the ground state of bilayer graphene. Phys. Rev. B 85, 245451 (2012).
Kharitonov, M. Antiferromagnetic state in bilayer graphene. Phys. Rev. B 86, 195435 (2012).
Zhang, F. & MacDonald, A. H. Distinguishing spontaneous quantum Hall states in bilayer graphene. Phys. Rev. Lett. 108, 186804 (2012).
Lemonik, Y., Aleiner, I. L., Toke, C. & Falko, V. I. Spontaneous symmetry breaking and Lifshitz transition in bilayer graphene. Phys. Rev. B 82, 201408 (2010).
Vafek, O. & Yang, K. Many-body instability of Coulomb interacting bilayer graphene: Renormalization group approach. Phys. Rev. B 81, 041401 (2010).
Nandkishore, R. & Levitov, L. Quantum anomalous Hall state in bilayer graphene. Phys. Rev. B 82, 115124 (2010).
Castro, E. V., Peres, N. M. R., Stauber, T. & Silva, N. A. P. Low-density ferromagnetism in biased bilayer graphene. Phys. Rev. Lett. 100, 186803 (2008).
Mayorov, A. S. et al. Interaction-driven spectrum reconstruction in bilayer graphene. Science 333, 860–863 (2011).
McCann, E. & Falko, V. I. Landau-level degeneracy and quantum Hall effect in a graphite bilayer. Phys. Rev. Lett. 96, 086805 (2006).
Barlas, Y., Ct, R., Nomura, K. & MacDonald, A. H. Intra-Landau-level cyclotron resonance in bilayer graphene. Phys. Rev. Lett. 101, 097601 (2008).
Das Sarma, S., Sachdev, S. & Zheng, L. Double-layer quantum Hall antiferromagnetism at filling fraction ν = 2/m where m is an odd integer. Phys. Rev. Lett. 79, 917–920 (1997).
Pellegrini, V. et al. Evidence of soft-mode quantum phase transitions in electron double layers. Science 281, 799–802 (1998).
Grivei, E., Melinte, S., Bayot, V., Manoharan, H. C. & Shayegan, M. Multiple interacting bilayer electron system: Magnetotransport and heat capacity measurements. Phys. Rev. B 68, 193404 (2003).
Taychatanapat, T. & Jarillo-Herrero, P. Electronic transport in dual-gated bilayer graphene at large displacement fields. Phys. Rev. Lett. 105, 166601 (2010).
Roth, A. et al. Nonlocal transport in the quantum spin Hall state. Science 325, 294–297 (2009).
Dean, C. R. et al. Boron nitride substrates for high-quality graphene electronics. Nature Nanotech. 5, 722–726 (2010).
Acknowledgements
The authors thank M. Kharitonov for useful discussions. Portions of this experiment were conducted at the National High Magnetic Field Laboratory, which is supported by National Science Foundation Cooperative Agreement No. DMR-0654118, the State of Florida and the US Department of Energy. We thank S. Hannahs, T. Murphy and A. Suslov for experimental assistance at NHMFL. This work is supported by AFOSR MURI. P.M. acknowledges support from ONR MURI and FENA. A.F.Y. and P.K. acknowledge support from DOE (DE-FG02-05ER46215) for carrying out experiments and INDEX for sample fabrication.
Author information
Authors and Affiliations
Contributions
P.M., C.R.D. and A.F.Y. designed and conceived the experiment. T.T. and K.W. synthesized hBN samples, P.M. fabricated the samples. P.M., C.R.D. and A.F.Y. performed the measurements. P.M., C.R.D. and P.K. analysed the data and wrote the paper. J.H., K.L.S. and P.K. advised on experiments.
Corresponding author
Ethics declarations
Competing interests
The authors declare no competing financial interests.
Supplementary information
Supplementary Information
Supplementary Information (PDF 509 kb)
Rights and permissions
About this article
Cite this article
Maher, P., Dean, C., Young, A. et al. Evidence for a spin phase transition at charge neutrality in bilayer graphene. Nature Phys 9, 154–158 (2013). https://doi.org/10.1038/nphys2528
Received:
Accepted:
Published:
Issue date:
DOI: https://doi.org/10.1038/nphys2528
This article is cited by
-
Interacting multi-channel topological boundary modes in a quantum Hall valley system
Nature (2019)
-
Ferroelectric quantum Hall phase revealed by visualizing Landau level wavefunction interference
Nature Physics (2018)
-
Direct measurement of discrete valley and orbital quantum numbers in bilayer graphene
Nature Communications (2017)
-
Helical edge states and fractional quantum Hall effect in a graphene electron–hole bilayer
Nature Nanotechnology (2017)
-
Landau quantization of Dirac fermions in graphene and its multilayers
Frontiers of Physics (2017)


