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Evolution of the pseudogap from Fermi arcs to the nodal liquid

Abstract

The response of a material to external stimuli depends on its low-energy excitations. In conventional metals, these excitations are electrons on the Fermi surface—a contour in momentum (k) space that encloses all of the occupied states for non-interacting electrons. The pseudogap phase in the copper oxide superconductors, however, is a most unusual state of matter1. It is metallic, but part of its Fermi surface is ‘gapped out’ (refs 2, 3); low-energy electronic excitations occupy disconnected segments known as Fermi arcs4. Two main interpretations of its origin have been proposed: either the pseudogap is a precursor to superconductivity5, or it arises from another order competing with superconductivity6. Using angle-resolved photoemission spectroscopy, we show that the anisotropy of the pseudogap in k-space and the resulting arcs depend only on the ratio T/T*(x), where T*(x) is the temperature below which the pseudogap first develops at a given hole doping x. The arcs collapse linearly with T/T*(x) and extrapolate to zero extent as T→0. This suggests that the T=0 pseudogap state is a nodal liquid—a strange metallic state whose gapless excitations exist only at points in k-space, just as in a d-wave superconducting state.

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Figure 1: Symmetrized EDCs for underdoped samples along the Fermi surface.
Figure 2: Intensity maps at the Fermi energy for an underdoped Tc=70 K sample.
Figure 3: Gap size (normalized to its value at the antinode) as a function of Fermi surface angle (defined in Fig. 1e) for two particular reduced temperatures.
Figure 4: Loss of low-energy spectral weight L(φ) and scaling of arc lengths with T/T *.

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Acknowledgements

This work was supported by NSF DMR-0305253, the US DOE, Office of Science, under Contract Nos W-31-109-ENG-38 (ANL) and W-7405-Eng-82 (Ames), and the MEXT of Japan. The Synchrotron Radiation Center is supported by NSF DMR-0084402.

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Correspondence to J. C. Campuzano.

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Kanigel, A., Norman, M., Randeria, M. et al. Evolution of the pseudogap from Fermi arcs to the nodal liquid. Nature Phys 2, 447–451 (2006). https://doi.org/10.1038/nphys334

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