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Low-temperature vortex liquid in La2−xSrxCuO4

Abstract

In copper oxide superconductors, the lightly doped (small dopant concentration, x) region is of major interest1,2 because superconductivity, antiferromagnetism and the pseudogap state come together near a critical doping value, xc. But the way in which superconductivity is destroyed as x is decreased at very low temperatures, T, is not clear3,4,5,6,7. Does the pair condensate vanish abruptly at a critical value, xc? Or is phase coherence of the condensate destroyed by spontaneous vortices—as is the case at elevated T (refs 8, 9, 10)? So far, magnetization data at low T are very sparse in this region of the phase diagram. Here, we report torque magnetometry measurements on La2−xSrxCuO4, which show that, in zero magnetic field, quantum phase fluctuations destroy superconductivity at xc≈0.055. The phase-disordered condensate survives to x=0.03. In finite field H, the vortex solid-to-liquid transition occurs at H lower than the depairing field, Hc2. The resulting phase diagram reveals the large fraction of the xH plane occupied by the quantum vortex liquid.

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Figure 1: Magnetization curves in lightly doped LSCO.
Figure 2: Separation of magnetization into the spin term, ΔMs(T,H), and the diamagnetic term, Md(T,H).
Figure 3: The hysteresis curves and irreversibility field Hirr(T) in the vortex-solid phase.
Figure 4: The phase diagram of LSCO in the xH plane at low temperatures.

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References

  1. Lee, P. A., Nagaosa, N. & Wen, X. G. Doping a Mott insulator: Physics of high-temperature superconductivity. Rev. Mod. Phys. 78, 17–85 (2006).

    Article  ADS  Google Scholar 

  2. Anderson, P. W. Present status of the theory of the high-Tc cuprates. Low Temp. Phys. 32, 282–289 (2006).

    Article  ADS  Google Scholar 

  3. Doniach, S. Quantum fluctuations in two-dimensional superconductors. Phys. Rev. B 24, 5063–5070 (1981).

    Article  ADS  Google Scholar 

  4. Fisher, M. P. A., Weichman, P. B., Grinstein, G. & Fisher, D. S. Boson localization and the superfluid-insulator transition. Phys. Rev. B 40, 546–570 (1989).

    Article  ADS  Google Scholar 

  5. Fisher, M. P. A. & Lee, D. H. Correspondence between two-dimensional bosons and a bulk superconductor in a magnetic field. Phys. Rev. B 39, 2756–2759 (1989).

    Article  ADS  Google Scholar 

  6. Melikyan, A. & Tešanović, Z. A model of phase fluctuations in a lattice d-wave superconductor: application to the Cooper pair charge-density-wave in underdoped cuprates. Phys. Rev. B 71, 214511 (2005).

    Article  ADS  Google Scholar 

  7. Nikolic, P. & Sachdev, S. Effective action for vortex dynamics in clean d-wave superconductors. Phys. Rev. B 73, 134511 (2006).

    Article  ADS  Google Scholar 

  8. Emery, V. J. & Kivelson, S. A. Importance of phase fluctuations in superconductors with small superfluid density. Nature 374, 434–437 (1995).

    Article  ADS  Google Scholar 

  9. Wang, Y. et al. The onset of the vortex-like Nernst signal above Tc in La2−xSrxCuO4 and Bi2Sr2−yLayCuO6 . Phys. Rev. B 64, 224519 (2001).

    Article  ADS  Google Scholar 

  10. Wang, Y., Li, L. & Ong, N. P. Nernst effect in high-Tc superconductors. Phys. Rev. B 73, 024510 (2006).

    Article  ADS  Google Scholar 

  11. Keimer, B. et al. Magnetic excitations in pure, lightly doped, and weakly metallic La2CuO4 . Phys. Rev. B 46, 14034–14053 (1992).

    Article  ADS  Google Scholar 

  12. Niedermayer, Ch. et al. Common phase diagram for antiferromagnetism in La2−xSrxCuO4 and Y1−xCaxBa2CuO6 as seen by muon spin rotation. Phys. Rev. Lett. 80, 3843–3846 (1998).

    Article  ADS  Google Scholar 

  13. Lavrov, A. N., Ando, Y., Komiya, S. & Tsukada, I. Unusual magnetic susceptibility anisotropy in untwinned La2−xSrxCuO4 single crystals in the lightly doped region. Phys. Rev. Lett. 87, 017007 (2001).

    Article  ADS  Google Scholar 

  14. Wang, Y. et al. Field-enhanced diamagnetism in the pseudogap state of the cuprate Bi2Sr2CaCu2O8+δ superconductor in an intense magnetic field. Phys. Rev. Lett. 95, 247002 (2005).

    Article  ADS  Google Scholar 

  15. Li, L. et al. Strongly nonlinear magnetization above Tc in Bi2Sr2CaCu2O8+δ . Europhys. Lett. 72, 451–457 (2005).

    Article  ADS  Google Scholar 

  16. Farrell, D. E. et al. Experimental evidence for a transverse magnetization of the Abrikosov lattice in anisotropic superconductors. Phys. Rev. Lett. 61, 2805–2808 (1988).

    Article  ADS  Google Scholar 

  17. Bergemann, C. et al. Superconducting magnetization above the irreversibility line in Tl2Ba2CuO6+δ . Phys. Rev. B 57, 14387–14396 (1998).

    Article  ADS  Google Scholar 

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Acknowledgements

Valuable discussions with Y. Wang, Z. Tešanović, S. Sachdev, S. A. Kivelson, P. W. Anderson and J. C. Davis are acknowledged. The research at Princeton was supported by the National Science Foundation (NSF) through an MRSEC grant DMR 0213706. Research at CRIEPI was supported by a Grant-in-Aid for Science from the Japan Society for the Promotion of Science. The high-field measurements were carried out in the National High Magnetic Field Laboratory, Tallahassee, which is supported by NSF, the Department of Energy and the State of Florida.

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Correspondence to Lu Li or N. P. Ong.

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Li, L., Checkelsky, J., Komiya, S. et al. Low-temperature vortex liquid in La2−xSrxCuO4. Nature Phys 3, 311–314 (2007). https://doi.org/10.1038/nphys563

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