Introduction

The Rio Grande Rise (RGR) is an oceanic plateau located in the southwest Atlantic Ocean on the South American plate (Fig. 1a). Its large spatial extent and volume1 has led some to consider it a large igneous province (LIP)1,2,3, implying a rapid formation based on the common definition of a LIP4. However, its formation history remains poorly constrained due to little available geochronology, leaving its geodynamic origin uncertain.

Fig. 1: Bathymetric maps of the South Atlantic and Rio Grande rise.
figure 1

a Bathymetric map of the South Atlantic Ocean. The continental surface expressions of the Paraná and Etendeka LIPs are outlined in red, filled gray. The Mid-Atlantic Ridge (MAR) is denoted by the center black dashed line and the Vema Trough (thought to be an extinct spreading center2) is marked by a dashed line west of RGR. The two arrows in WR indicate the two geochemical subtracks of the WR Guyot Province18,19, with Tristan to the north and Gough to the south. Labeled yellow stars indicate the approximate locations of currently active hotspots. b Close-up bathymetric map of RGR with labeled dredge and drill (DSDP Hole 516 F) locations (diamonds and circle, respectively) and ages (in Ma). Red diamonds are dredge locations from cruise NBP1808 (this study) while three gray locations are from other campaigns that also produced ages7,10,12. Eruption ages are shown in black font, eruption age estimations in grey, minimum eruption ages in blue, maximum eruption ages in red. All uncertainties are 2σ standard errors, stacked uncertainties are 97.5% (top) and 2.5% (bottom) confidence intervals using weighted kernel density estimations (WKDE). Dashed outlines show our distinction of sub-provinces: West (W-RGR), Northeast (NE-RGR), and Southeast RGR (SE-RGR) as individual sub-regions that are roughly separated by the Centaurus Basin (CB, hatched pattern). The Cruzeiro do Sul Rift (lined pattern) incises both W- and SE-RGR. Maps were created in GMT70 and use GEBCO bathymetry71.

RGR is considered the conjugate of the older Walvis Ridge (WR), with both thought to have formed together at the Mid-Atlantic Ridge (MAR) axis sometime in the Cretaceous2,5,6,7. Both RGR and WR are thought to be expressions of the same Tristan-Gough (T-G) hotspot, attributed to a mantle plume currently active below Tristan da Cunha and Gough islands on the African Plate8. Recent studies on samples from the southeast RGR support this connection by showing geochemical similarities to WR and the T-G hotspot3,9.

Despite their supposed shared origin, RGR and WR differ greatly in their morphology: RGR forms a broad feature, whereas WR is continuous and comparatively narrow, and extends westward as younger seamounts of the WR Guyot Province on the African plate, which have no conjugate on the South American plate. These differences imply different expressions of the T-G hotspot on either side of the MAR, the underlying geodynamic processes of which remain unclear.

RGR has a complex structure that includes several massifs, tectonic basins, and rift zones (Fig. 1b). Deep Sea Drilling Project (DSDP) Hole 516F cored into the basement of the W(est)-RGR producing 40Ar/39Ar ages from 82.0 ± 0.5 to 86.0 ± 4.0 Ma7,10,11. Eocene age volcaniclastic sediments were also recovered from DSDP Hole 516F11. This late stage Eocene volcanism is also found in 46 Ma alkaline lavas dredged from sites along the Cruzeiro do Sul Rift7,12 which is a large rift valley of unknown origin trending NW-SE that dissects both the W- and SE-RGR (Fig. 1). These initial sparse age data suggest that RGR could have had a prolonged eruptive history with multiple periods of construction, similar to other oceanic plateaus13,14,15 and oceanic mid-plate superstructures16.

The WR is also complex and includes several sub-regions, each with their own unique characteristics. The oldest portion, nearest the African continent, is the E-W trending Frio Ridge which formed around 115 Ma7 (Fig. 1a). This transitions into the N-S trending Valdivia Bank (VB) which is thought to be the conjugate of W-RGR, forming together at the MAR between ~90 and 80 Ma2,6,7. Around 29 °S WR changes from a relatively continuous bathymetric high into a ~ 400 km wide region of seamounts—called the Guyot Province—that trend southwest towards the modern MAR. The WR Guyot Province contains two isotopically distinct and age progressive seamount trails, the Tristan Track and Gough Track7,17,18,19,20,21. Although the Gough Track can be traced back to the earliest stages of the WR, the Tristan Track does not emerge until the WR splits into the Guyot Province at about 70 Ma18,19, which is when the T-G hotspot is thought to have become intraplate under the African plate only. Recent isotopic data show that the Jean Charcot Seamounts and parts of RGR have Tristan affinities that extend back perhaps to ~100 Ma on the South American Plate, suggesting that Tristan and Gough are both long-lived plume components9.

Several aspects of the RGR-WR system make it an important case study for hotspots and large igneous provinces (LIPs). The T-G plume system is one of only a few hotspots with a continuous record of volcanism from the present back to the proposed inception of volcanism in the form of a LIP22. It is also notable in that the plume appears to have produced multiple episodes of high-volume volcanism: the Paraná-Etendeka Flood Basalts (135–132 Ma23,24), and RGR and VB ( ~ 90–80 Ma7,10,11,21). Because the size of RGR is similar to the Paraná and other LIPs, some have speculated that RGR may also result from high-flux, LIP volcanism. Importantly however, the LIP nature of RGR has so far been unclear due to a lack of geochronological evidence. In addition, the T-G plume system seems to have been located at or near the MAR axis for a long period with influence on this spreading ridge and the South Atlantic asthenosphere9,25,26,27,28. Both the RGR and WR also have experienced late-stage Eocene off-axis volcanism that cannot be attributed to the T-G plume system.

Understanding the combined geochemical and geochronological history of RGR therefore is critical in advancing our knowledge on the geodynamics of the overall T-G plume system, its influence on the geochemical makeup of South Atlantic asthenosphere, and its relationship with the opening of the South Atlantic basin. While WR has received considerable attention with numerous sampling campaigns, RGR was sparsely sampled until recently, and first-order questions about its emplacement history remain unanswered3,9,29,30. This paper presents a broad geochronologic history of RGR, examines its relationship to WR, and evaluates the role of the T-G plume in its creation.

Results

Thirty-nine analyses from 36 individual samples in 19 dredge locations were dated by incremental step heating 40Ar/39Ar analysis31. A summary of the results can be found in Table 1 with more detailed results in Supplementary Notes 1 and 2. Many samples show non-ideal degassing behavior due to the difficulties of dating old, very low-K, submarine LIP basalts32 and some degree of alteration (Supplementary Note 3). The increased resolution from ARGUS-VI mass spectrometers equipped with 1013 Ω resistors measuring 39Ar, 38Ar and 37Ar, an electron multiplier measuring 36Ar, and only the large 40Ar signal being measured by a 1012 Ω resistor, resulted in highly precise measurements for each step, despite low K content for most samples. This high precision combined with some amount of (likely) alteration resulted in many samples showing scatter among consecutive steps, and therefore high calculated MSWD values. High MSWD values themselves do not rule out these samples from being considered reliable age plateaus33, but the highly precise individual steps do result in calculated weighted mean age uncertainties that are unrealistically small given the amount of scatter among individual step ages (Fig. 2b). Another way of quantifying their uncertainty must be used.

Fig. 2: Example 40Ar/39Ar age spectra, weighted kernel density estimations (WKDEs), and inverse isochrons.
figure 2

a NBP1808-D26-27 is a sample where the traditional age plateau is preferred and (b) NBP1808-D06-18 is a sample where the WKDE is preferred, an example of an experiment that has increased scatter resulting in a high MSWD ( > 50, and much higher than the MSWDmax = 1.78) and an unrealistically low weighted mean age plateau uncertainty of ± 0.83 Ma (2σ standard error). The WKDE 2.5% and 97.5% confidence intervals (blue dotted lines) do a better job of capturing this sample’s uncertainty ( + 3.49, −4.40 Ma), and all the individual steps fall inside this range. The magenta line denotes the ArArCALC weighted mean age and its height the weighted mean plateau age 2σ standard error.

Table 1 Summary of ages

We use a tiered system to decide which age and associated uncertainty is best for a given experiment. The first (and default) tier is the standard weighted mean plateau age and 2σ standard error (e.g., Fig 2a). If a sample’s plateau age MSWD is higher than the MSWD 2σ confidence interval, the next tier is the inverse isochron age and 2σ standard error. If a sample’s inverse isochron MSWD is also higher than its MSWD 2σ confidence interval, then the final tier is a weighted kernel density estimation (WKDE) and 2.5% and 97.5% confidence intervals (a 95% confidence envelope) are used for the uncertainty. Here the MSWD 2σ confidence interval (or MSWDmax) is defined as the maximum MSWD expected given the number of data, given by the expression:

$${{MSWD}}_{\max }=1+2\,\times \,{(2/n-2)}^{1/2}$$
(1)

where \(n\) corresponds to the number of steps in the age plateau or inverse isochron34,35. An MSWD > MSWDmax means that the amount of scatter among the steps is greater than what can be expected given the analytical uncertainties of individual steps with 95% confidence34. Increasing numbers of steps in an age plateau or isochron decreases this MSWDmax towards a value of 1. Increasing the analytical resolution of individual steps tends to cause MSWD values to increase. In modern high-resolution mass spectrometry we are typically increasing the number of steps in experiments while decreasing analytical uncertainties, which taken together are resulting in MSWD and MSWDmax values diverging in opposite directions. This is in part why many of our measured sample MSWDs fall outside their MSWDmax limit.

WKDEs are generated assuming a Gaussian age distribution for each individual step and weighing each step by the amount of 39Ar(K) released (i.e., the step size, calculated as a percentage of the total amount released in the entire experiment). This results in age density distributions that allow us to calculate the 2.5% and 97.5% confidence intervals (encompassing a 95% confidence envelope) as an estimation of the uncertainty for each age, and the median is used for the age estimation itself. Our WKDEs are generally less precise but appear to better capture the actual uncertainty in analyses with moderate to considerable scatter (e.g., Fig 2b). Importantly, all the WKDE median ages are within the 2σ standard error of the calculated standard weighted mean plateau age (supplementary Table 1), but the only thing that changes to any considerable degree is the associated uncertainty of the age. WKDE uncertainties are on average about 3.5X larger than the standard weighted mean age uncertainty. Despite this increase, the 2σ uncertainties of individual WKDEs are still about ± 3% (average) and as little as 0.1% (in a few samples). This is more than sufficient to address geodynamic questions about RGR’s formation.

Analyses from 36 samples sourced from 16 dredge locations yielded 10 eruption ages, eight eruption age estimations, six minimum eruption age estimations, one maximum eruption age estimation, and 10 samples did not yield a reliable age. An additional sample (NBP1808-D11-01) yields an age plateau from a glass analysis, but this likely contains excess 40Ar, and is therefore an overestimation of the age, and is not further considered in the discussion (Supplementary Note 4). NBP1808-D31-06 is considered a maximum age because it displays a slight stepwise decrease in age from low to high-T steps. Minimum ages are often interpreted as minimums due to evidence of 40Ar* loss in low-T steps and slight saddle shapes (see Supplementary Note 7 for age spectra), evidence of sericitization36. Altogether, our ages for RGR range from 83.6 to 41.3 Ma.

Several dredges recovered samples that span a large variation in age (e.g., dredges NBP1808-D7, -D9, -D12, and -D21). These dredged locations with high escarpments along the periphery of the sub-plateaus, or in the case of NBP1808-D21 from the deeply incised Cruzeiro do Sul Rift. These all dredged between 850 and 1650 m of vertical stratigraphy with deep starting depths between 4050 and 5250 m. Samples from these locations contain a variety of textures and mineralogy (see Supplementary Note 5 for detailed petrography) indicating that they come from different volcanic events. This, along with their variations in age shows that these locations were erupted over a prolonged period, encompassing multiple eruptive events that record a prolonged emplacement history. The longest duration of volcanism was sampled at NBP1808-D9, where volcanism spans over 20 Myr from initial eruptions at 78.5 Ma to as late as 57.8 Ma.

In the geographical age distribution, it is notable that W-RGR ages span the entire age range and include a distinctly younger group of Eocene ages (51.9–41.3 Ma) that all come from dredges along the Cruzeiro do Sul rift (Fig. 1b). However, when excluding these Eocene ages, the W-RGR is the oldest portion of RGR ranging from 83.6 to 64.4 Ma. The NE-RGR and SE-RGR also have wide age ranges, but somewhat younger, ranging from 79.7 to 50.6 Ma and 71.8 to 52.0 Ma, respectively. Therefore, all three sub-regions have overlapping eruptive histories, indicating that RGR as a whole has an emplacement history that spans >30 Myrs.

Discussion

Prolonged emplacement of Rio Grande Rise with Walvis Ridge

RGR has long been assumed to be a LIP due to its large size and the volume of lava produced1. Our new ages demonstrate that RGR was emplaced over a prolonged period in stark contrast to the conventional understanding that LIPs are rapidly emplaced features4. As a result of more detailed geochronology studies, prolonged emplacement of oceanic LIPs is increasingly observed. This includes the largest oceanic LIPs: Ontong Java and Kerguelen, which are also the best sampled, and both have emplacement timescales >5 Myrs and Kerguelen perhaps up to 30 Myrs14,37. In contrast, terrestrial LIPs such as the Deccan, Paraná and Siberian Traps were largely emplaced in <1 Myr38,39,40.

Despite the many new dates for RGR in this study and the large age database that exists for WR, the earliest stages of emplacement remain unclear. Our ages from NBP1808-D01 (83.6 & 81.9 Ma) are similar to the oldest ages from DSDP Hole 516F in W-RGR and those from the southeast VB in WR7,21, but these ages are few and come from large volcanic features. In addition, DSDP Hole 516F is located near the center of W-RGR and the penetration is shallow, so it does not capture the earliest phases of volcanism. Given the broad range of ages that exists between DSDP Hole 516F and our other two locations in W-RGR (85.9–64.4 Ma), an earlier phase may exist and could extend the emplacement of W-RGR further back in time. The initial emplacement of W-RGR and VB likely coincided with an eastward ridge jump that left the Vema Trough, an abandoned spreading center, on the South American Plate (Fig. 1a) around the end of the Cretaceous Quiet Period2,41. The younger Eocene ages (51.9–41.3 Ma) from three locations in W-RGR must be part of a distinct, late stage eruptive event7,12 based on the different composition of samples compared to the older locations. Our ages indicate that this Eocene event was more widespread and occurred over a longer period—at least 10 Myrs—than previously known (see further discussion below).

Our spatio-temporal resolution is higher for the emplacement of NE-RGR and SE-RGR (21 ages from 11 locations) compared to W-RGR. W-RGR and VB appear to be conjugate features given their similar ages, but this implies that NE-RGR does not have a conjugate feature on the African Plate. Current plate reconstructions place the MAR within NE-RGR and increasingly further away from VB between 75 and 65 Ma (Fig. 3), which would require an asymmetric accretion of overthickened crust on the South American plate, but normal crust on the African plate, a configuration contradicted by a typical symmetric overthickening of crust for active ridge-centered plumes (e.g., Iceland). This discrepancy could be solved by the presence of a temporary microplate that was later incorporated into the South American plate2,42, a scenario that is not yet incorporated into available plate reconstruction models of the South Atlantic41,43. Four locations in the NE-RGR produced ages between 80 and 75 Ma and, of these, the oldest three samples are located 180-230 km away from each other, indicating they could have erupted on conjugate spreading centers that form the edges of this microplate (Fig. 3). In this scenario, an eastward ridge jump likely incorporated the microplate (and the entire NE-RGR) into the South American plate by Chron C32n.1n (71.4 Ma)44 and regular spreading resumed afterwards (as shown in Fig. 3 in the 65 Ma panel).

Fig. 3: Plate tectonic reconstructions of the South Atlantic from 85 to 45 Ma.
figure 3

Reconstructions were made in GPlates72 using the rotation parameters of Zahirovic et al.73 and plotted in GMT70. Each dated panel shows the locations of dated samples from RGR (this study) and WR6,7,10,11,20,21. Symbol color denotes timing of volcanism relative to reconstruction age. Active volcanism (within 5 Myrs of the reconstruction time) is shown by red symbols, recently active (within 5-10 Myrs) by orange symbols, and inactive ( > 10 Myrs) by black symbols. The hatched region indicates the approximate area of a proposed microplate2 now incorporated into the South American plate. The red line is the paleo-MAR, white lines are fracture zones including PFZ Peleg Fracture Zone, RFZ Rachel Fracture Zone, and dashed black lines are isochrons (labeled in the 45 Ma plot with chron numbers and ages in Ma) from Seton et al.43.

The SE-RGR is the conjugate to the WR segment where it bifurcates into the discontinuous Guyot Province (Fig. 3). This is an important region as it corresponds to the emergence of the Tristan sub-track on the African Plate near the 29°S WR bifurcation point (Fig. 1A). It is suggested that this bifurcation occurred when the T-G plume transitioned from being ridge-centered to intraplate on the African Plate only at ~70 Ma18,19. Our ages from SE-RGR extend as young as 52 Ma and imply that this did not occur for at least another 10 Myrs. After 52 Ma, volcanism occurred only on the African plate (Fig. 3, 45 Ma), producing the WR Guyot Province7,18,19,20,26 and volcanism ceased on the South American plate, except for the further afield Eocene volcanism in the W-RGR.

Late-stage Eocene volcanism

Three dredge sites (NBP1808-D28, -D30 and -D31) located along the Cruzeiro do Sul Rift in the W-RGR yielded Eocene ages ranging from 51.9 to 41.3 Ma. Two of these sites are located near DSDP Site 516 and two dredge sites (RC11-2RD and RGR1-D08; Fig. 1B) previously provided evidence of Eocene volcanism7,12. Most samples dredged from throughout RGR are plagioclase or olivine-phyric, or aphyric tholeiitic basalts, which are indicative of high degrees of partial melting. Our Eocene samples come from alkalic rock types, some of which include biotite phenocrysts, further indicating the difference between these samples and the older main-phase samples from the W-RGR. This compositional difference indicates that these young ages are not younger alteration ages, but in fact a separate, later and lower-degree (and deeper) melting event. NBP1808-D30 and -D31 are located northwest in the W-RGR and along its crest, providing further evidence of late-stage volcanism in the region near previously dated examples7,12. NBP1808-D28 is located southeast in the W-RGR, and extends the known region of this late-stage event to almost the full ~300 km length of the Cruzeiro do Sul Rift in the W-RGR. This shows that Eocene volcanism was more geographically widespread than previously known, possibly over the whole W-RGR and indicating that this likely was a major rejuvenated magmatic event.

The Eocene volcanism in the W-RGR could be related to the nearby Jean-Charcot Seamounts that bisect a portion of the W-RGR and that are geochemically similar3. Eocene volcanism is somewhat age-progressive (Fig. 4) and co-parallel with the (scattered) age progression of RGR itself. The direction of the Jean-Charcot Seamounts is also co-parallel to the overall trend of volcanism on the South American plate, which is generally progressing towards the southeast. No ages are currently available from the Jean-Charcot Seamounts, but it is possible that the Eocene volcanism that is capping the older eruptive portion of the W-RGR is a younger extension of the Jean-Charcot Seamount volcanism, creating a co-parallel set of age-progressive volcanism. This is in contrast to the model of Homrighausen et al.9, who suggested they are older ( ~ 100–80 Ma) based on their guyot-like structures and predicted crustal subsidence models. They suggested that the Jean-Charcot Seamounts are therefore related to the main eruptive phase of W-RGR. Extending the age progression of the W-RGR Eocene volcanism to the Jean-Charcot Seamounts would imply that its northwestern-most seamount formed approximately 65 Ma, about 35 Myrs later than the ages proposed by Homrighausen et al.9 (Fig. 4).

Fig. 4: Age vs distance from Gough Island.
figure 4

RGR is generally age-progressive. The Jean-Charcot Seamounts could either be age-progressive with respect to the main-phase of RGR (Homrighausen et al.9 model), or with respect to the late-stage Eocene volcanism at W-RGR (our model). Note that we have shown the Jean-Charcot seamounts schematically with the oval field which spans the distance from the nearest to closest from Gough, while in reality there are over 20 individual seamounts.

On- versus off-axis emplacement

Comparing the eruption age of a sample to the age of the underlying seafloor gives the age of the oceanic lithosphere at the time that the sample was erupted. This Δ age of a sample (Table 1) is calculated by subtracting the sample age from the modeled age of the seafloor, using the age model of Seton et al.43 for the latter.

The SE-RGR and more than half of the NE-RGR erupted at or very near the MAR axis between ~85 and 60 Ma, while W-RGR erupted more off-axis (Fig. 5). Near-zero Δ age values indicate that excess volcanism was active at the ridge axis while increasing Δ age values indicate progressively greater distance of off-axis emplacement. With a half spreading rate of 25 km Myr1 (roughly the rate at this time in the South Atlantic), a sample with a Δ age = 5 Myr was emplaced 125 km off the ridge axis. Given the volume and flux of lavas erupted to form RGR, which is upwards of 2000–3000 m above the surrounding seafloor and with a total crustal thickness of ~25 km45, it is likely that individual eruptive vents were not all centered directly at the MAR axis. Flows were also likely able to travel some distance from vents, up to tens or hundreds of kilometers, as has been shown from other submarine eruptions46,47. Therefore, samples with Δ age <5 Myr ( < 125 km) are considered to have erupted on-axis; and samples with a Δ age = 5–10 Myr near-axis (125–250 km).

Fig. 5: Δ Age of RGR and WR samples.
figure 5

a Sample age vs Δ age for RGR (gray symbols) and WR (black circles = Gough track, white squares = Tristan track). The shaded blue region is considered on axis. Walvis Ridge ages are from refs. 6,7,10,20,21 and RGR literature ages are from refs. 7,10,12. b Bathymetric map showing the locations and Δ age (colors of symbols) of all samples with ages from RGR and Walvis Ridge. Symbols are the same as A), the MAR is the red line down the center and gray lines are fracture zones. Map made in GMT70.

Overall, almost all volcanism throughout the RGR occurred between ~85 and 55 Ma (hatched region in Fig. 5a) and was mostly on-axis or near-axis of the MAR. Several locations in the NE-RGR and one in SE-RGR show continued (off-axis) volcanism for >10 Myr, after the oldest initial RGR eruptions. The locations with highest Δ age values (dredges NBP1808-D7, -D9, -D12, and -D21) all come from places that dredged large portions ( > 800 m) of the volcanic stratigraphy (Supplementary Note 5) and suggest that volcanism continued up to ~450 km off the ridge axis.

Three dredge locations at RGR contain negative Δ age values ranging from −2.0 to −3.9 Myr, indicating that the current age model needs refinement in this region during the Cretaceous43. These negative Δ age values from the RGR are coincident with slightly positive Δ age values from the WR (Fig. 5a), which may suggest that the paleo-MAR was slightly more east compared to the current reconstructions. The proposed microplate or ridge jumps2,42 could also account for such minor errors in the plate reconstructions.

Long-term Tristan-Gough plume interaction with the Mid-Atlantic ridge

Backtracked locations of RGR and WR volcanism using half-stage poles of the South American and African Plates41 show where those samples were erupted relative to the present-day MAR geometry (Fig. 6a). This shows that T-G volcanism migrated from north to south relative to the ridge by some combination of absolute plate motion and/or plume motion. Some absolute plate motion and plume motion models also indicate southward plume drift (Fig. 6b)48,49,50 but these models are subject to considerable uncertainty further back in time, in particular prior to 60–80 Ma. This southward migration of volcanism crosses what we are calling the Peleg and Rachel Fracture Zones (PFZ & RFZ: named after the closest named seamounts in the WR) during the time at which volcanism transitioned from being MAR-centered to intraplate (Fig. 6a). Together, the PFZ and RFZ account for > 450 km of lateral offset of the MAR spreading axis and they mark the southern extent of the microplate activity42. Magnetic isochrons show that this lateral offset of the paleo-MAR was also present, with a similar offset distance, at least as far back as the late Cretaceous41 (Fig. 3). We postulate that this combined large offset, in conjunction with the southward migration of the T-G plume (relative to the MAR), is responsible for the transition from MAR-centered to intraplate volcanism on the African Plate.

Fig. 6: Backtracked locations of RGR and WR volcanism.
figure 6

a Rotated to the modern ridge using half-stage rotation parameters of Pérez-Díaz & Eagles41. b Four different absolute plate motion models, which show the location of T-G plume volcanism relative to the modern ridge, and a general southward motion of the plume through time. Absolute plate motion models used: 1 = mantle reference frame49, 2 = moving hotspots model48, 3 = moving hotspots model50, 4 = global hybrid model50. WR ages come from the same references as those in Fig. 3. Colors correspond to the age of each sample. The MAR is the thick black line in the middle of each panel, fracture zones are grey lines with two important fracture zones highlighted in magenta in panel (a): PFZ Peleg Fracture Zone, RFZ Rachel Fracture Zone. The dotted portions of these extend into the regions of the RGR and WR where they are overprinted by volcanism. The blue circle in (a) shows the bifurcation point of WR, note that this occurs exactly where the PFZ intersects WR. W-RGR late-stage Eocene volcanism is circled in orange. Other off and near-axis volcanism during the formation of W-RGR and late stages of NE-RGR is circled in grey in panel (a). The green arrow in (a) shows the apparent westward shift in WR volcanism at PFZ and the shift to the African Plate only south of the RFZ. The dotted black box in (a) outlines the areas in panel b. Each map was made in GMT70.

With the exception of some late-stage volcanism that occurred off the ridge axis (e.g. RGR Eocene volcanism, circled in orange in Fig. 6), volcanism north of the PFZ lasted from ~120 Ma until ~70 Ma and was largely ridge centered. However, this Cretaceous volcanism also is characterized by a spatial variability around the MAR that is likely the result of the elevated magma fluxes forming W-RGR and NE-RGR and VB, which are the most voluminous portions of the RGR and WR, respectively. Some samples in the NE-RGR (included in the grey circle in Fig. 6) appear to have formed more off-axis, but we offer that they also could have formed as part of the microplate, which had two or more overlapping spreading segments separated by an unknown, but likely substantial ( > 100 km), distance. The less voluminous SE-RGR was formed between the PFZ and RFZ, at the time of bifurcation of WR into the Guyot Province (Figs. 3 & 6). This began at ~70 Ma and continued until ~55 Ma, during the time period when the T-G plume was transitioning from being ridge-centered to off-axis10. This largely fits with the model put forward by Homrighausen et al.9 with distinct Tristan and Gough ‘plumelets’ straddling the MAR prior to ~70 Ma, with the northwestern Tristan plumelet finally crossing the MAR by 60 Ma.

An eastward migration of the MAR around the PFZ and RFZ occurred sometime between Chron 34 and 25 (83.6–57.1 Ma), resulting in asymmetric crustal accretion (Supplementary Fig. 4). This is the time and place of SE-RGR emplacement and, as discussed, during the time when the plume was transitioning from ridge-centered to intraplate. There is also an apparent westward (from north to south) shift of WR volcanism immediately south of the PFZ (light green arrow in Fig. 6a) concurrent with the westward lateral offset of the MAR at PFZ and the bifurcation of the WR. This could indicate that the T-G plume and MAR were trying to remain coupled during this period between ~70 and 60 Ma. This resulted in shifting the ridge eastward and the plume westward, pulling each other towards a common center. South of the RFZ, and from 60 Ma to the present day, volcanism became entirely intraplate, restricted to the African Plate only, and decoupled from the ridge.

Changes in the Tristan-Gough Plume Production Rate through Time

Changes in the T-G plume magmatic production rate have been estimated in several previous studies51,52,53. These assumed a perfectly age-progressive hotspot track in which active magmatism occurs along a transect perpendicular to a line fitted through the hotspot track. These methods allow for a granular estimation of flux through time, but they neglect the fact that magmatism of this scale is distributed over a wide spatial area at any given time. Furthermore, only one estimation included both the VB, RGR, and volcanism >80 Ma51, and these studies all assumed that the entirety of RGR is >70 Ma, which we have shown is incorrect. Our geochronological record of RGR allows us to more accurately include it into estimations of the long-term T-G plume production rate.

It has been debated whether or not part of RGR is continental in origin5,29,30,45. Old continental crust was recovered in dredges29, but were described as being subrounded and covered in Mn-crust, suggesting they may be dropstones instead of in-situ crustal material. Geophysical evidence is inconclusive regarding a possible continental crustal component of RGR45. Geochemical evidence, however, indicates no evidence of continental influence (via assimilation) of the definitively in-situ basalts recovered from RGR during expedition MSM-823. Therefore, while we acknowledge that new evidence could find evidence that part of RGR is continental in origin, we assume that all of RGR is basaltic in nature.

We use residual bathymetry to find the volume of erupted lava throughout RGR and WR, using the volume above the base level, characterized by a break in slope at the 800 m contour (Supplementary Fig. 5). In this analysis we use the residual bathymetry (Fig. 7a) from CEED (https://www.earthdynamics.org/page5.html) which uses lithospheric thermal subsidence from Crosby & McKenzie54 and the isostatic correction method from Sykes55 with sediment thicknesses subtracted from the GEBCO (2014) grid56. We then use the excess magmatic volume grid from Huang & Li52 (Fig. 7b) to also calculate the total excess magma produced which includes the crustal root. Both calculations were done using GMT grdvolume and subdivided into a number of areas: RGR into W, NE, and SE; and WR into VB and its Guyot Province into 10 Myr increments based on literature ages of WR volcanism6,7,10,20,21 (Fig. 7). Our method averages the production rate over these respective areas, which has the advantage of not assuming a perfectly age-progressive nature of the T-G hotspot, but the disadvantage in that it misses shorter period pulses or variations in the production rate.

Fig. 7: Excess volcanism from the T-G plume through time.
figure 7

a The residual bathymetry in the South Atlantic was used to calculate the extrusive volume of the T-G plume through time, using the 800 m contour (the thin black contour line), which is the closest contour to the break in slope throughout RGR/WR. Profiles A-A’ through F-F’ for RGR and WR can be found in Supplementary Fig 5. b Total magmatic volume generated by the T-G plume uses the excess crustal volume estimations from Huang & Li52. The subdivisions (outlined in black in (a) and blue in (b)) are based on the age of WR volcanism in 10 Myr increments, using ages from the literature6,7,10,20,21, and for RGR include our W, NE, and SE subdivisions. The thin line denotes areas with excess volume, and the thick red line down the middle marks the MAR. Maps were made in GMT70.

The entirety of RGR has an erupted volume of ~6.7 × 105 km3, similar to the Deccan Traps57, and nearly 9.1 × 105 km3 when including VB in WR (but not the younger Guyot Province or Frio Ridge; Table 2). This is still less than half the erupted volume of the Siberian Traps and the Paraná-Etendeka, each with erupted volumes >20 × 105 km339,58 and is an order of magnitude less than the Ontong Java Plateau with an erupted volume >80 × 105 km359. The total erupted volume of the T-G hotspot from the emplacement of W-RGR/VB to the present day, including the WR Guyot Province, is ~15 × 105 km3. Maximum eruption rates were about 0.03 km3 yr1 during the emplacement of W-RGR/VB, less than modern-day Hawai’i60.

Table 2 Magmatic production rates for RGR and WR

Total magmatic volumes are on average ~5.5X greater than erupted volumes in the combined RGR and WR. Maximum total magmatic production rate estimations (total excess volume) indicate that the entirety of RGR and VB (RGR + VB) were ~0.26 km3 yr−1 (Table 2). W-RGR is the most voluminous portion of the three sub-regions (about 3/5 of the total volume, and nearly half when adjusted for surface area) and has a total production rate of ~0.15 km3 yr−1. VB and NE-RGR have slightly lower rates of ~0.10 to 0.13 km3 yr−1. The SE-RGR formed at a much lower rate of about 0.03 km3 yr−1, further suggesting that the T-G hotspot was waning in strength, even before the plume had become entirely intraplate53. This could explain why the T-G plume did not have the strength to (re)capture the MAR after it moved across the PFZ and RFZ as it reportedly did successfully at the end of the Cretaceous Quiet Period2,41. After the plume became entirely intraplate in the WR Guyot Province, production rates averaged ~0.03 km3 yr−1 from 50 Ma to the present, similar to other estimates53.

Assuming an average full spreading rate of 5 cm yr−1 in the South Atlantic, the magmatic production rate at the ridge is 3.5 × 10−4 km3 yr−1 per ridge km (km3 km−1 yr−1). To compare this with the total T-G plume production rates, we must normalize the latter rates to the diameter of the plume affecting the MAR. The plume’s diameter is estimated to be 400 km based on the spatial extent of volcanism in the Guyot Province, which in turn is close to the N-S length of RGR and VB. Production rates normalized to this 400 km ridge length are highest during the emplacement of W-RGR and VB at 7 × 10-4 km3 km-1 yr-1, and when we add this to MAR production, this essentially triples the overall magmatic output in this region. This combined rate decreases in the SE-RGR and the 60-70 Ma portion of the Guyot Province (the conjugate to the SE-RGR) to <2.5 × 10-4 km3 km-1 yr-1. After the plume moved off the ridge axis after 50 Ma, the overall production rate was reduced even further to <1 × 10-4 km3 km-1 yr-1.

A present analog to RGR is Iceland, which is a modern example of a mantle plume centered at (or near) a spreading ridge axis. Iceland is an extensively studied volcanic system with complex plume-ridge interactions that have influenced the expression of the plume as well as the northern MAR over the past >20 Myr61. Total magmatic production rates in Iceland are estimated to be ~0.25 to 0.30 km3 yr−162,63 and thus about the same as the combined W-RGR/VB, supporting their similar geodynamic origins. Other modern examples of ridge-centered plumes include the Galapagos and Azores, which have similar magmatic production rates between ~0.14 and 0.30 km3 yr−162,64. The correspondence in magma production rates between the RGR and Iceland, Galapagos, and Azores supports a mantle plume stem centered on a ridge axis having formed RGR, and not a secondary high-flux pulse of the T-G plume.

RGR/VB eruption rates are much lower than terrestrial LIP equivalents, such as the Deccan and Siberian Traps, and the Paraná-Etendeka, which all three had eruption rates >1 km3 yr−1 and pulsed peak rates much higher still23,38,39. It is possible that RGR and VB had peak production rates higher than the long-term averages we are calculating, but limited sampling prevents us from resolving these peak rates. However, to approach rates similar to the Deccan and Siberian Traps, the entirety of RGR/VB would have had to have been emplaced in <1 Ma. Given the broad geochronological coverage now available, this appears highly unlikely, implying that eruption rates for RGR/VB emplacement were one to two orders of magnitude less than terrestrial LIPs. This establishes that, despite the similarities in size and volume between RGR and terrestrial LIPs, the emplacement dynamics of RGR were quite different. According to the definition of Bryan & Ernst4 LIPs are characterized by igneous pulse(s) of short 1–5 Myr duration, during which >75% of the total igneous volume has been emplaced. RGR therefore does not qualify as a LIP based on the Bryan and Ernst definition. Other oceanic plateaus (e.g., Ontong Java, Kerguelen, Shatsky Rise) also do not meet this rapid formation criteria14,37,65, and yet are still commonly ascribed as LIPs. The vast differences in magmatic production rate among LIPs, including oceanic plateaus, likely results from important differences among their geodynamic origins (i.e., a plume head vs a plume stem interacting with a spreading center) and this also likely plays a role in the differences of their environmental impacts66.

Methods

40Ar/39Ar dating

Thirty-two locations were dredged from RGR and the surrounding area (see Supplementary Note 2 for a dredging summary). Thirty-five samples from 19 dredge locations were chosen for 40Ar/39Ar analysis. Samples were crushed with a steel jaw crusher and sieved to between ~100–175 and 250–300 μm and washed in water to remove fine-grained particles. Several phases were selected for dating and separated differently depending on the selected phase(s). Groundmass samples were magnetically separated using a Frantz magnetic barrier separator either once or twice, and the fraction with the least abundance of clearly altered grains was used. Samples were then leached first using 1 N and 6 N HCl, then 1 N and 3 N HNO3 for one hour at each strength, and thoroughly rinsed with 18 mΩ distilled water after each leaching step. Plagioclase and other feldspars were separated also using a Frantz magnetic barrier separator, with progressively higher magnetic strengths until a relatively pure fraction of mostly feldspar remained. The feldspar concentrates were then leached the same way as groundmass, but with an additional 5% HF leach for between 3 and 5 min after the 3 N HNO3 leach, and again thoroughly rinsed with 18 mΩ distilled water afterwards. Two glass samples were separated in part using a Frantz but mostly by handpicking fresh grains out from the matrix. One of these had a duplicate analyzed which was leached using our standard procedure described for groundmass above. Two biotite samples were separated using the 300-600 μm size fraction and the paper shake method where a small amount of grains are poured onto a sheet of paper and lightly shaken back and forth at an angle so that the rounder, non-biotite grains fall away, leaving almost only biotite remaining on the paper. The biotite samples were leached the same way as groundmass.

After leaching, samples were re-sieved to their original size fraction and hand-picked under a binocular microscope to remove any remaining altered grains, and feldspars with large or abundant melt inclusions. Samples were weighed and packed into Al-foil packets and labeled. Fish Canyon Tuff (FCT) sanidines were used as flux monitors (using the age of 28.201 ± 0.046 Ma67) and ten crystals (500–600 μm) were packed into Cu-foil packets. Samples and flux monitors were loaded into glass vials starting with a flux monitor and alternating between samples and flux monitors every two or three samples up to 7 cm in total length. The glass vials were vacuum-sealed with a blow torch and irradiated for six hours in Oregon State University’s TRIGA reactor CLICIT facility. Two FCT flux monitor crystals were measured individually by total fusion and J-values were calculated by parabolic interpolation of the 39Ar/40Ar value of sequential FCT flux monitor measurements within a vial. Most samples had between 7 and 11 mg of material loaded into copper tray wells such that each was filled to 1 to 2 grains high. Samples were pre-cleaned at low laser power (between 0.2 and 0.8%) for 60 s prior to analysis. Samples were degassed for 60 s per step using a 30 W Synrad CO2 laser with a Synrad FH Flyer marking head. Released gas was cleaned using three AP10 getters at 21 °C and one GP50 getter at 450 °C for 2 to 3 min before being expanded into the mass spectrometer. Between 20 and 50 incremental heating steps were measured using an ARGUS VI multi-collector mass spectrometer. 40Ar, 39Ar, 38Ar, and 37Ar were measured on faraday cups with 1013 Ω resistors (40Ar was measured on a 1012 Ω resistor) and 36Ar was measured using a CDD electron multiplier. Signals were regressed using exponential fits and abundances were extrapolated to time zero, defined as the moment the gas was introduced to the mass spectrometer from the extraction line. Blanks were measured at least every three steps after which a polynomial (up to fourth order) fit was applied and the signal subtracted from each step, while propagating blank uncertainties. Mass discrimination was calculated using a linear law relationship with the composition of air being 298.56 ± 0.3168. Collector calibrations were determined from air shot runs by “peak hopping” the 36Ar signal between the L2 Faraday collector outfitted with a 1013 Ω resistor and the CDD electron multiplier, and those ratios were then used to correct the 36Ar from the samples measured on the CDD electron multiplier. The decay constants from Min et al.69 were used and the following production ratios were used: 36Ar/37Ar(Ca) = 2.7 × 104 ± 0.17%; 38Ar/37Ar(Ca) = 1.8 × 104 ± 9.63%; 39Ar/37Ar(Ca) = 6.43 × 10−4 ± 0.92%; 40Ar/39Ar(K) = 6.07 × 10-4 ± 9.65%; 38Ar/39Ar(K) = 1.2077 × 102 ± 0.09%; all uncertainties are % 1σ standard deviations. Data reduction was done using ArArCALC35 and Python.