The fabrication of artificial crystals by reassembling monolayer semiconductors enables on-demand engineering of their excitonic properties. Here, the authors report an efficient stacking method to fabricate millimetre-scale van der Waals homo-/hetero-crystals, demonstrating enhanced monolayer-like photoluminescence emission and quadrupolar interlayer exciton emission.
- Qianlu Sun
- Jiamin Lin
- Weigao Xu