Excitonics provides a promising way to manipulate light-matter interactions for advanced optical applications, yet controlling core-exciton dynamics in the X-ray regime is challenging. Here, the authors combine experiments with an ab initio approach developed specifically for modelling pump-probe excitations, revealing how photoexcited carrier distributions can be used to control core-exciton resonances at absorption edges.
- Thomas C. Rossi
- Lu Qiao
- Renske M. van der Veen