Fig. 3: Strong-field quantum control of dressed He populations. | Nature

Fig. 3: Strong-field quantum control of dressed He populations.

From: Strong-field quantum control in the extreme ultraviolet domain using pulse shaping

Fig. 3: Strong-field quantum control of dressed He populations.

a, Photoelectron spectra obtained for phase-shaped XUV pulses (see labels for GDD values; photon energy = 21.25 eV; Ieff = 2.8(2) × 1,014 W cm−2). The control of the dressed-state populations is directly reflected in the relative change of amplitude in the photoelectron bands. The small peak at 18.13 eV results from imperfect removal of the lower intensity contribution from the aberrated focus. b, Calculations of the time-dependent Schrödinger equation for a single active electron (TDSE-SAE) and a single laser intensity corresponding to the experimental Ieff = 2.8 × 1014 W cm2 (dark colours). Spectral fringes reflect here the temporal progression of the Rabi frequency during the light–matter interaction. The broadened photoelectron spectra (light colours) account for experimental broadening effects caused by the focal intensity averaging and the instrument response function. a.u., arbitrary units.

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