Abstract
Broadband photodetectors in the visible and short-wave infrared wavelengths have garnered significant interest in recent years as a desirable method to achieve better detection in adverse weather conditions. Many material combinations have been proposed to replace expensive III-V based photodetectors; however, the photodetection performance of these novel material and device concepts showed undesirable performances due to uncontrollable charge-trap-based photomultiplication, preventing fast photoresponse and gain. To solve this issue, we devised an engineered potential trap in Ge/MoS2 double junction phototransistor which show a high responsivity of 7.6 A/W (corresponding to an external quantum efficiency of 2,024%) as well as a fast photoresponse of 88.1 µs. The maximum photocurrent gain reaches 29.1 with broadband imaging capability. This excellent performance is achieved through photogenerated hole confined in p-Ge clad by MoS2 and n-Ge induced multiple electrons, which diminished rapidly via recombination upon removal of illumination. Our device concept enables creation of highly sensitive fast broadband imaging based on mixed dimensional van der Waals heterojunctions.
Data availability
The datasets used and/or analysed during the current study available from the corresponding author on reasonable request.
References
Naboulsi, M. A. Fog Attenuation prediction for optical and infrared waves. Opt. Eng. 43(2), 319. https://doi.org/10.1117/1.1637611 (2004).
Driggers, R. G., Hodgkin, V. & Vollmerhausen, R. What good is SWIR? Passive day comparison of VIS, NIR, and SWIR. Infrared Imaging Syst. Des. Anal. Model. Test. XXIV. 8706, 87060L. https://doi.org/10.1117/12.2016467 (2013).
Martin, T., Brubaker, R., Dixon, P., Gagliardi, M. A. & Sudol, T. 640x512 InGaAs focal plane array camera for visible and SWIR imaging. Infrared Technol. Appl. XXXI. 5783, 12. https://doi.org/10.1117/12.603406 (2005).
Malchow, D., Battaglia, J., Brubaker, R. & Ettenberg, M. High speed short wave infrared (SWIR) imaging and range gating cameras, in Thermosense XXIX, Vol. 6541, 654106. https://doi.org/10.1117/12.721747 (2007).
Bernini, N., Bertozzi, M., Cerri, P. & Fedriga, R. I. SWIR cameras for the automotive field: two test cases. ISRN Automot. Eng. 2014, 1–11. https://doi.org/10.1155/2014/858979 (2014).
Tsuboi, S. & Jin, T. Shortwave-infrared (SWIR) fluorescence molecular imaging using indocyanine green-antibody conjugates for the optical diagnostics of cancerous tumours. RSC Adv. 10(47), 28171–28179. https://doi.org/10.1039/d0ra04710d (2020).
Qi, J. et al. Real-Time and high-resolution bioimaging with bright aggregation-induced emission dots in short-wave infrared region. Adv. Mater. 30(12), 1706856. https://doi.org/10.1002/adma.201706856 (2018).
Yu, Z. et al. High-Resolution shortwave infrared imaging of vascular disorders using gold nanoclusters. ACS Nano. 14(4), 4973–4981. https://doi.org/10.1021/acsnano.0c01174 (2020).
Narang, N. & Bourlai, T. Face recognition in the SWIR band when using single sensor multi-wavelength imaging systems. Image Vis. Comput. 33, 26–43. https://doi.org/10.1016/j.imavis.2014.10.005 (2015).
Goossens, S. et al. Broadband image sensor array based on graphene-CMOS integration. Nat. Photonics. 11(6), 366–371. https://doi.org/10.1038/nphoton.2017.75 (2017).
Ni, Z. et al. Plasmonic silicon quantum Dots enabled High-Sensitivity ultrabroadband photodetection of Graphene-Based hybrid phototransistors. ACS Nano. 11(10), 9854–9862. https://doi.org/10.1021/acsnano.7b03569 (2017).
Kufer, D. et al. Hybrid 2D-0D MoS2-PbS quantum Dot photodetectors. Adv. Mater. 27(1), 176–180. https://doi.org/10.1002/adma.201402471 (2015).
Cao, R. et al. Black Phosphorous/Indium Selenide photoconductive detector for visible and Near-Infrared light with high sensitivity. Adv. Opt. Mater. 7(12), 1–7. https://doi.org/10.1002/adom.201900020 (2019).
Ye, L., Li, H., Chen, Z. & Xu, J. Near-Infrared photodetector based on MoS2/Black phosphorus heterojunction. ACS Photonics. 3(4), 692–699. https://doi.org/10.1021/acsphotonics.6b00079 (2016).
Geum, D. M. et al. Arrayed MoS2–In0.53Ga0.47As Van der Waals heterostructure for High-Speed and broadband detection from visible to Shortwave-Infrared light. Small https://doi.org/10.1002/smll.202007357 (2021).
Heves, E. & Gurbuz, Y. Highly responsive, solution-based Al/PbS and Au-Ti/PbS Schottky photodiodes for SWIR detection. IEEE Sens. J. 14(3), 816–820 (2014).
Kim, S. G. et al. Infrared detectable MoS2 phototransistor and its application to artificial multilevel Optic-Neural synapse. ACS Nano. 13(9), 10294–10300. https://doi.org/10.1021/acsnano.9b03683 (2019).
Hwang, A. et al. Visible and infrared dual-band imaging via Ge/MoS2van der Waals heterostructure. Sci. Adv. 7(51), 1–9. https://doi.org/10.1126/sciadv.abj2521 (2021).
Lee, C. H. et al. Design of p-WSe 2 /n‐Ge heterojunctions for High‐Speed broadband photodetectors. Adv. Funct. Mater. 2107992, 2107992. https://doi.org/10.1002/adfm.202107992 (2021).
Choi, W. et al. Recent development of two-dimensional transition metal dichalcogenides and their applications. Mater. Today. 20(3), 116–130. https://doi.org/10.1016/j.mattod.2016.10.002 (2017).
Lopez-Sanchez, O. et al. Light generation and harvesting in a Van der Waals heterostructure. ACS Nano. 8(3), 3042–3048. https://doi.org/10.1021/nn500480u (2014).
Vashishtha, P. et al. Epitaxial interface-driven photoresponse enhancement in monolayer WS2-MoS2 lateral heterostructures. Adv. Funct. Mater., Early View. https://doi.org/10.1002/adfm.202512962 (2025)
Vashishtha, P. et al. Self-powered broadband photodetection of MoS2/Sb2Se3 heterostructure. ACS Appl. Opt. Mater. 1, 1952. https://doi.org/10.1021/acsaom.3c00300 (2023).
Park, Y., Hwang, A. J., Lee, C., Yoo, G. & Heo, J. Broadband photodetection of MoS2/p-Ge/n-Ge bipolar heterojunction phototransistor. in Conference on Lasers and Electro-Optics, CLEO 2021 - Proceedings STh5B.3 (2021). https://doi.org/10.1364/cleo_si.2021.sth5b.3.
Zhao, Z. Y. & Liu, Q. L. Study of the layer-dependent properties of MoS2 nanosheets with different crystal structures by DFT calculations. Catal. Sci. Technol. 8(7), 1867–1879. https://doi.org/10.1039/c7cy02252b (2018).
Trommer, J. et al. Enabling energy efficiency and Polarity control in germanium nanowire transistors by individually gated nanojunctions. ACS Nano. 11(2), 1704–1711. https://doi.org/10.1021/acsnano.6b07531 (2017).
Su, B. W. et al. A gate-tunable symmetric bipolar junction transistor fabricated: Via femtosecond laser processing. Nanoscale Adv. 2(4), 1733–1740 (2020). https://doi.org/10.1039/d0na00201a
Li, H., Ye, L. & Xu, J. High-Performance broadband Floating-Base bipolar phototransistor based on WSe2/BP/MoS2 heterostructure. ACS Photonics. 4(4), 823–829. https://doi.org/10.1021/acsphotonics.6b00778 (2017).
Prucnal, S. et al. Superconductivity in single-crystalline aluminum- and gallium-hyperdoped germanium. Phys. Rev. Mater. 3(5), 1–10. https://doi.org/10.1103/PhysRevMaterials.3.054802 (2019).
Lee, C. et al. Anomalous lattice vibrations of single- and few-layer MoS2. ACS Nano. 4(5), 2695–2700. https://doi.org/10.1021/nn1003937 (2010).
Nishimura, T., Luo, X., Matsumoto, S., Yajima, T. & Toriumi, A. Almost pinning-free bismuth/Ge and /Si interfaces. AIP Adv. 9(9), 095013 https://doi.org/10.1063/1.5115535 (2019).
Anderson, B. & Anderson, R. Fundamentals of Semiconductor Devices1st edn (McGraw-Hill College, 2004).
Choudhary, N. et al. Two-dimensional lateral heterojunction through bandgap engineering of MoS2 via oxygen plasma. J. Phys. Condens. Matter. 28(36), 364002 https://doi.org/10.1088/0953-8984/28/36/364002 (2016).
Yan, X. et al. High performance amplifier element realization via MoS2/GaTe heterostructures. Adv. Sci. 5(4), 1–7. https://doi.org/10.1002/advs.201700830 (2018).
Eng, P. C., Song, S. & Ping, B. State-of-the-art photodetectors for optoelectronic integration at telecommunication wavelength. Nanophotonics 4(1), 277–302 https://doi.org/10.1515/nanoph-2015-0012 (2015).
Funding
This study was supported by the National R&D Program through the National Research Foundation of Korea (NRF) funded by the Ministry of Science and ICT (RS-2024-00438811, RS-2025-00564261, RS-2025-02217113).
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Y.P. fabricated the devices and performed the electrical and optical measurements. H.B.J and H.Y.J performed the material characterizations. Y.P., M.J., S.S., G.Y., and J.H. analyzed the experiments and wrote the manuscript. All authors contributed to the discussion and analysis of the results of the manuscript. J.H. supervised the project.
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Park, Y., Jung, M., Jeong, H.B. et al. Fast photo-carrier multiplication by engineered potential trap in MoS2/Ge double junction phototransistor. Sci Rep (2026). https://doi.org/10.1038/s41598-026-35134-z
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DOI: https://doi.org/10.1038/s41598-026-35134-z