Abstract
Nanowire arrays are excellent nanostructured target materials for high-energy density (HED) science and applications because of their enhanced energy absorption properties. However, investigations of the spatiotemporal dynamics of laser-irradiated nanowire arrays remain limited, since conventional time-resolved diagnostics cannot capture the rapid plasma-state transitions. This study reports spatiotemporally resolved measurements of laser energy absorption and electron transport in laser-irradiated nanowire arrays using an X-ray free-electron laser (XFEL). The XFEL measurements showed that the nanowire array is promptly heated to an electron temperature of ~ 120 eV at the main-pulse interaction peak, followed by a further increase to ~ 140 eV around 10 ps, which was associated with wire collapse. The experimental results also confirmed that further enlargement of the heated area was suppressed by the restricted electron transport in nanowire arrays. These observations advance our understanding of HED plasma formation and evolution within the laser-irradiated nanowire arrays, laying a foundation for various applications.
Data availability
The data that support the findings of this study are available from the corresponding author upon reasonable request.
References
Strickland, D. & Mourou, G. Compression of amplified chirped optical pulses. Opt. Commun. 56, 219–221 (1985).
Nuckolls, J., Wood, L., Thiessen, A. & Zimmerman, G. Laser compression of matter to super-high densities: Thermonuclear (CTR) applications. Nature 239, 139–142 (1972).
Abu-Shawareb, H. et al. Achievement of target gain larger than unity in an inertial fusion experiment. Phys. Rev. Lett. 132, 065104 (2024).
Remington, B. A., Arnett, D., Paul, R., Drake, R. P. & Takabe, H. Modeling astrophysical phenomena in the laboratory with intense lasers. Science 284, 1488–1493 (1999).
Daido, H., Nishiuchi, M. & Pirozhkov, A. S. Review of laser-driven ion sources and their applications. Rep. Prog Phys. 75, 056401 (2012).
Zhidkov, A. et al. Prepulse effects on the interaction of intense femtosecond laser pulses with high-Z solids. Phys. Rev. E. 62, 7232 (2000).
Takizawa, R. et al. Boosting fast ignition heating through interaction between ultrahigh-contrast heating lasers and a cone-shaped target. Phys. Rev. Res. 7, 023081 (2025).
Chopineau, L. et al. Identification of coupling Mechanisms between ultraintense laser light and dense plasmas. Phys. Rev. X. 9, 011050 (2019).
Ping, Y. et al. Absorption of short laser pulses on solid targets in the ultrarelativistic regime. Phys. Rev. Lett. 100, 085004 (2008).
Purvis, M. A. et al. Relativistic plasma nanophotonics for ultrahigh energy density physics. Nat. Photonics. 7, 796–800 (2013).
Lad, A. D. et al. Luminous, relativistic, directional electron bunches from an intense laser driven grating plasma. Sci. Rep. 12, 16818 (2022).
Fedeli, L. et al. Electron acceleration by relativistic surface plasmons in laser-grating interaction. Phys. Rev. Lett. 116, 015001 (2016).
Shou, Y. et al. Brilliant femtosecond-laser-driven hard X-ray flashes from carbon nanotube plasma. Nat. Photonics. 17, 137–142 (2023).
Gizzi, L. A. et al. Intense proton acceleration in ultrarelativistic interaction with nanochannels. Phys. Rev. Res. 2, 033451 (2020).
Sumeruk, H. A. et al. Control of strong-laser-field coupling to electrons in solid targets with wavelength-scale spheres. Phys. Rev. Lett. 98, 045001 (2007).
Rocca, J. J. et al. Ultra-intense femtosecond laser interactions with aligned nanostructures. Optica 11, 437–453 (2024).
Bargsten, C. et al. Energy penetration into arrays of aligned nanowires irradiated with relativistic intensities: Scaling to terabar pressures. Sci. Adv. 3, e1601558 (2017).
Kaymak, V., Pukhov, A., Shlyaptsev, V. N. & Rocca, J. J. Nanoscale ultradense Z-pinch formation from laser-irradiated nanowire arrays. Phys. Rev. Lett. 117, 035004 (2016).
Tian, J. M. et al. Generation mechanism of 100 MG magnetic fields in the interaction of ultra-intense laser pulse with nanostructured target. High. Power Laser Sci. Eng. 8, e16 (2020).
Tanaka, D. et al. Ultrahigh-energy density state in nanowire arrays irradiated with picosecond kilojoule-class ultra-intense laser. AIP Adv. 13, 125118 (2023).
Humphries, O. S. et al. Time evolution of transient plasma states from nanowire arrays irradiated at relativistic intensities. Commun. Phys. 3, 170 (2020).
Hollinger, R. et al. Efficient picosecond x-ray pulse generation from plasmas in the radiation dominated regime. Optica 4, 1344 (2017).
Eftekhari-Zadeh, E. et al. Laser energy absorption and X-ray generation in nanowire arrays irradiated by relativistically intense ultra-high contrast femtosecond laser pulses. Phys. Plasmas. 29, 013301 (2022).
Curtis, A. et al. Micro-scale fusion in dense relativistic nanowire array plasmas. Nat. Commun. 9, 1077 (2018).
Kong, D. et al. High-energy-density plasma in femtosecond-laser-irradiated nanowire-array targets for nuclear reactions. Matter Radiat. Extremes. 7, 064403 (2022).
Shou, Y. et al. High-efficiency water-window X-ray generation from nanowire array targets irradiated with femtosecond laser pulses. Opt. Express. 29, 5427 (2021).
Vallieres, S. et al. Enhanced laser-driven proton acceleration using nanowire targets. Sci. Rep. 11, 2226 (2021).
Cristoforetti, G. et al. Transition from coherent to stochastic electron heating in ultrashort relativistic laser interaction with structured targets. Sci. Rep. 7, 1479 (2017).
Maeda, Y. et al. Observation of ultra-high energy density state with x-ray free electron laser SACLA. High. Energy Density Phys. 36, 100813 (2020).
Park, J. et al. Absolute laser energy absorption measurement of relativistic 0.7 ps laser pulses in nanowire arrays. Phys. Plasmas. 28, 023302 (2021).
Sawada, H. et al. Spatiotemporal dynamics of fast electron heating in solid-density matter via XFEL. Nat. Commun. 15, 7528 (2024).
Sawada, H. et al. Ultrafast time-resolved 2D imaging of laser-driven fast electron transport in solid density matter using an x-ray free electron laser. Rev. Sci. Instrum. 94, 033511 (2023).
Laso Garcia, A. et al. Cylindrical compression of thin wires by irradiation with a Joule-class short-pulse laser. Nat. Commun. 15, 7896 (2024).
Kraus, D. et al. The structure of liquid carbon elucidated by in situ X-ray diffraction. Nature 642, 351–355 (2025).
Vassholz, M. et al. Pump-probe X-ray holographic imaging of laser-induced cavitation bubbles with femtosecond FEL pulses. Nat. Commun. 12, 3468 (2021).
Katagiri, K. et al. Transonic dislocation propagation in diamond. Science 382, 69–72 (2023).
Johnson, A. S. et al. Ultrafast X-ray imaging of the light-induced phase transition in VO2. Nat. Phys. 19, 215–220 (2023).
Tono, K. et al. Beamline, experimental stations and photon beam diagnostics for the hard x-ray free electron laser of SACLA. New. J. Phys. 15, 083035 (2013).
Yabuuchi, T. et al. An experimental platform using high-power, high-intensity optical lasers with the hard X-ray free-electron laser at SACLA. J. Synchrotron Radiat. 26, 585–594 (2019).
Kameshima, T. et al. Development of an X-ray imaging detector to resolve 200 nm line-and-space patterns by using transparent ceramics layers bonded by solid-state diffusion. Opt. Lett. 44, 1403 (2019).
Dorchies, F. et al. X-ray absorption K edge as a diagnostic of the electronic temperature in warm dense aluminum. Phys. Rev. B. 92, 085117 (2015).
Hansen, S. B. et al. Fluorescence and absorption spectroscopy for warm dense matter studies and ICF plasma diagnostics. Phys. Plasmas. 25, 056301 (2018).
Chung, H. K., Chen, M. H., Morgan, W. L., Ralchenko, Y. & Lee, R. W. FLYCHK: Generalized population kinetics and spectral model for rapid spectroscopic analysis for all elements. High. Energy Density Phys. 1, 3–12 (2005).
Henke, B. L., Gullikson, E. M. & Davis, J. C. X-Ray Interactions: Photoabsorption, scattering, transmission, and reflection at E = 50 – 30,000 eV, Z = 1–92. Data Nucl. Data Tables. 54, 181–342 (1993).
Tanaka, D. et al. Experimental investigation on nanowire array irradiated with ultrahigh intensity laser at X-ray free electron laser facility SACLA: Fabrication of nanowire array target and its application to ultrafast time-resolved measurements. J. Appl. Phys. 137, 125901 (2025).
Szymańska, E. et al. The K x-ray line structures of the 3d-transition metals in warm dense plasma. High. Energy Density Phys. 20, 29–33 (2016).
Sentoku, Y. & Kemp, A. J. Numerical methods for particle simulations at extreme densities and temperatures: Weighted particles, relativistic collisions and reduced currents. J. Comput. Phys. 227, 6846–6861 (2008).
Takabe, H. et al. Scalings of implosion experiments for high neutron yield. Phys. Fluids. 31, 2884–2893 (1988).
Acknowledgements
The XFEL experiments were performed at BL2 of SACLA with the approval of the Japan Synchrotron Radiation Research Institute (JASRI) (Proposal No. 2024B8051, 2024A8013, 2023A8015, 2023A8018, and 2021B8070). The authors would like to acknowledge the dedicated technical support provided by the staff at SACLA for XFEL operation and X-ray diagnostics. Authors would like to acknowledge Editage for English language editing.
Funding
The XFEL experiments were performed at BL2 of SACLA with the approval of the Japan Synchrotron Radiation Research Institute (JASRI) (Proposal No. 2024B8051, 2024A8013, 2023A8015, 2023A8018, and 2021B8070). This work was performed under the Institute of Laser Engineering (ILE) joint research project at The University of Osaka (Contract subjects 2025B2-016SAWADA, 2024B2-019SAWADA, and 2023B2-018SAWADA). D. T. received support from the Japan Society for the Promotion of Science (KAKENHI Grant No. 23KJ1526). D. T. also received support from the SACLA Research Support Program for Graduate Students. H. S. was supported by the National Science Foundation under Grant No. 2010502 through the NSF/DOE Partnership in Basic Plasma Science and Engineering. C. N. was partially supported by JST SPRING (Grant number JPMJSP2138).
Author information
Authors and Affiliations
Contributions
D. T. wrote the original manuscript after receiving input and feedback from H. S., C. N., Y. T., T. Y., Y. S., N. O., K. Y., and K. Shigemori. D. T. led the formal analysis and visualization with support from H. S., D. T., H. S., C. N., S. M., T. S., I. N., S. H., T. Y., K. M., K. Sueda, and K. Shigemori performed the experiments and acquired data. T. Y., K. M., Y. I., and K. Sueda operated the high-power femtosecond laser system. Y. S. conducted PIC simulation. D. T. prepared the nanowire array samples with the support of T. Somekawa, T. Shimizu, S. S., and K. Y. K. Shigemori, who proposed and organized this study.
Corresponding author
Ethics declarations
Competing interests
The authors declare no competing interests.
Additional information
Publisher’s note
Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.
Rights and permissions
Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/.
About this article
Cite this article
Tanaka, D., Sawada, H., Nakatsuji, C. et al. Ultrafast plasma dynamics in laser-irradiated nanowire arrays probed with an X-ray free-electron laser. Sci Rep (2026). https://doi.org/10.1038/s41598-026-47126-0
Received:
Accepted:
Published:
DOI: https://doi.org/10.1038/s41598-026-47126-0