Abstract
Entanglement dynamics are fundamental to quantum technologies, yet controlling their temporal evolution in a reversible and stable manner remains challenging. We propose a solid-state framework based on the Ruderman–Kittel–Kasuya–Yosida interaction, realizable in gate-defined quantum dots or suspended structures, in which two spin qubits couple to a central spin qudit that mediates an effective, time-dependent exchange. The dynamics are governed by an exchange-time integral that unifies interaction strength and physical time into a single scalar control variable, enabling time-reversible and cyclic navigation of the Hilbert space. Crucially, we show that out-of-phase modulation grants access to higher entanglement subspaces, while introducing damping to the exchange modulation achieves stabilized trajectories that drive the system toward stationary entanglement values. This framework provides a systematic route for shaping entanglement dynamics, particularly in the near-boundary regime, using exchange control alone, overcoming the limitations of monotonic evolution and offering practical strategies for entanglement stabilization in realistic solid-state architectures, with direct relevance to quantum metrology and environment-assisted entanglement engineering.
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All data generated or analysed during this study are included in this published article (and its Supplementary Information files). The codes used during the current study are available from the corresponding author on reasonable request.
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The codes used during the current study are available from the corresponding author on reasonable request.
References
Życzkowski, K., Horodecki, P., Horodecki, M. & Horodecki, R. Dynamics of quantum entanglement. Phys. Rev. A 65, 012101. https://doi.org/10.1103/PhysRevA.65.012101 (2001).
Horodecki, R., Horodecki, P., Horodecki, M. & Horodecki, K. Quantum entanglement. Rev. Mod. Phys. 81, 865–942. https://doi.org/10.1103/RevModPhys.81.865 (2009).
Bennett, C. H. & DiVincenzo, D. P. Quantum information and computation. Nature 404, 247–255 (2000).
Khalili, F. Y. & Polzik, E. S. Overcoming the standard quantum limit in gravitational wave detectors using spin systems with a negative effective mass. Phys. Rev. Lett. 121, 031101. https://doi.org/10.1103/PhysRevLett.121.031101 (2018).
Zeuthen, E., Polzik, E. S. & Khalili, F. Y. Gravitational wave detection beyond the standard quantum limit using a negative-mass spin system and virtual rigidity. Phys. Rev. D 100, 062004 (2019).
Ekert, A. K. Quantum cryptography based on bell’s theorem. Phys. Rev. Lett. 67, 661–663. https://doi.org/10.1103/PhysRevLett.67.661 (1991).
Shor, P. W. & Preskill, J. Simple proof of security of the bb84 quantum key distribution protocol. Phys. Rev. Lett. 85, 441 (2000).
Gisin, N., Ribordy, G., Tittel, W. & Zbinden, H. Quantum cryptography. Rev. Mod. Phys. 74, 145 (2002).
Bennett, C. H. Quantum information. Phys. Scr. 1998, 210 (1998).
DiVincenzo, D. P. Quantum computation. Science 270, 255–261 (1995).
Steane, A. Quantum computing. Rep. Prog. Phys. 61, 117 (1998).
DiVincenzo, D. P. The physical implementation of quantum computation. Fortschritte der Physik: Progr. Phys. 48, 771–783 (2000).
Ladd, T. D. et al. Quantum computers. Nature 464, 45–53 (2010).
Nielsen, M. A. & Chuang, I. L. Quantum computation and quantum information (Cambridge university press, 2010).
Madsen, L. S. et al. Quantum computational advantage with a programmable photonic processor. Nature 606, 75–81 (2022).
Preskill, J. Quantum computing in the nisq era and beyond. Quantum 2, 79 (2018).
Riera-Sàbat, F., Sekatski, P. & Dür, W. Remotely controlled entanglement generation. Quantum 7, 904 (2023).
Zhang, Z. et al. Entanglement-based quantum information technology: a tutorial. Adv. Opt. Photon. 16, 60–162 (2024).
Wang, T.-L. et al. Remote entanglement generation via enhanced quantum state transfer. arXiv:2506.06669 (2025).
Arute, F. et al. Quantum supremacy using a programmable superconducting processor. Nature 574, 505–510 (2019).
Cirac, J. I. & Zoller, P. Quantum computations with cold trapped ions. Phys. Rev. Lett. 74, 4091–4094. https://doi.org/10.1103/PhysRevLett.74.4091 (1995).
Monroe, C. et al. Large-scale modular quantum-computer architecture with atomic memory and photonic interconnects. Phys. Rev. A 89, 022317 (2014).
Zhong, H.-S. et al. Quantum computational advantage using photons. Science 370, 1460–1463 (2020).
Humphreys, P. C. et al. Deterministic delivery of remote entanglement on a quantum network. Nature 558, 268–273 (2018).
Tyryshkin, A. M. et al. Electron spin coherence exceeding seconds in high-purity silicon. Nat. Mater. 11, 143–147 (2012).
Pla, J. J. et al. High-fidelity readout and control of a nuclear spin qubit in silicon. Nature 496, 334–338 (2013).
Watson, T. F. et al. A programmable two-qubit quantum processor in silicon. Nature 555, 633–637 (2018).
Loss, D. & DiVincenzo, D. P. Quantum computation with quantum dots. Phys. Rev. A 57, 120–126. https://doi.org/10.1103/PhysRevA.57.120 (1998).
Nowack, K. C., Koppens, F., Nazarov, Y. V. & Vandersypen, L. Coherent control of a single electron spin with electric fields. Science 318, 1430–1433 (2007).
Petta, J. R. et al. Coherent manipulation of coupled electron spins in semiconductor quantum dots. Science 309, 2180–2184 (2005).
Zajac, D. M. et al. Resonantly driven cnot gate for electron spins. Science 359, 439–442 (2018).
Bluhm, H. et al. Dephasing time of gaas electron-spin qubits coupled to a nuclear bath exceeding 200 \(\mu\)s. Nat. Phys. 7, 109–113 (2011).
Chen, S.-H. Origin and early growth of entanglement by \(sd\) exchange with gate voltage controllable outcome. Phys. Rev. B 109, 045308. https://doi.org/10.1103/PhysRevB.109.045308 (2024).
Lin, L.-C., Tan, S. G., Chang, C.-R., Sun, S.-J. & Chen, S.-H. Entanglement induced by heisenberg exchange between an electron in a nested quantum dot and a qubit with relative motion. New J. Phys. (2025).
Vavilov, M. G. & Glazman, L. I. Transport spectroscopy of kondo quantum dots coupled by rkky interaction. Phys. Rev. Lett. 94, 086805. https://doi.org/10.1103/PhysRevLett.94.086805 (2005).
Petersson, K. D. et al. Circuit quantum electrodynamics with a spin qubit. Nature 490, 380–383 (2012).
Yang, G., Hsu, C.-H., Stano, P., Klinovaja, J. & Loss, D. Long-distance entanglement of spin qubits via quantum hall edge states. Phys. Rev. B 93, 075301. https://doi.org/10.1103/PhysRevB.93.075301 (2016).
Wang, J.-N. et al. Unified formulations for rkky interaction, side kondo behavior, and fano antiresonance in a hybrid tripartite quantum dot device with filtered density of states. Phys. Rev. B 106, 035428. https://doi.org/10.1103/PhysRevB.106.035428 (2022).
Vonhoff, F., Fischer, A., Deltenre, K. & Anders, F. B. Microscopic origin of the effective spin-spin interaction in a semiconductor quantum dot ensemble. Phys. Rev. Lett. 129, 167701. https://doi.org/10.1103/PhysRevLett.129.167701 (2022).
Utsumi, Y., Martinek, J., Bruno, P. & Imamura, H. Indirect exchange interaction between two quantum dots in an aharonov-bohm ring. Phys. Rev. B 69, 155320 (2004).
Stocker, L. & Zilberberg, O. Coherent exchange-coupled nonlocal kondo impurities. Phys. Rev. Res. 6, L022058 (2024).
Chen, S.-H., Maekawa, S., Liu, M.-H. & Chang, C.-R. Mirror symmetry and exchange of magnetic impurities mediated by electrons of rashba spin-orbit interaction in a four-terminal landauer setup. J. Phys. D Appl. Phys. 43, 015003 (2009).
Allerdt, A., Büsser, C. A., Martins, G. B. & Feiguin, A. E. Kondo versus indirect exchange: Role of lattice and actual range of rkky interactions in real materials. Phys. Rev. B 91, 085101. https://doi.org/10.1103/PhysRevB.91.085101 (2015).
Mousavi, F. M. & Farghadan, R. Electrical control of ruderman-kittel-kasuya-yosida exchange interaction in zigzag edge mos2 nanoflakes. J. Phys. Chem. Solids 158, 110242 (2021).
Kettemann, S. Competition between kondo effect and rkky coupling. arXiv:2408.03112 (2024).
Ruderman, M. A. & Kittel, C. Indirect exchange coupling of nuclear magnetic moments by conduction electrons. Phys. Rev. 96, 99 (1954).
Kasuya, T. A theory of metallic ferro- and antiferromagnetism. Progr. Theoret. Phys. 16, 45 (1956).
Yosida, K. Magnetic properties of cu-mn alloys. Phys. Rev. 106, 893 (1957).
Cho, S. Y. & McKenzie, R. H. Quantum entanglement in the two-impurity kondo model. Phys. Rev. A 73, 012109. https://doi.org/10.1103/PhysRevA.73.012109 (2006).
Elman, S. J., Bartlett, S. D. & Doherty, A. C. Long-range entanglement for spin qubits via quantum hall edge modes. Phys. Rev. B 96, 115407. https://doi.org/10.1103/PhysRevB.96.115407 (2017).
Klotz, M., Tangemann, A., Opferkuch, D. & Kubanek, A. Bipartite entanglement in a nuclear spin register mediated by a quasi-free electron spin. Nat. Commun. 17, 2325. https://doi.org/10.1038/s41467-026-70154-3 (2026).
Yu, T. & Eberly, J. H. Finite-time disentanglement via spontaneous emission. Phys. Rev. Lett. 93, 140404. https://doi.org/10.1103/PhysRevLett.93.140404 (2004).
Yu, T. & Eberly, J. Sudden death of entanglement: Classical noise effects. Opt. Commun. 264, 393–397 (2006).
Yu, T. & Eberly, J. Quantum open system theory: Bipartite aspects. Phys. Rev. Lett. 97, 140403 (2006).
Ann, K. & Jaeger, G. Local-dephasing-induced entanglement sudden death in two-component finite-dimensional systems. Phys. Rev. A 76, 044101. https://doi.org/10.1103/PhysRevA.76.044101 (2007).
Yu, T. & Eberly, J. H. Sudden death of entanglement. Science 323, 598–601 (2009).
Yuan, X.-Z., Goan, H.-S. & Zhu, K.-D. Non-Markovian reduced dynamics and entanglement evolution of two coupled spins in a quantum spin environment. Phys. Rev. B 75, 045331. https://doi.org/10.1103/PhysRevB.75.045331 (2007).
Wang, F. et al. Observation of entanglement sudden death and rebirth by controlling a solid-state spin bath. Phys. Rev. B 98, 064306. https://doi.org/10.1103/PhysRevB.98.064306 (2018).
Chen, S.-H., Tan, S. G. & Huang, C.-C. General recipe for immediate entanglement death and birth via bell states: environmental heisenberg exchange with transition as an example. Phys. Scr. 100, 065114 (2025).
Almeida, M. P. et al. Environment-induced sudden death of entanglement. Science 316, 579–582 (2007).
Hutton, A. & Bose, S. Mediated entanglement and correlations in a star network of interacting spins. Phys. Rev. A 69, 042312. https://doi.org/10.1103/PhysRevA.69.042312 (2004).
Bazhanov, D. I., Sivkov, I. N. & Stepanyuk, V. S. Engineering of entanglement and spin state transfer via quantum chains of atomic spins at large separations. Sci. Rep. 8, 14118 (2018).
Stocker, L., Sack, S. H., Ferguson, M. S. & Zilberberg, O. Entanglement-based observables for quantum impurities. Phys. Rev. Res. 4, 043177. https://doi.org/10.1103/PhysRevResearch.4.043177 (2022).
Mondal, P., Suresh, A. & Nikolić, B. K. When can localized spins interacting with conduction electrons in ferro- or antiferromagnets be described classically via the landau-lifshitz equation: Transition from quantum many-body entangled to quantum-classical nonequilibrium states. Phys. Rev. B 104, 214401. https://doi.org/10.1103/PhysRevB.104.214401 (2021).
Garcia-Gaitan, F. & Nikolić, B. K. Fate of entanglement in magnetism under Lindbladian or non-Markovian dynamics and conditions for their transition to Landau-Lifshitz-Gilbert classical dynamics. Phys. Rev. B 109, L180408. https://doi.org/10.1103/PhysRevB.109.L180408 (2024).
Mortezapour, A., Borji, M. A. & Franco, R. L. Protecting entanglement by adjusting the velocities of moving qubits inside non-markovian environments. Laser Phys. Lett. 14, 055201 (2017).
Huan, T., Zhou, R. & Ian, H. Dynamic entanglement transfer in a double-cavity optomechanical system. Phys. Rev. A 92, 022301. https://doi.org/10.1103/PhysRevA.92.022301 (2015).
Obada, A. F., Hessian, H. & Hashem, M. Quantum entanglement in a system of two moving atoms interacting with a single mode field. Phys. Scr. 81, 055303 (2010).
Pandit, M., Das, S., Roy, S. S., Dhar, H. S. & Sen, U. Effects of cavity-cavity interaction on the entanglement dynamics of a generalized double jaynes-cummings model. J. Phys. B: At. Mol. Opt. Phys. 51, 045501 (2018).
Costa, A. Jr. & Bose, S. Impurity scattering induced entanglement of ballistic electrons. Phys. Rev. Lett. 87, 277901 (2001).
Sharma, A. & Tulapurkar, A. A. Transmission-based tomography for spin qubits. Phys. Rev. A 103, 052430 (2021).
Leon, A. O., d’Albuquerque e Castro, J., Retamal, J. C., Cahaya, A. B. & Altbir, D.,. Manipulation of the rkky exchange by voltages. Phys. Rev. B100, 014403. https://doi.org/10.1103/PhysRevB.100.014403 (2019).
Tran, B. X. et al. Field-free control and switching of perpendicular magnetization by voltage induced manipulation of rkky interaction. Appl. Phys. Lett.124 (2024).
Trényi, R. et al. Activation of metrologically useful genuine multipartite entanglement. New J. Phys. 26, 023034 (2024).
Hahn, E. L. Spin echoes. Phys. Rev. 80, 580–594. https://doi.org/10.1103/PhysRev.80.580 (1950).
Yosida, K. Bound state due to the \(s-d\) exchange interaction. Phys. Rev. 147, 223–227. https://doi.org/10.1103/PhysRev.147.223 (1966).
Allerdt, A., Feiguin, A. E. & Das Sarma, S. Competition between kondo effect and rkky physics in graphene magnetism. Phys. Rev. B95, 104402 (2017). https://doi.org/10.1103/PhysRevB.95.104402.
Doniach, S. The kondo lattice and weak antiferromagnetism. Physica B+C91, 231–234 (1977). https://www.sciencedirect.com/science/article/pii/0378436377901905.
Kroha, J. Interplay of Kondo effect and RKKY interaction. In Pavarini, E., Koch, E., Scalettar, R. & Martin, R. M. (eds.) The Physics of Correlated Insulators, Metals, and Superconductors Modeling and Simulation, vol. 7 (Verlag des Forschungszentrum Jülich, 2017).
Hill, S. A. & Wootters, W. K. Entanglement of a pair of quantum bits. Phys. Rev. Lett. 78, 5022–5025. https://doi.org/10.1103/PhysRevLett.78.5022 (1997).
Wootters, W. K. Entanglement of formation of an arbitrary state of two qubits. Phys. Rev. Lett. 80, 2245–2248. https://doi.org/10.1103/PhysRevLett.80.2245 (1998).
Rungta, P., Bužek, V., Caves, C. M., Hillery, M. & Milburn, G. J. Universal state inversion and concurrence in arbitrary dimensions. Phys. Rev. A 64, 042315. https://doi.org/10.1103/PhysRevA.64.042315 (2001).
Walls, D. F. Squeezed states of light. Nature 306, 141–146 (1983).
Wu, L.-A., Xiao, M. & Kimble, H. Squeezed states of light from an optical parametric oscillator. J. Opt. Soc. Am. B 4, 1465–1475 (1987).
Pirkkalainen, J.-M., Damskägg, E., Brandt, M., Massel, F. & Sillanpää, M. A. Squeezing of quantum noise of motion in a micromechanical resonator. Phys. Rev. Lett. 115, 243601. https://doi.org/10.1103/PhysRevLett.115.243601 (2015).
Marti, S. et al. Quantum squeezing in a nonlinear mechanical oscillator. Nat. Phys. 20, 1448–1453 (2024).
Acknowledgements
One of the authors (S.-H.C.) thanks Chang Yen Jui and Tsung-Wei Huang for valuable discussions.
Funding
S.G.T. was supported by the National Science and Technology Council (NSTC) of Taiwan under Grant No. NSTC 114-2112-M-034-001. C.-R.C. was supported by the NSTC under Grant No. NSTC 114-2112-M-033-005.
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S.-H.C. proposed the setup, conducted the theoretical investigation and performed the numerical simulations and analysis. S.G.T. and C.-R.C. contributed to the device design and the improvement of modeling and device realizability. All authors discussed the results and reviewed the manuscript.
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Chen, SH., Tan, S.G. & Chang, CR. Navigating entanglement via Ruderman–Kittel–Kasuya–Yosida exchange: oscillatory, boundary-residing, pulsed, and damping-stabilized trajectories. Sci Rep (2026). https://doi.org/10.1038/s41598-026-47292-1
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DOI: https://doi.org/10.1038/s41598-026-47292-1


