Table 1 Overview of experiments

Experiment code	Generation method	Temperature (°C)	Aqueous media	Additive type	Additive concentration	Sampling time (h)
A1	jet	30 to 0	ASW	-	-	8^a, -^b, -^c
A2	jet	30 to 0	NSW	-	-	8^a, -^b, -^c
A3	waterfall	30 to 0	ASW	-	-	12^a, -^b, -^c
A4	waterfall	30 to 0	NSW	-	-	12^a, -^b, -^c
B1	jet	0	ASW	SDS	0. 5 μM	-^a, 1^b, 10^c
B2	jet	5	ASW	SDS	0. 5 μM	-^a, 1^b, 10^c
B3	jet	10	ASW	SDS	0. 5 μM	-^a, 1^b, 10^c
B4	jet	15	ASW	SDS	0. 5 μM	-^a, 1^b, 10^c
B5	jet	20	ASW	SDS	0. 5 μM	-^a, 1^b, 10^c
B6	jet	25	ASW	SDS	0. 5 μM	-^a, 1^b, 10^c
C1	jet	0	ASW	Algal DOC	635 ± 31 μM C	-^a, 0.5^b, 10^c
C2	jet	5	ASW	Algal DOC	635 ± 31 μM C	-^a, 0.5^b, 10^c
C3	jet	10	ASW	Algal DOC	635 ± 31 μM C	-^a, 0.5^b, 10^c
C4	jet	15	ASW	Algal DOC	635 ± 31 μM C	-^a, 0.5^b, 10^c
C5	jet	20	ASW	Algal DOC	635 ± 31 μM C	-^a, 0.5^b, 10^c
C6	jet	25	ASW	Algal DOC	635 ± 31 μM C	-^a, 0.5^b, 10^c

“ASW”, “NSW”, “SDS”, and “Algal DOC” stand for artificial seawater, natural seawater, sodium dodecyl sulfate, and algal dissolved organic carbon, respectively. The notations “a”, “b”, and “c” represent the sampling time of SMPS, DKL-2, and DLPI+, respectively.

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