Abstract
Organic electrochemical transistors could be used in in-sensor computing and wearable healthcare applications. However, they lack the conformity and stretchability needed to minimize mechanical mismatch between the devices and human body, are challenging to fabricate at a scale with small feature sizes and high density, and require miniaturized readout systems for practical on-body applications. Here we report a wearable in-sensor computing platform based on stretchable organic electrochemical transistor arrays. The platform offers more than 50% stretchability by using an adhesive supramolecular buffer layer during fabrication that improves robustness at interfaces under strain. We fabricate stretchable transistor arrays with feature sizes down to 100 μm using a high-resolution six-channel inkjet printing system. We also develop a coin-sized data readout system for biosignal acquisition. We show that our coin-sized, smartwatch-compatible electronic module can provide wearable in-sensor edge computing.
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Data availability
Data that support the findings of this study are available from the corresponding authors upon reasonable request.
Code availability
The code used for RC is available via GitHub at https://github.com/HKU-WISE-Group/OECT-RC.
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Acknowledgements
We thank P. K. L. Chan, C. Wong, J. Chan and P. S. Yip from the HKU Central Fabrication Lab for support on device fabrication, N. Wong and X. Meng for discussions on the low-power biochips, K. Wu, S. Xue and C. Li for discussions on materials synthesis, and N. Tien and C. K. Chui for generous support on the printing facilities and wet lab resources at Tam Wing Fan Innovation Wing. S.Z. acknowledges the Collaborative Research Fund (C7005-23Y) and the Theme-based Research Scheme (T45-701/22-R) from the Research Grants Council of the Hong Kong SAR Government; Innovation and Technology Fund (Mainland-Hong Kong Joint Funding Scheme, MHP/053/21, MHP/066/20) from the Hong Kong SAR Government; and the Shenzhen-Hong Kong-Macau Technology Research Programme (SGDX20210823103537034) from the Shenzhen Science and Technology Innovation Committee. The PERfECT readout platform is funded by the HKU Innovation Wing Two Research Fund and Technology Start-up Support Scheme for Universities (TSSSU/HKU/23/13).
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S.Z., Z.W. and D.L. conceived the idea. S.Z. acquired funding and supervised the whole research. D.L., X.T., J.B. and S.W. conducted the experiments and collected the data. X.T., J.B. and S.W. contributed to the algorithm design and simulation. S.Z., X.T. and J.B. designed the PERfECT readout system for wearable data analysis. X.T. and J.B. coded the AI-embedded program in PERfECT for in-sensor computing with an ISOECT array. D.L., X.T., J.B. and Y.W. contributed to the fabrication of the ISOECT array. D.L., X.T., Y.W. and S.D. contributed to the ISOECT device characterization. S.Z. and D.L. drafted the manuscript. All authors contributed to revising the manuscript.
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Liu, D., Tian, X., Bai, J. et al. A wearable in-sensor computing platform based on stretchable organic electrochemical transistors. Nat Electron 7, 1176–1185 (2024). https://doi.org/10.1038/s41928-024-01250-9
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DOI: https://doi.org/10.1038/s41928-024-01250-9


