Skip to main content

Thank you for visiting nature.com. You are using a browser version with limited support for CSS. To obtain the best experience, we recommend you use a more up to date browser (or turn off compatibility mode in Internet Explorer). In the meantime, to ensure continued support, we are displaying the site without styles and JavaScript.

  • Perspective
  • Published:

Sub-diffraction confinement in dielectrics with narwhal wavefunctions

Abstract

The ability to confine light below the diffraction limit — coherently and without loss — has long been considered unattainable in transparent dielectrics. This limitation steered nanophotonics towards plasmonics, in which subwavelength confinement can be achieved at the expense of material absorption. Singular nanophotonics, also called singulonics, is an emerging regime in nanophotonics, which can overcome the trade-off between confinement and loss by leveraging the singular dispersion equation in lossless dielectric media, giving rise to highly localized singular modes, called narwhal wavefunctions. This framework establishes a rigorous, lossless pathway to sub-diffraction confinement, grounded in Maxwell’s equations and governed by the interplay between spatial and momentum uncertainties. This Perspective presents the theoretical foundations and experimental realizations of singular nanophotonics, contrasts it with conventional plasmonic and dielectric approaches and explores its broad implications and challenges.

This is a preview of subscription content, access via your institution

Access options

Buy this article

USD 39.95

Prices may be subject to local taxes which are calculated during checkout

Fig. 1: Dispersion equation of dielectric, plasmonic and singulonic modes.
Fig. 2: Boundary-condition enhancement versus narwhal-wavefunction confinement.
Fig. 3: Quality factor versus inverse of the mode volume with representative optical cavities.
Fig. 4: Field localization enabled by momentum-space mode locking.
Fig. 5: Singular dispersion as a unifying mechanism for atomic-scale photonic applications.

Similar content being viewed by others

References

  1. Stelzer, E. H. K. & Grill, S. The uncertainty principle applied to estimate focal spot dimensions. Opt. Commun. 173, 51–56 (2000).

    Article  ADS  Google Scholar 

  2. Busch, P., Heinonen, T. & Lahti, P. Heisenberg’s uncertainty principle. Phys. Rep. 452, 155–176 (2007).

    Article  ADS  Google Scholar 

  3. Shim, H., Monticone, F. & Miller, O. D. Fundamental limits to the refractive index of transparent optical materials. Adv. Mater. 33, 2103946 (2021).

    Article  Google Scholar 

  4. Khurgin, J. B. Expanding the photonic palette: exploring high index materials. ACS Photon. 9, 743–751 (2022).

    Article  Google Scholar 

  5. Barnes, W. L., Dereux, A. & Ebbesen, T. W. Surface plasmon subwavelength optics. Nature 424, 824–830 (2003).

    Article  ADS  Google Scholar 

  6. Schuller, J. A. et al. Plasmonics for extreme light concentration and manipulation. Nat. Mater. 9, 193–204 (2010).

    Article  ADS  Google Scholar 

  7. Kauranen, M. & Zayats, A. V. Nonlinear plasmonics. Nat. Photon. 6, 737–748 (2012).

    Article  ADS  Google Scholar 

  8. Tame, M. S. et al. Quantum plasmonics. Nat. Phys. 9, 329–340 (2013).

    Article  Google Scholar 

  9. Tsakmakidis, K. L., Hess, O., Boyd, R. W. & Zhang, X. Ultraslow waves on the nanoscale. Science 358, eaan5196 (2017).

    Article  Google Scholar 

  10. Ma, R. M. & Oulton, R. F. Applications of nanolasers. Nat. Nanotechnol. 14, 12–22 (2019).

    Article  ADS  Google Scholar 

  11. Xu, H., Bjerneld, E. J., Käll, M. & Börjesson, L. Spectroscopy of single hemoglobin molecules by surface enhanced Raman scattering. Phys. Rev. Lett. 83, 4357–4360 (1999).

    Article  ADS  Google Scholar 

  12. Akimov, A. V. et al. Generation of single optical plasmons in metallic nanowires coupled to quantum dots. Nature 450, 402–406 (2007).

    Article  ADS  Google Scholar 

  13. Hill, M. T. et al. Lasing in metal–insulator–metal sub-wavelength plasmonic waveguides. Opt. Express 17, 11107–11112 (2009).

    Article  ADS  Google Scholar 

  14. Noginov, M. A. et al. Demonstration of a spaser-based nanolaser. Nature 460, 1110–1112 (2009).

    Article  ADS  Google Scholar 

  15. Oulton, R. F. et al. Plasmon lasers at deep subwavelength scale. Nature 461, 629–632 (2009).

    Article  ADS  Google Scholar 

  16. Ma, R. M., Oulton, R. F., Sorger, V. J., Bartal, G. & Zhang, X. Room-temperature sub-diffraction-limited plasmon laser by total internal reflection. Nat. Mater. 10, 110–113 (2011).

    Article  ADS  Google Scholar 

  17. Zhang, R. et al. Chemical mapping of a single molecule by plasmon-enhanced Raman scattering. Nature 498, 82–86 (2013).

    Article  ADS  Google Scholar 

  18. Marinica, D. C. et al. Active quantum plasmonics. Sci. Adv. 1, e1501095 (2015).

    Article  ADS  Google Scholar 

  19. Chikkaraddy, R. et al. Single-molecule strong coupling at room temperature in plasmonic nanocavities. Nature 535, 127–130 (2016).

    Article  ADS  Google Scholar 

  20. Baumberg, J. J., Aizpurua, J., Mikkelsen, M. H. & Smith, D. R. Extreme nanophotonics from ultrathin metallic gaps. Nat. Mater. 18, 668–678 (2019).

    Article  ADS  Google Scholar 

  21. Wang, Y. et al. Stable, high-performance sodium-based plasmonic devices in the near infrared. Nature 581, 401–405 (2020).

    Article  ADS  Google Scholar 

  22. Khurgin, J. B. How to deal with the loss in plasmonics and metamaterials. Nat. Nanotechnol. 10, 2–6 (2015).

    Article  ADS  Google Scholar 

  23. Ouyang, Y. H., Luan, H. Y., Zhao, Z. W., Mao, W. Z. & Ma, R. M. Singular dielectric nanolaser with atomic-scale field localization. Nature 632, 287–293 (2024).

    Article  ADS  Google Scholar 

  24. Mao, W. Z., Luan, H. Y. & Ma, R.-M. Singulonics: narwhal-shaped wavefunctions for sub-diffraction-limited nanophotonics and imaging. eLight 5, 27 (2025).

    Article  Google Scholar 

  25. Bouhelier, A., Beversluis, M., Hartschuh, A. & Novotny, L. Near-field second-harmonic generation induced by local field enhancement. Phys. Rev. Lett. 90, 013903 (2003).

    Article  ADS  Google Scholar 

  26. Gramotnev, D. K. & Bozhevolnyi, S. I. Plasmonics beyond the diffraction limit. Nat. Photon. 4, 83–91 (2010).

    Article  ADS  Google Scholar 

  27. Hess, O. et al. Active nanoplasmonic metamaterials. Nat. Mater. 11, 573–584 (2012).

    Article  ADS  Google Scholar 

  28. Khajavikhan, M. et al. Thresholdless nanoscale coaxial lasers. Nature 482, 204–207 (2012).

    Article  ADS  Google Scholar 

  29. Hess, O. & Tsakmakidis, K. L. Metamaterials with quantum gain. Science 339, 654–655 (2013).

    Article  ADS  Google Scholar 

  30. Akselrod, G. M. et al. Probing the mechanisms of large purcell enhancement in plasmonic nanoantennas. Nat. Photon. 8, 835–840 (2014).

    Article  ADS  Google Scholar 

  31. Tsakmakidis, K. L., Pickering, T. W., Hamm, J. M., Page, A. F. & Hess, O. Completely stopped and dispersionless light in plasmonic waveguides. Phys. Rev. Lett. 112, 167401 (2014).

    Article  ADS  Google Scholar 

  32. Tsakmakidis, K. L., Boyd, R. W., Yablonovitch, E. & Zhang, X. Large spontaneous-emission enhancements in metallic nanostructures: towards LEDs faster than lasers. Opt. Express 24, 17916–17927 (2016).

    Article  ADS  Google Scholar 

  33. Galanzha, E. I. et al. Spaser as a biological probe. Nat. Commun. 8, 15528 (2017).

    Article  ADS  Google Scholar 

  34. Wang, S. et al. High-yield plasmonic nanolasers with superior stability for sensing in aqueous solution. ACS Photon. 4, 1355–1360 (2017).

    Article  Google Scholar 

  35. Azzam, S. I. et al. Ten years of spasers and plasmonic nanolasers. Light Sci. Appl. 9, 90 (2020).

    Article  ADS  Google Scholar 

  36. Boltasseva, A. & Atwater, H. A. Low-loss plasmonic metamaterials. Science 331, 290–291 (2011).

    Article  ADS  Google Scholar 

  37. Naik, G. V., Shalaev, V. M. & Boltasseva, A. Alternative plasmonic materials: beyond gold and silver. Adv. Mater. 25, 3264–3294 (2013).

    Article  Google Scholar 

  38. Khurgin, J. B. Replacing noble metals with alternative materials in plasmonics and metamaterials: how good an idea? Phil. Trans. R. Soc. A 375, 20160068 (2017).

    Article  ADS  Google Scholar 

  39. Alcaraz Iranzo, D. et al. Probing the ultimate plasmon confinement limits with a van der Waals heterostructure. Science 360, 291–295 (2018).

    Article  ADS  Google Scholar 

  40. Mao, X. R., Shao, Z. K., Luan, H. Y., Wang, S. L. & Ma, R. M. Magic-angle lasers in nanostructured moiré superlattice. Nat. Nanotechnol. 16, 1099–1105 (2021).

    Article  ADS  Google Scholar 

  41. Ma, R. M. et al. Twisted lattice nanocavity with theoretical quality factor exceeding 200 billion. Fundam. Res. 3, 537–543 (2023).

    Article  Google Scholar 

  42. Luan, H. Y., Ouyang, Y. H., Zhao, Z. W., Mao, W. Z. & Ma, R. M. Reconfigurable moiré nanolaser arrays with phase synchronization. Nature 624, 282–288 (2023).

    Article  ADS  Google Scholar 

  43. Hu, S. & Weiss, S. M. Design of photonic crystal cavities for extreme light concentration. ACS Photon. 3, 1647–1653 (2016).

    Article  Google Scholar 

  44. Choi, H., Heuck, M. & Englund, D. Self-similar nanocavity design with ultrasmall mode volume for single-photon nonlinearities. Phys. Rev. Lett. 118, 223605 (2017).

    Article  ADS  Google Scholar 

  45. Hu, S. et al. Experimental realization of deep-subwavelength confinement in dielectric optical resonators. Sci. Adv. 4, eaat2355 (2018).

    Article  ADS  Google Scholar 

  46. Albrechtsen, M. et al. Nanometer-scale photon confinement in topology-optimized dielectric cavities. Nat. Commun. 13, 6281 (2022).

    Article  ADS  Google Scholar 

  47. Babar, A. N. et al. Self-assembled photonic cavities with atomic-scale confinement. Nature 624, 57–63 (2023).

    Article  ADS  Google Scholar 

  48. Xiong, M. et al. A nanolaser with extreme dielectric confinement. Sci. Adv. 11, eadx3865 (2025).

    Article  Google Scholar 

  49. Hajnal, J. V. Singularities in the transverse fields of electromagnetic waves. I. Theory. Proc. R. Soc. Lond. A 414, 433–446 (1987).

    Article  ADS  MathSciNet  Google Scholar 

  50. Hajnal, J. V. Singularities in the transverse fields of electromagnetic waves. II. Observations on the electric field. Proc. R. Soc. Lond. A 414, 447–468 (1987).

    Article  ADS  MathSciNet  Google Scholar 

  51. Hajnal, J. V. Observations of singularities in the electric and magnetic fields of freely propagating microwaves. Proc. R. Soc. Lond. A 430, 413–421 (1990).

    Article  ADS  Google Scholar 

  52. Allen, L., Beijersbergen, M. W., Spreeuw, R. J. C. & Woerdman, J. P. Orbital angular momentum of light and the transformation of Laguerre–Gaussian laser modes. Phys. Rev. A 45, 8185–8189 (1992).

    Article  ADS  Google Scholar 

  53. Dennis, M. R., O’Holleran, K. & Padgett, M. J. Singular optics: optical vortices and polarization singularities. Prog. Opt. 53, 293–363 (2009).

    Article  ADS  Google Scholar 

  54. Wang, X. Y., Chen, H. Z., Li, Y., Li, B. & Ma, R. M. Microscale vortex laser with controlled topological charge. Chin. Phys. B 25, 124211 (2016).

    Article  ADS  Google Scholar 

  55. Chen, H. Z. et al. Revealing the missing dimension at an exceptional point. Nat. Phys. 16, 571–578 (2020).

    Article  Google Scholar 

  56. Yang, Z. Q., Shao, Z. K., Chen, H. Z., Mao, X. R. & Ma, R. M. Spin-momentum-locked edge mode for topological vortex lasing. Phys. Rev. Lett. 125, 013903 (2020).

    Article  ADS  Google Scholar 

  57. Ni, J. et al. Multidimensional phase singularities in nanophotonics. Science 374, eabj0039 (2021).

    Article  Google Scholar 

  58. Sang, Y. G. et al. Topological polarization singular lasing with highly efficient radiation channel. Nat. Commun. 13, 6485 (2022).

    Article  ADS  Google Scholar 

  59. Wang, X. Y. et al. Vortex radiation from a single emitter in a chiral plasmonic nanocavity. Nanophotonics 11, 1905–1911 (2022).

    Article  Google Scholar 

  60. Berry, M. V. The singularities of light: intensity, phase, polarisation. Light Sci. Appl. 12, 238 (2023).

    Article  ADS  Google Scholar 

  61. Sommerfeld, A. Mathematische Theorie der Diffraction: mit einer tafel. Math. Ann. 47, 317–374 (1896).

    Article  MathSciNet  Google Scholar 

  62. Meixner, J. The behavior of electromagnetic fields at edges. IEEE Trans. Antennas Propag. 20, 442–446 (1972).

    Article  ADS  Google Scholar 

  63. Nie, S. & Emory, S. R. Probing single molecules and single nanoparticles by surface-enhanced Raman scattering. Science 275, 1102–1106 (1997).

    Article  Google Scholar 

  64. Xu, H., Aizpurua, J., Käll, M. & Apell, P. Electromagnetic contributions to single-molecule sensitivity in surface-enhanced Raman scattering. Phys. Rev. E 62, 4318–4324 (2000).

    Article  ADS  Google Scholar 

  65. Gramotnev, D. K. & Bozhevolnyi, S. I. Nanofocusing of electromagnetic radiation. Nat. Photon. 8, 13–22 (2014).

    Article  ADS  Google Scholar 

  66. Li, Y. et al. Boosting light−matter interactions in plasmonic nanogaps. Adv. Mater. 36, 2405186 (2024).

    Article  Google Scholar 

  67. Stewart, M. E. et al. Nanostructured plasmonic sensors. Chem. Rev. 108, 494–521 (2008).

    Article  Google Scholar 

  68. Ma, R. M., Ota, S., Li, Y., Yang, S. & Zhang, X. Explosives detection in a lasing plasmon nanocavity. Nat. Nanotechnol. 9, 600–604 (2014).

    Article  ADS  Google Scholar 

  69. Wang, X. Y. et al. Lasing enhanced surface plasmon resonance sensing. Nanophotonics 6, 472–478 (2017).

    Article  Google Scholar 

  70. Lee, J., Crampton, K. T., Tallarida, N. & Apkarian, V. A. Visualizing vibrational normal modes of a single molecule with atomically confined light. Nature 568, 78–82 (2019).

    Article  ADS  Google Scholar 

  71. Zhang, Z., Nest, L., Wang, S., Wang, S. Y. & Ma, R. M. Lasing-enhanced surface plasmon resonance spectroscopy and sensing. Photon. Res. 9, 1699–1714 (2021).

    Article  Google Scholar 

  72. Mühlschlegel, P., Eisler, H. J., Martin, O. J. F., Hecht, B. & Pohl, D. W. Resonant optical antennas. Science 308, 1607–1609 (2005).

    Article  ADS  Google Scholar 

  73. Kim, S. et al. High-harmonic generation by resonant plasmon field enhancement. Nature 453, 757–760 (2008).

    Article  ADS  Google Scholar 

  74. Kinkhabwala, A. et al. Large single-molecule fluorescence enhancements produced by a bowtie nanoantenna. Nat. Photon. 3, 654–657 (2009).

    Article  ADS  Google Scholar 

  75. Yu, N. et al. Bowtie plasmonic quantum cascade laser antenna. Opt. Express 15, 13272–13281 (2007).

    Article  ADS  Google Scholar 

  76. Suh, J. Y. et al. Plasmonic bowtie nanolaser arrays. Nano Lett. 12, 5769–5774 (2012).

    Article  ADS  Google Scholar 

  77. Mie, G. Beiträge zur optik trüber medien, speziell kolloidaler metallösungen. Ann. Phys. 330, 377–445 (1908).

    Article  Google Scholar 

  78. Kuznetsov, A. I., Miroshnichenko, A. E., Brongersma, M. L., Kivshar, Y. S. & Luk’yanchuk, B. Optically resonant dielectric nanostructures. Science 354, aag2472 (2016).

    Article  Google Scholar 

  79. Berry, M. V. Logarithmic pinpricks in wavefunctions. Eur. J. Phys. 45, 025304 (2024).

    Article  Google Scholar 

  80. Kato, T. Perturbation Theory of Linear Operators (Springer, 1966).

  81. Miri, M.-A. & Alù, A. Exceptional points in optics and photonics. Science 363, eaar7709 (2019).

    Article  MathSciNet  Google Scholar 

  82. Yu, N. et al. Light propagation with phase discontinuities: generalized laws of reflection and refraction. Science 334, 333–337 (2011).

    Article  ADS  Google Scholar 

  83. Sun, S. et al. Gradient-index meta-surfaces as a bridge linking propagating waves and surface waves. Nat. Mater. 11, 426–431 (2012).

    Article  ADS  Google Scholar 

  84. Schulz, S. A. et al. Roadmap on photonic metasurfaces. Appl. Phys. Lett. 124, 260701 (2024).

    Article  ADS  Google Scholar 

  85. Ha, S. T. et al. Directional lasing in resonant semiconductor nanoantenna arrays. Nat. Nanotechnol. 13, 1042–1047 (2018).

    Article  ADS  Google Scholar 

  86. Liu, S. et al. Resonantly enhanced second-harmonic generation using III–V semiconductor all-dielectric metasurfaces. Nano Lett. 16, 5426–5432 (2016).

    Article  ADS  Google Scholar 

  87. Koshelev, K. et al. Subwavelength dielectric resonators for nonlinear nanophotonics. Science 367, 288–292 (2020).

    Article  ADS  Google Scholar 

  88. Almeida, V. R., Xu, Q., Barrios, C. A. & Lipson, M. Guiding and confining light in void nanostructure. Opt. Lett. 29, 1209–1211 (2004).

    Article  ADS  Google Scholar 

  89. Kita, S., Hachuda, S., Nozaki, K. & Baba, T. Nanoslot laser. Appl. Phys. Lett. 97, 161108 (2010).

    Article  ADS  Google Scholar 

  90. Wu, H. et al. Photonic nanolaser with extreme optical field confinement. Phys. Rev. Lett. 129, 013902 (2022).

    Article  ADS  Google Scholar 

  91. Barrios, C. A. et al. Slot-waveguide biochemical sensor. Opt. Lett. 32, 3080–3082 (2007).

    Article  ADS  Google Scholar 

  92. Dell’Olio, F. & Passaro, V. M. Optical sensing by optimized silicon slot waveguides. Opt. Express 15, 4977–4993 (2007).

    Article  ADS  Google Scholar 

  93. Baehr-Jones, T. et al. Nonlinear polymer-clad silicon slot waveguide modulator with a half wave voltage of 0.25 V. Appl. Phys. Lett. 92, 163303 (2008).

    Article  ADS  Google Scholar 

  94. Koos, C. et al. All-optical high-speed signal processing with silicon–organic hybrid slot waveguides. Nat. Photon. 3, 216–219 (2009).

    Article  ADS  Google Scholar 

  95. Lu, Q., Shu, F.-J. & Zou, C.-L. Extremely local electric field enhancement and light confinement in dielectric waveguide. IEEE Photon. Technol. Lett. 26, 1426–1429 (2014).

    Article  ADS  Google Scholar 

  96. Vernooy, D. W., Ilchenko, V. S., Mabuchi, H., Streed, E. W. & Kimble, H. J. High-Q measurements of fused-silica microspheres in the near infrared. Opt. Lett. 23, 247–249 (1998).

    Article  ADS  Google Scholar 

  97. Kippenberg, T. J., Spillane, S. M. & Vahala, K. J. Demonstration of ultra-high-Q small mode volume toroid microcavities on a chip. Appl. Phys. Lett. 85, 6113–6115 (2004).

    Article  ADS  Google Scholar 

  98. Spillane, S. M. et al. Ultrahigh-Q toroidal microresonators for cavity quantum electrodynamics. Phys. Rev. A 71, 013817 (2005).

    Article  ADS  Google Scholar 

  99. Del’Haye, P. et al. Optical frequency comb generation from a monolithic microresonator. Nature 450, 1214–1217 (2007).

    Article  ADS  Google Scholar 

  100. Savchenkov, A. A., Matsko, A. B., Ilchenko, V. S. & Maleki, L. Optical resonators with ten million finesse. Opt. Express 15, 6768–6773 (2007).

    Article  ADS  Google Scholar 

  101. Pöllinger, M., O’Shea, D., Warken, F. & Rauschenbeutel, A. Ultrahigh-Q tunable whispering-gallery-mode microresonator. Phys. Rev. Lett. 103, 053901 (2009).

    Article  ADS  Google Scholar 

  102. Zhu, J. et al. On-chip single nanoparticle detection and sizing by mode splitting in an ultrahigh-Q microresonator. Nat. Photon. 4, 46–49 (2010).

    Article  ADS  Google Scholar 

  103. Jiang, X. et al. Chaos-assisted broadband momentum transformation in optical microresonators. Science 358, 344–347 (2017).

    Article  ADS  Google Scholar 

  104. Shitikov, A. E. et al. Billion Q-factor in silicon WGM resonators. Optica 5, 1525–1528 (2018).

    Article  ADS  Google Scholar 

  105. Song, B. S., Noda, S., Asano, T. & Akahane, Y. Ultra-high-Q photonic double-heterostructure nanocavity. Nat. Mater. 4, 207–210 (2005).

    Article  ADS  Google Scholar 

  106. Quan, Q. & Lončar, M. Deterministic design of wavelength scale, ultra-high Q photonic crystal nanobeam cavities. Opt. Express 19, 18529–18542 (2011).

    Article  ADS  Google Scholar 

  107. Lai, Y. et al. Genetically designed L3 photonic crystal nanocavities with measured quality factor exceeding one million. Appl. Phys. Lett. 104, 241101 (2014).

    Article  ADS  Google Scholar 

  108. Alpeggiani, F., Andreani, L. C. & Gerace, D. Effective bichromatic potential for ultra-high Q-factor photonic crystal slab cavities. Appl. Phys. Lett. 107, 261110 (2015).

    Article  ADS  Google Scholar 

  109. Minkov, M., Savona, V. & Gerace, D. Photonic crystal slab cavity simultaneously optimized for ultra-high Q/V and vertical radiation coupling. Appl. Phys. Lett. 111, 131104 (2017).

    Article  ADS  Google Scholar 

  110. Asano, T., Ochi, Y., Takahashi, Y., Kishimoto, K. & Noda, S. Photonic crystal nanocavity with a Q factor exceeding eleven million. Opt. Express 25, 1769–1777 (2017).

    Article  ADS  Google Scholar 

  111. Asano, T. & Noda, S. Optimization of photonic crystal nanocavities based on deep learning. Opt. Express 26, 32704–32717 (2018).

    Article  ADS  Google Scholar 

  112. Li, M. et al. Photon-level tuning of photonic nanocavities. Optica 6, 860–863 (2019).

    Article  ADS  Google Scholar 

  113. Song, B. S. et al. Ultrahigh-Q photonic crystal nanocavities based on 4H silicon carbide. Optica 6, 991–995 (2019).

    Article  ADS  Google Scholar 

  114. Ciracì, C. et al. Probing the ultimate limits of plasmonic enhancement. Science 337, 1072–1074 (2012).

    Article  ADS  Google Scholar 

  115. Kern, J. et al. Atomic-scale confinement of resonant optical fields. Nano Lett. 12, 5504–5509 (2012).

    Article  ADS  Google Scholar 

  116. Epstein, I. et al. Far-field excitation of single graphene plasmon cavities with ultracompressed mode volumes. Science 368, 1219–1223 (2020).

    Article  ADS  Google Scholar 

  117. Li, W., Zhou, Q., Zhang, P. & Chen, X. W. Bright optical eigenmode of 1 nm3 mode volume. Phys. Rev. Lett. 126, 257401 (2021).

    Article  ADS  Google Scholar 

  118. Liu, Z. et al. High-Q quasibound states in the continuum for nonlinear metasurfaces. Phys. Rev. Lett. 123, 253901 (2019).

    Article  ADS  Google Scholar 

  119. Chen, Z. et al. Observation of miniaturized bound states in the continuum with ultra-high quality factors. Sci. Bull. 67, 359–366 (2021).

    Article  Google Scholar 

  120. Yu, Y. et al. Ultra-coherent Fano laser based on a bound state in the continuum. Nat. Photon. 15, 758–764 (2021).

    Article  ADS  Google Scholar 

  121. Khurgin, J. B. Light slowing down in moiré fiber gratings and its implications for nonlinear optics. Phys. Rev. A 62, 013821 (2000).

    Article  ADS  Google Scholar 

  122. Raun, A., Tang, H., Ni, X., Mazur, E. & Hu, E. L. GaN magic angle laser in a merged moiré photonic crystal. ACS Photon. 10, 3001–3007 (2023).

    Article  Google Scholar 

  123. Guan, J. et al. Far-field coupling between moiré photonic lattices. Nat. Nanotechnol. 18, 514–520 (2023).

    Article  ADS  Google Scholar 

  124. Wang, X. et al. Experimental demonstration of high-efficiency harmonic generation in photonic moiré superlattice microcavities. Nano Lett. 24, 11327–11333 (2024).

    Article  ADS  Google Scholar 

  125. Ji, Y. et al. Giantly enhancing harmonic generations by a moiré superlattice nanocavity. Photon. Res. 13, 2697 (2025).

    Article  Google Scholar 

  126. Yan, S. et al. Cavity quantum electrodynamics with moiré photonic crystal nanocavity. Nat. Commun. 16, 4634 (2025).

    Article  ADS  Google Scholar 

  127. Wang, Y. T. et al. Moiré cavity quantum electrodynamics. Sci. Adv. 11, eadv8115 (2025).

    Article  ADS  Google Scholar 

  128. Chen, J. et al. Magic-angle magnonic nanocavity in a magnetic moiré superlattice. Phys. Rev. B 105, 094445 (2022).

    Article  ADS  Google Scholar 

  129. Jin, F. et al. Exciton polariton condensation in a perovskite moiré flat band at room temperature. Sci. Adv. 11, eadx2361 (2025).

    Article  ADS  Google Scholar 

  130. Hopfield, J. J. & Thomas, D. G. Theoretical and experimental effects of spatial dispersion on the optical properties of crystals. Phys. Rev. 132, 563–572 (1963).

    Article  ADS  Google Scholar 

  131. Khurgin, J. B. Ultimate limit of field confinement by surface plasmon polaritons. Faraday Discuss. 178, 109–122 (2015).

    Article  ADS  Google Scholar 

  132. Raza, S. Nonlocal optical response in metallic nanostructures. J. Phys. Condens. Matter 27, 183204 (2015).

    Article  ADS  Google Scholar 

  133. Khurgin, J., Tsai, W. Y., Tsai, D. P. & Sun, G. Landau damping and limit to field confinement and enhancement in plasmonic dimers. ACS Photon. 4, 2871–2880 (2017).

    Article  Google Scholar 

  134. Monticone, F. et al. Nonlocality in photonic materials and metamaterials: roadmap. Opt. Mater. Express 15, 1544–1709 (2025).

    Article  ADS  Google Scholar 

  135. Ma, R. M. Nanolaser technology with atomic-scale field localization. Nat. Rev. Electr. Eng. 1, 632–633 (2024).

    Article  Google Scholar 

  136. Yokoyama, H. & Brorson, S. D. Rate equation analysis of microcavity lasers. J. Appl. Phys. 66, 4801–4805 (1989).

    Article  ADS  Google Scholar 

  137. Yokoyama, H. et al. Controlling spontaneous emission and threshold-less laser oscillation with optical microcavities. Opt. Quant. Electron. 24, S245–S272 (1992).

    Article  Google Scholar 

  138. Altug, H., Englund, D. & Vučković, J. Ultrafast photonic crystal nanocavity laser. Nat. Phys. 2, 484–488 (2006).

    Article  Google Scholar 

  139. Ma, R. M., Oulton, R. F., Sorger, V. J. & Zhang, X. Plasmon lasers: coherent light source at molecular scales. Laser Photon. Rev. 7, 1–21 (2013).

    Article  ADS  Google Scholar 

  140. Hill, M. T. & Gather, M. C. Advances in small lasers. Nat. Photon. 8, 908–918 (2014).

    Article  ADS  Google Scholar 

  141. Wang, S. et al. Unusual scaling laws for plasmonic nanolasers beyond the diffraction limit. Nat. Commun. 8, 1889 (2017).

    Article  ADS  Google Scholar 

  142. Wang, S. L., Wang, S., Man, X. K. & Ma, R. M. Loss and gain in a plasmonic nanolaser. Nanophotonics 9, 3403–3408 (2020).

    Article  Google Scholar 

  143. Ma, R. M. Lasing under ultralow pumping. Nat. Mater. 18, 1152–1153 (2019).

    Article  ADS  Google Scholar 

  144. Dai, S. et al. Tunable phonon polaritons in atomically thin van der Waals crystals of boron nitride. Science 343, 1125–1129 (2014).

    Article  ADS  Google Scholar 

  145. Ma, W. et al. In-plane anisotropic and ultra-low-loss polaritons in a natural van der Waals crystal. Nature 562, 557–562 (2018).

    Article  ADS  Google Scholar 

  146. Hu, G. et al. Topological polaritons and photonic magic angles in twisted α-MoO3 bilayers. Nature 582, 209–213 (2020).

    Article  ADS  Google Scholar 

  147. Purcell, E. M. Spontaneous emission probabilities at radio frequencies. Phys. Rev. 69, 681 (1946).

    Google Scholar 

  148. Jaynes, E. T. & Cummings, F. W. Comparison of quantum and semiclassical radiation theories with application to the beam maser. Proc. IEEE 51, 89–109 (1963).

    Article  ADS  Google Scholar 

  149. Haroche, S. & Kleppner, D. Cavity quantum electrodynamics. Phys. Today 42, 24–30 (1989).

    Article  ADS  Google Scholar 

  150. Vahala, K. J. Optical microcavities. Nature 424, 839–846 (2003).

    Article  ADS  Google Scholar 

  151. Haroche, S. Nobel Lecture: controlling photons in a box and exploring the quantum to classical boundary. Rev. Mod. Phys. 85, 1083–1102 (2013).

    Article  ADS  Google Scholar 

  152. Frisk Kockum, A., Miranowicz, A., De Liberato, S., Savasta, S. & Nori, F. Ultrastrong coupling between light and matter. Nat. Rev. Phys. 1, 19–40 (2019).

    Article  Google Scholar 

  153. Raimond, J. M., Brune, M. & Haroche, S. Colloquium: manipulating quantum entanglement with atoms and photons in a cavity. Rev. Mod. Phys. 73, 565 (2001).

    Article  ADS  MathSciNet  Google Scholar 

  154. Yoshie, T. et al. Vacuum Rabi splitting with a single quantum dot in a photonic crystal nanocavity. Nature 432, 200–203 (2004).

    Article  ADS  Google Scholar 

  155. Birnbaum, K. M. et al. Photon blockade in an optical cavity with one trapped atom. Nature 436, 87–90 (2005).

    Article  ADS  Google Scholar 

  156. Tiecke, T. G. et al. Nanophotonic quantum phase switch with a single atom. Nature 508, 241–244 (2014).

    Article  ADS  Google Scholar 

  157. Reiserer, A. & Rempe, G. Cavity-based quantum networks with single atoms and optical photons. Rev. Mod. Phys. 87, 1379–1418 (2015).

    Article  ADS  Google Scholar 

  158. Lu, C. Y. & Pan, J. W. Quantum-dot single-photon sources for the quantum internet. Nat. Nanotechnol. 16, 1294–1296 (2021).

    Article  ADS  Google Scholar 

  159. Betzig, E. & Trautman, J. K. Near-field optics: microscopy, spectroscopy, and surface modification beyond the diffraction limit. Science 257, 189–195 (1992).

    Article  ADS  Google Scholar 

  160. Chen, X. et al. Modern scattering type scanning near-field optical microscopy for advanced material research. Adv. Mater. 31, 1804774 (2019).

    Article  Google Scholar 

  161. Di Francia, G. T. Super-gain antennas and optical resolving power. Nuovo Cimento Suppl. 9, 426–438 (1952).

    Article  Google Scholar 

  162. Berry, M. V. Evanescent and real waves in quantum billiards and Gaussian beams. J. Phys. A Math. Gen. 27, L391–L398 (1994).

    Article  ADS  MathSciNet  Google Scholar 

  163. Berry, M. V. & Jeffrey, M. R. Progress in Optics Vol. 50, 13–50 (Elsevier, 2007).

  164. Rogers, E. T. F. et al. A super-oscillatory lens optical microscope for subwavelength imaging. Nat. Mater. 11, 432–435 (2012).

    Article  ADS  Google Scholar 

  165. Berry, M. et al. Roadmap on superoscillations. J. Opt. 21, 053002 (2019).

    Article  ADS  Google Scholar 

  166. Hell, S. W. & Wichmann, J. Breaking the diffraction resolution limit by stimulated emission: stimulated-emission-depletion fluorescence microscopy. Opt. Lett. 19, 780 (1994).

    Article  ADS  Google Scholar 

  167. Blom, H. & Widengren, J. Stimulated emission depletion microscopy. Chem. Rev. 117, 7377–7427 (2017).

    Article  Google Scholar 

  168. Gustafsson, M. G. L. Surpassing the lateral resolution limit by a factor of two using structured illumination microscopy. J. Microsc. 198, 82–87 (2000).

    Article  Google Scholar 

  169. Heintzmann, R. & Huser, T. Super-resolution structured illumination microscopy. Chem. Rev. 117, 13890–13908 (2017).

    Article  Google Scholar 

  170. Dutt, A., Mohanty, A., Gaeta, A. L. & Lipson, M. Nonlinear and quantum photonics using integrated optical materials. Nat. Rev. Mater. 9, 321–346 (2024).

    Article  ADS  Google Scholar 

  171. Chen, H. et al. Sub-50-ns ultrafast upconversion luminescence of a rare-earth-doped nanoparticle. Nat. Photon. 16, 651–657 (2022).

    Article  ADS  Google Scholar 

  172. Chen, Y. Nanofabrication by electron beam lithography and its applications: a review. Microelectron. Eng. 135, 57–72 (2015).

    Article  Google Scholar 

  173. Scholder, O. et al. Helium focused ion beam fabricated plasmonic antennas with sub-5 nm gaps. Nanotechnology 24, 395301 (2013).

    Article  Google Scholar 

  174. Mortensen, N. et al. A generalized non-local optical response theory for plasmonic nanostructures. Nat. Commun. 5, 3809 (2014).

    Article  ADS  Google Scholar 

  175. Esteban, R. et al. Bridging quantum and classical plasmonics with a quantum-corrected model. Nat. Commun. 3, 825 (2012).

    Article  ADS  Google Scholar 

  176. Teperik, T. V., Nordlander, P., Aizpurua, J. & Borisov, A. G. Robust subnanometric plasmon ruler by rescaling of the nonlocal optical response. Phys. Rev. Lett. 110, 263901 (2013).

    Article  ADS  Google Scholar 

  177. Toscano, G. et al. Resonance shifts and spill-out effects in self-consistent hydrodynamic nanoplasmonics. Nat. Commun. 6, 7132 (2015).

    Article  ADS  Google Scholar 

  178. Buhmann, S. Y. Dispersion Forces I: Macroscopic Quantum Electrodynamics and Ground-State Casimir, Casimir–Polder and van der Waals Forces. Springer Tracts in Modern Physics Vol. 247 (Springer, 2012).

Download references

Acknowledgements

This work is supported by the National Natural Science Foundation of China (grant nos 12225402, 12450005, 62321004 and 92250302), the National Key R&D Program of China (grant no. 2022YFA1404700) and the New Cornerstone Science Foundation through the XPLORER PRIZE. K.L.T. acknowledges support for this research by the General Secretariat for Research and Technology and the Hellenic Foundation for Research and Innovation (HFRI) under Grant no. 4509. K.L.T.’s part was also carried out within the framework of the National Recovery and Resilience Plan Greece 2.0, funded by the European Union — Next Generation EU (Implementation body: HFRI) under Grant no. 16909.

Author information

Authors and Affiliations

Authors

Contributions

R.-M.M. drafted the manuscript. All authors discussed and revised the manuscript.

Corresponding author

Correspondence to Ren-Min Ma  (马仁敏).

Ethics declarations

Competing interests

The authors declare no competing interests.

Peer review

Peer review information

Nature Reviews Physics thanks Qingdong Ou and the other, anonymous, reviewer(s) for their contribution to the peer review of this work.

Additional information

Publisher’s note Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Rights and permissions

Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Ma, RM., Tsakmakidis, K.L., Luan, HY. et al. Sub-diffraction confinement in dielectrics with narwhal wavefunctions. Nat Rev Phys 8, 240–252 (2026). https://doi.org/10.1038/s42254-026-00924-x

Download citation

  • Accepted:

  • Published:

  • Version of record:

  • Issue date:

  • DOI: https://doi.org/10.1038/s42254-026-00924-x

Search

Quick links

Nature Briefing

Sign up for the Nature Briefing newsletter — what matters in science, free to your inbox daily.

Get the most important science stories of the day, free in your inbox. Sign up for Nature Briefing