Time-resolved lightwave-driven scanning tunnelling spectroscopy is developed to investigate how the spin–orbit-split energy levels of a selenium vacancy within a WSe2 monolayer shift under phonon displacement. Ultrafast snapshots of the electronic tunnelling spectra reveal transient energy shifts up to 40 meV.
- C. Roelcke
- L. Z. Kastner
- Y. A. Gerasimenko
