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Showing 1–3 of 3 results
Advanced filters: Author: Aditya Prajapati Clear advanced filters

  • Precise control of the oxidant — that is, preventing overoxidation — is the missing link in low-temperature methane upgrading. Now, the electro-splitting of carbonate on rutile IrO2 is shown to cover the surface with on-top oxygen adatoms that act as tethered, single-step hydrogen abstractors. One subset can pull the hydrogen from methane to form a methoxy intermediate, while the neighbouring site can protonate this intermediate to form methanol. Together, this mechanism delivers a room-temperature conversion of methane to methanol with >90% selectivity.

    • Aditya Prajapati
    News & Views
    Nature Catalysis
    Volume: 8, P: 629-630

  • This Perspective argues that early assessments of technology-market fit, as well as how the physics governing system performance evolves with scale, can de-risk technology development and accelerate deployment. The authors highlight tools and processes that can be used to assess both these factors at an early stage.

    • Thomas Moore
    • Andrew A. Wong
    • Sarah E. Baker
    Reviews
    Nature Chemical Engineering
    Volume: 1, P: 731-740

  • In situ and operando techniques are useful towards mechanistic investigations of electrocatalytic systems but must be carried out and interpreted properly. Here, the authors provide a set of guidelines for best practices in the use these methods.

    • Aditya Prajapati
    • Christopher Hahn
    • Nikolay Kornienko
    ReviewsOpen Access
    Nature Communications
    Volume: 16, P: 1-20