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Showing 1–2 of 2 results
Advanced filters: Author: Alexander V. Soudackov Clear advanced filters

  • Although interfacial proton-coupled electron transfers are critical reaction steps in chemical and biological processes, studies investigating these reactions are complicated by surface heterogeneity. Now, interfacial proton-coupled electron transfer kinetics are studied and modelled at isolated, well-defined active sites to provide a foundation for understanding complex reactions involved in energy conversion and catalysis.

    • Noah B. Lewis
    • Ryan P. Bisbey
    • Yogesh Surendranath
    Research
    Nature Chemistry
    Volume: 16, P: 343-352

  • Kinetic isotope effect studies can provide valuable insights into the complex mechanisms of the oxygen reduction reaction; however, inaccessibility to ultra-high-purity D2O has made this difficult. Now, a methodology to prepare ultra-pure D2O has been developed and inverse kinetic isotope effects have subsequently been measured for the oxygen reduction reaction on platinum single-crystal surfaces, providing mechanistic insights.

    • Yao Yang
    • Rishi G. Agarwal
    • Héctor D. Abruña
    Research
    Nature Chemistry
    Volume: 15, P: 271-277