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Showing 1–5 of 5 results
Advanced filters: Author: Andreas F. M. Kilbinger Clear advanced filters

  • Ring-opening metathesis polymerization (ROMP) offers good control over dispersity, but the requirement of one initiator per chain can be expensive and problematic for purification. Now, a reversible cyclohexenyl-containing chain-transfer agent is described, thus allowing a catalytic living ROMP process to produce narrow dispersity polymers and block copolymers.

    • Amit A. Nagarkar
    • Andreas F. M. Kilbinger
    Research
    Nature Chemistry
    Volume: 7, P: 718-723

  • Two phosphine-based reagents can be used to prepare aromatic acid chlorides in the presence of either primary or secondary amines. This approach enables the living polycondensation of aromatic amino acids under mild conditions and can be used to make block copolymers as well as helical aromatic amide foldamers.

    • Subhajit Pal
    • Dinh Phuong Trinh Nguyen
    • Andreas F. M. Kilbinger
    Research
    Nature Chemistry
    Volume: 13, P: 705-713

  • In a ruthenium-catalysed living ring-opening metathesis polymerization, one metal centre is required for each polymer chain, and this requires high catalyst loadings when aiming for short polymer chains. Now, it has been shown that a degenerative reversible chain-transfer process enables the synthesis of ring-opened metathesis polymers with controlled molecular weight, using only catalytic amounts of a ruthenium complex.

    • Mohammad Yasir
    • Peng Liu
    • Andreas F. M. Kilbinger
    Research
    Nature Chemistry
    Volume: 11, P: 488-494

  • Ring-opening metathesis polymerization (ROMP) is a powerful and highly functional-group-tolerant technique for synthesizing polymers. However, this tolerance presents a great challenge for the selective introduction of functional end-groups. This Review discusses currently available end-functionalization strategies and also highlights factors to be considered when choosing the most appropriate approach.

    • Stefan Hilf
    • Andreas F. M. Kilbinger
    Reviews
    Nature Chemistry
    Volume: 1, P: 537-546