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Showing 1–5 of 5 results
Advanced filters: Author: Daniel T. Gryko Clear advanced filters

  • Multi component reactions (MCRs) can build complex scaffolds from multiple starting materials in just one step without purification of intermediates but until now MCRs have been discovered rather than designed. Here, the authors demonstrate an algorithmic approach based in the knowledge of reaction mechanisms and rules of physical-organic chemistry to design autonomously MCRs in large numbers.

    • Rafał Roszak
    • Louis Gadina
    • Bartosz A. Grzybowski
    ResearchOpen Access
    Nature Communications
    Volume: 15, P: 1-13

  • The selectivity and activity of enzymes is largely attributed to the well-defined cavities around their active sites, defined by the secondary coordination sphere. Here, the authors show that similar strategies may be applied to tune the selectivity of synthetic rhodium hydroformylation catalysts.

    • Vladica Bocokić
    • Ayfer Kalkan
    • Joost N. H. Reek
    Research
    Nature Communications
    Volume: 4, P: 1-9

  • Heteroatom doping of buckybowls is a viable route to tune their intrinsic physico-chemical properties, but their synthesis remains challenging. Here, the authors report on a combined in-solution and on-surface synthetic strategy towards the fabrication of a buckybowl containing two fused nitrogen-doped pentagonal rings.

    • Shantanu Mishra
    • Maciej Krzeszewski
    • Daniel T. Gryko
    ResearchOpen Access
    Nature Communications
    Volume: 9, P: 1-9

  • Owing to their electron-withdrawing nature, nitro-groups are desirable in the design of electron-deficient light-sensitizing aromatic π-conjugated molecules, but most nitro-aromatics are not fluorescent. Here, the authors show how balanced donor-acceptor coupling ensures fast radiative deactivation and slow intersystem crossing in bis-nitrotetraphenylpyrrolopyrroles.

    • Yevgen M. Poronik
    • Glib V. Baryshnikov
    • Valentine I. Vullev
    ResearchOpen Access
    Communications Chemistry
    Volume: 3, P: 1-18