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Showing 1–3 of 3 results
Advanced filters: Author: Giovanni Bistoni Clear advanced filters

  • An unsymmetric, strong and confined chiral acid, a highly fluorinated imino-imidodiphosphate, catalyses the selective conversion of neral to (1R,6S)-trans-isopiperitenol, enabling sustainable routes to menthol and cannabinoids.

    • Joyce A. A. Grimm
    • Hui Zhou
    • Benjamin List
    ResearchOpen Access
    Nature
    Volume: 615, P: 634-639

  • Utilizing the electrophilicity of ambiphilic silyl nitronates in asymmetric synthesis has remained elusive. Now, silylium-based Lewis acids are used for their activation, achieving the catalytic asymmetric nucleophilic addition of silyl ketene acetals to silyl nitronates for the synthesis of β3-amino acids.

    • Sayantani Das
    • Benjamin Mitschke
    • Benjamin List
    ResearchOpen Access
    Nature Catalysis
    Volume: 4, P: 1043-1049

  • Precursors for the release of phosphorus mononitride in solution under mild conditions have remained elusive. Now, an explosive anthracene-stabilized azidophosphine has shown PN transfer reactivity in the synthesis of an Fe–NP complex. The PN ligand is N-bonded, as the Fe–N interaction shows significant covalent character and a less unfavourable Pauli repulsion than its Fe–P counterpart.

    • André K. Eckhardt
    • Martin-Louis Y. Riu
    • Christopher C. Cummins
    Research
    Nature Chemistry
    Volume: 14, P: 928-934