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Showing 1–6 of 6 results
Advanced filters: Author: Leon Jacobse Clear advanced filters

  • Electrocatalyst degradation driven by oxidation is a major barrier to a sustainable energy society. Here, the authors study the oxidation of Pt(111), a prominent model system, under oxygen evolution conditions, resolving self-limiting layer-by-layer growth of a sub-nanometer disordered PtO2 film.

    • Leon Jacobse
    • Ralf Schuster
    • Andreas Stierle
    ResearchOpen Access
    Nature Communications
    Volume: 17, P: 1-9

  • The oxygen evolution reaction proceeds over a surface that undergoes (frustrated) phase transitions to accommodate bias-dependent excess charge. Now it has been shown that this excess charge is intimately linked to the interfacial solvation of ions and the pre-organization of the transition state, providing insight into intrinsic catalyst activities.

    • Ricardo Martínez-Hincapié
    • Janis Timoshenko
    • Sebastian Z. Oener
    ResearchOpen Access
    Nature Chemistry
    Volume: 18, P: 835-843

  • Two Co single crystal surfaces remain metallic up to 1 bar during Fischer-Tropsch synthesis. The observed intermediates support the carbide mechanism as the reaction pathway. By adding and removing CO we can follow the dynamics of the (dis)appearance of intermediates.

    • Patrick Lömker
    • David Degerman
    • Anders Nilsson
    ResearchOpen Access
    Nature Communications
    Volume: 16, P: 1-10

  • In homoepitaxial crystal growth, four established modes describe atom deposition on a single crystal surface. Here the authors present a model that shows that, for each adatom growth mode, there exists an analogous but inverse version for vacancy growth. This also applies to combined growth.

    • Marcel J. Rost
    • Leon Jacobse
    • Marc T. M. Koper
    ResearchOpen Access
    Nature Communications
    Volume: 10, P: 1-7