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Showing 1–4 of 4 results
Advanced filters: Author: Liangshu Zhong Clear advanced filters

  • Lower olefins are hydrocarbons that are widely used in the chemical industry, and can be generated from syngas by the ‘Fischer–Tropsch to olefins’ process; here, a new catalyst is described that can generate lower olefins from syngas with high selectivity, with little formation of undesirable methane.

    • Liangshu Zhong
    • Fei Yu
    • Hui Wang
    Research
    Nature
    Volume: 538, P: 84-87

  • It is still a great challenge to synthesize value-added products with two or more carbons directly from CO2. Now, a bifunctional catalyst composed of reducible metal oxides (In2O3) and zeolites (HZSM-5) is prepared and yields high selectivity to gasoline-range hydrocarbons (78.6%) with a high octane number directly from CO2 hydrogenation.

    • Peng Gao
    • Shenggang Li
    • Yuhan Sun
    Research
    Nature Chemistry
    Volume: 9, P: 1019-1024

  • Zhong et al report sodium-promoted metallic Ru nanoparticles for the direct production of olefins from syngas with ultrahigh carbon efficiency where the total selectivity of undesired CH4 and CO2 is suppressed to only 5% for over 500 hours on stream.

    • Hailing Yu
    • Caiqi Wang
    • Liangshu Zhong
    ResearchOpen Access
    Nature Communications
    Volume: 13, P: 1-10

  • Understanding the structures of interfacial active sites is crucial in heterogeneous catalysis. Here the authors demonstrate that a ZrO2-Ru interface site significantly enhances reactivity in the Fischer-Tropsch to olefins process by altering the H-assisted CO dissociation route due to the presence of hydroxy species associated with Zr-OH*.

    • Hailing Yu
    • Caiqi Wang
    • Liangshu Zhong
    ResearchOpen Access
    Nature Communications
    Volume: 15, P: 1-11