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Showing 1–5 of 5 results
Advanced filters: Author: Matthew Jouny Clear advanced filters

  • The electroreduction of CO2-derived CO is a promising technology for the sustainable production of value-added chemicals. Now, it is shown how C–N bonds can be formed electrochemically through CO electroreduction on a Cu surface in the presence of amines. The formation of acetamides is observed through nucleophilic addition to a ketene intermediate.

    • Matthew Jouny
    • Jing-Jing Lv
    • Feng Jiao
    Research
    Nature Chemistry
    Volume: 11, P: 846-851

  • The low solubility of CO in aqueous electrolytes limits the implementation of CO electrolysers, since low current densities are typically achieved despite the fact that they deliver rather high Faradaic efficiencies to multi-carbon products. Now, Jiao and co-workers report a CO flow electrolyser with a well-controlled electrode–electrolyte interface that can achieve multi-carbon Faradaic efficiencies of 91% with a partial current density of 630 mA cm–2.

    • Matthew Jouny
    • Wesley Luc
    • Feng Jiao
    Research
    Nature Catalysis
    Volume: 1, P: 748-755

  • Upgrading CO to high-value multicarbon products is a promising avenue for fuel and chemical feedstock production. Here triangular Cu nanosheets that selectively expose the (111) surface exhibit a high acetate partial current density (131 mA cm–2) and Faradaic efficiency (48%) in CO electroreduction.

    • Wesley Luc
    • Xianbiao Fu
    • Yijin Kang
    Research
    Nature Catalysis
    Volume: 2, P: 423-430

  • Carbon monoxide can be electrochemically transformed to multi-carbon products selectively at high rates, raising the prospect of a two-step pathway to transform CO2 into value-added chemical products. This Perspective highlights recent progress complemented by a techno-economic analysis of the two-step conversion process and cradle-to-gate lifecycle assessment.

    • Matthew Jouny
    • Gregory S. Hutchings
    • Feng Jiao
    Reviews
    Nature Catalysis
    Volume: 2, P: 1062-1070