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Ultrafast transition from coherent to incoherent polariton nonlinearities in a hybrid 1L-WS₂/plasmon structure

Strongly enhanced optical nonlinearities and an ultrafast transition from coherent to incoherent polariton excitations are demonstrated by coupling an atomically thin WS₂ layer to a plasmonic nanostructure using ultrafast multidimensional spectroscopy.

Daniel Timmer
Moritz Gittinger
Christoph Lienau
ResearchOpen Access21 Jan 2026
Nature Nanotechnology

P: 1-7
Plasmon mediated coherent population oscillations in molecular aggregates

The authors uncover a coherent, long-range transport of excitons in organic semiconductors that are strongly coupled to spatially structured plasmon fields by tracing ultrafast Rabi oscillations using two-dimensional electronic spectroscopy.

Daniel Timmer
Moritz Gittinger
Christoph Lienau
ResearchOpen Access05 Dec 2023
Nature Communications

Volume: 14, P: 1-10

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Ultrafast transition from coherent to incoherent polariton nonlinearities in a hybrid 1L-WS2/plasmon structure

Plasmon mediated coherent population oscillations in molecular aggregates

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Ultrafast transition from coherent to incoherent polariton nonlinearities in a hybrid 1L-WS₂/plasmon structure