Pump-probe spectroscopy is routinely used to interrogate ultrafast valence electronic and vibrational dynamics in complex systems. Here, the authors extend this technique to the X-ray regime using a sequence of femtosecond X-ray pulses to understand core-valence interactions in a solvated molecular complex.
- Robert B. Weakly
- Chelsea E. Liekhus-Schmaltz
- Munira Khalil
