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Showing 1–3 of 3 results
Advanced filters: Author: Vickery L. Arcus Clear advanced filters

  • Soil microbial respiration responses to warming have important implications for biogeochemical feedbacks. Here, using data from temperature gradients, the authors show that the rate of thermal adaptation of soil microbial respiration is lower than the rate of warming despite large community changes.

    • Charlotte J. Alster
    • Allycia van de Laar
    • Louis A. Schipper
    ResearchOpen Access
    Nature Communications
    Volume: 14, P: 1-12

  • Computationally designed enzymes can be substantially improved by directed evolution. Now, it has been shown that evolution can introduce a dynamic network that selectively tightens the transition-state ensemble, giving rise to a negative activation heat capacity. Targeting such transition state conformational dynamics may expedite de novo enzyme creation.

    • H. Adrian Bunzel
    • J. L. Ross Anderson
    • Adrian J. Mulholland
    Research
    Nature Chemistry
    Volume: 13, P: 1017-1022

  • Heat capacity changes affect the temperature dependence of enzyme catalysis, with implications for thermoadaptation, however their physical basis is unknown. Here the authors show that heat capacity changes are calculable by simulation, revealing distinct dynamical contributions from regions remote from the active site.

    • Marc W. van der Kamp
    • Erica J. Prentice
    • Vickery L. Arcus
    ResearchOpen Access
    Nature Communications
    Volume: 9, P: 1-7