Abstract
In the era of digital information, realizing efficient and durable data storage solutions is paramount. Innovations in storage capacity, data throughput, device lifespan and energy consumption are pressing necessities for the continuous progression of practical digital data storage technologies. Here we present a diamond storage medium that exploits fluorescent vacancy centres as robust storage units and provides a high storage density of 14.8 Tbit cm−3, a short write time of 200 fs and an estimated ultralong maintenance-free lifespan on the scale of millions of years. High-speed readout through plane and volume imaging is demonstrated with a high fidelity exceeding 99%, showing that the approach addresses the practical demands of digital data storage and provides a promising solution for future storage requirements.
This is a preview of subscription content, access via your institution
Access options
Access Nature and 54 other Nature Portfolio journals
Get Nature+, our best-value online-access subscription
$32.99 / 30 days
cancel any time
Subscribe to this journal
Receive 12 print issues and online access
$259.00 per year
only $21.58 per issue
Buy this article
- Purchase on SpringerLink
- Instant access to full article PDF
Prices may be subject to local taxes which are calculated during checkout




Similar content being viewed by others
Data availability
The data used to produce the plots within this paper are available via figshare at https://doi.org/10.6084/m9.figshare.26322568 (ref. 59).
Code availability
The necessary code used to produce the plots within this paper are available via figshare at https://doi.org/10.6084/m9.figshare.26322568 (ref. 59).
References
Irie, M., Fukaminato, T., Sasaki, T., Tamai, N. & Kawai, T. A digital fluorescent molecular photoswitch. Nature 420, 759–760 (2002).
Zijlstra, P., Chon, J. W. M. & Gu, M. Five-dimensional optical recording mediated by surface plasmons in gold nanorods. Nature 459, 410–413 (2009).
Grotjohann, T. et al. Diffraction-unlimited all-optical imaging and writing with a photochromic GFP. Nature 478, 204–208 (2011).
Goldman, N. et al. Towards practical, high-capacity, low-maintenance information storage in synthesized DNA. Nature 494, 77–80 (2013).
Lambert, C.-H. et al. All-optical control of ferromagnetic thin films and nanostructures. Science 345, 1337–1340 (2014).
Shipman, S. L., Nivala, J., Macklis, J. D. & Church, G. M. CRISPR–Cas encoding of a digital movie into the genomes of a population of living bacteria. Nature 547, 345–349 (2017).
Sun, K. et al. Three-dimensional direct lithography of stable perovskite nanocrystals in glass. Science 375, 307–310 (2022).
Xiong, B. et al. Breaking the limitation of polarization multiplexing in optical metasurfaces with engineered noise. Science 379, 294–299 (2023).
Gu, M., Li, X. & Cao, Y. Optical storage arrays: a perspective for future big data storage. Light Sci. Appl. 3, e117 (2014).
Gu, M., Zhang, Q. & Lamon, S. Nanomaterials for optical data storage. Nat. Rev. Mater. 1, 16070 (2016).
Zhang, J., Gecevičius, M., Beresna, M. & Kazansky, P. G. Seemingly unlimited lifetime data storage in nanostructured glass. Phys. Rev. Lett. 112, 033901 (2014).
Zhang, Q., Xia, Z., Cheng, Y.-B. & Gu, M. High-capacity optical long data memory based on enhanced Young’s modulus in nanoplasmonic hybrid glass composites. Nat. Commun. 9, 1183 (2018).
Gao, L., Zhang, Q., Evans, R. A. & Gu, M. 4D ultra-high-density long data storage supported by a solid-state optically active polymeric material with high thermal stability. Adv. Opt. Mater. 9, 2100487 (2021).
Lei, Y. et al. High speed ultrafast laser anisotropic nanostructuring by energy deposition control via near-field enhancement. Optica 8, 1365–1371 (2021).
Wang, H. et al. 100-layer error-free 5D optical data storage by ultrafast laser nanostructuring in glass. Laser Photon. Rev. 16, 2100563 (2022).
Wang, Z. et al. 3D imprinting of voxel-level structural colors in lithium niobate crystal. Adv. Mater. 35, 2303256 (2023).
Li, X., Zhang, Q., Chen, X. & Gu, M. Giant refractive-index modulation by two-photon reduction of fluorescent graphene oxides for multimode optical recording. Sci. Rep. 3, 2819 (2013).
Dai, Q. et al. Encoding random hot spots of a volume gold nanorod assembly for ultralow energy memory. Adv. Mater. 29, 1701918 (2017).
Lei, Y. et al. Efficient ultrafast laser writing with elliptical polarization. Light Sci. Appl. 12, 74 (2023).
Li, X., Cao, Y., Tian, N., Fu, L. & Gu, M. Multifocal optical nanoscopy for big data recording at 30 TB capacity and gigabits/second data rate. Optica 2, 567–570 (2015).
Lee, W. et al. A rewritable optical storage medium of silk proteins using near-field nano-optics. Nat. Nanotechnol. 15, 941–947 (2020).
Yuan, X. et al. Ultra-high capacity for three-dimensional optical data storage inside transparent fluorescent tape. Opt. Lett. 45, 1535–1538 (2020).
Lamon, S., Wu, Y., Zhang, Q., Liu, X. & Gu, M. Nanoscale optical writing through upconversion resonance energy transfer. Sci. Adv. 7, eabe2209 (2021).
Han, F. et al. Three-dimensional nanofabrication via ultrafast laser patterning and kinetically regulated material assembly. Science 378, 1325–1331 (2022).
Zhao, M. et al. A 3D nanoscale optical disk memory with petabit capacity. Nature 626, 772–778 (2024).
Sarid, D. & Schechtman, B. H. A roadmap for optical data storage applications. Opt. Photon. News 18, 32–37 (2007).
Zhang, C. et al. Luminescence modulation of ordered upconversion nanopatterns by a photochromic diarylethene: rewritable optical storage with nondestructive readout. Adv. Mater. 22, 633–637 (2010).
Dhomkar, S., Henshaw, J., Jayakumar, H. & Meriles, C. A. Long-term data storage in diamond. Sci. Adv. 2, e1600911 (2016).
Aslam, N., Waldherr, G., Neumann, P., Jelezko, F. & Wrachtrup, J. Photo-induced ionization dynamics of the nitrogen vacancy defect in diamond investigated by single-shot charge state detection. New J. Phys. 15, 013064 (2013).
Wolfowicz, G. et al. Optical charge state control of spin defects in 4H-SiC. Nat. Commun. 8, 1876 (2017).
Lozovoi, A. et al. Optical activation and detection of charge transport between individual colour centres in diamond. Nat. Electron. 4, 717–724 (2021).
Loubser, J. H. N. & Wyk, J. A. V. Electron spin resonance in the study of diamond. Rep. Prog. Phys. 41, 1201–1248 (1978).
Walker, J. Optical absorption and luminescence in diamond. Rep. Prog. Phys. 42, 1605–1659 (1979).
Eaton-Magaña, S., Breeding, C. M. & Bassoo, R. Low-temperature annealing and kinetics of radiation stains in natural diamond. Diam. Relat. Mater. 132, 109649 (2023).
Subedi, S., Fedorov, V., Mirov, S. & Markham, M. Spectroscopy of GR1 centers in synthetic diamonds. Opt. Mater. Express 11, 757 (2021).
Eaton, S. M. et al. Heat accumulation effects in femtosecond laser-written waveguides with variable repetition rate. Opt. Express 13, 4708–4716 (2005).
Lin, Z. & Hong, M. Femtosecond laser precision engineering: from micron, submicron, to nanoscale. Ultrafast Sci. 2021, 9783514 (2021).
Mauclair, C., Mermillod-Blondin, A., Huot, N., Audouard, E. & Stoian, R. Ultrafast laser writing of homogeneous longitudinal waveguides in glasses using dynamic wavefront correction. Opt. Express 16, 5481–5492 (2008).
Jesacher, A., Marshall, G. D., Wilson, T. & Booth, M. J. Adaptive optics for direct laser writing with plasma emission aberration sensing. Opt. Express 18, 656–661 (2010).
Simmonds, R. D., Salter, P. S., Jesacher, A. & Booth, M. J. Three dimensional laser microfabrication in diamond using a dual adaptive optics system. Opt. Express 19, 24122–24128 (2011).
Hering, J., Waller, E. H. & Freymann, G. V. Automated aberration correction of arbitrary laser modes in high numerical aperture systems. Opt. Express 24, 28500–28508 (2016).
Wiecha, P. R., Lecestre, A., Mallet, N. & Larrieu, G. Pushing the limits of optical information storage using deep learning. Nat. Nanotechnol. 14, 237–244 (2019).
Li, X., Lan, T.-H., Tien, C.-H. & Gu, M. Three-dimensional orientation-unlimited polarization encryption by a single optically configured vectorial beam. Nat. Commun. 3, 998 (2012).
Lu, Y. et al. Tunable lifetime multiplexing using luminescent nanocrystals. Nat. Photon. 8, 32–36 (2014).
Laube, C. et al. Fluorescence lifetime control of nitrogen vacancy centers in nanodiamonds for long-term information storage. ACS Nano 17, 15401–15410 (2023).
Lagomarsino, S. et al. Photoionization of monocrystalline CVD diamond irradiated with ultrashort intense laser pulse. Phys. Rev. B 93, 085128 (2016).
Griffiths, B. et al. Microscopic processes during ultra-fast laser generation of Frenkel defects in diamond. Phys. Rev. B 104, 174303 (2021).
Gray, F. Pulse code communication. US patent 2632058 (1953).
Sakakura, M., Lei, Y., Wang, L., Yu, Y.-H. & Kazansky, P. G. Ultralow-loss geometric phase and polarization shaping by ultrafast laser writing in silica glass. Light Sci. Appl. 9, 15 (2020).
Khaw, I. et al. Flat-field illumination for quantitative fluorescence imaging. Opt. Express 26, 15276–15288 (2018).
Zhao, Z., Xin, B., Li, L. & Huang, Z.-L. High-power homogeneous illumination for super-resolution localization microscopy with large field-of-view. Opt. Express 25, 13382–13395 (2017).
Mau, A., Friedl, K., Leterrier, C., Bourg, N. & Lévêque-Fort, S. Fast widefield scan provides tunable and uniform illumination optimizing super-resolution microscopy on large fields. Nat. Commun. 12, 3077 (2021).
Descloux, A. et al. Combined multi-plane phase retrieval and super-resolution optical fluctuation imaging for 4D cell microscopy. Nat. Photon. 12, 165–172 (2018).
Scherrer, J. R., Lynch, G. F., Zhang, J. J. & Fee, M. S. An optical design enabling lightweight and large field-of-view head-mounted microscopes. Nat. Methods 20, 546–549 (2023).
Hasegawa, S., Ito, H., Toyoda, H. & Hayasaki, Y. Massively parallel femtosecond laser processing. Opt. Express 24, 18513–18524 (2016).
Chen, Y.-C. et al. Laser writing of individual nitrogen-vacancy defects in diamond with near-unity yield. Optica 6, 662–667 (2019).
Kim, S.-W., Takaya, R., Hirano, S. & Kasu, M. Two-inch high-quality (001) diamond heteroepitaxial growth on sapphire (1120) misoriented substrate by step-flow mode. Appl. Phys. Express 14, 115501 (2021).
Rittweger, E., Wildanger, D. & Hell, S. W. Far-field fluorescence nanoscopy of diamond color centers by ground state depletion. Europhys. Lett. 86, 14001 (2009).
Zhou, J.-Y. et al. Open data for “Terabit-scale high-fidelity diamond data storage”. figshare https://doi.org/10.6084/m9.figshare.26322568 (2024).
Acknowledgements
We thank Q. Chen for technical support in the femtosecond direct writing system; D. Liu for help in image denoising; and G. Muratori for granting us permission to use his painting. This work is supported by the National Natural Science Foundation of China (grant numbers T2325023, 92265204, T2125011, 12104446, 12104447, 12274400 and 123B1019), the CAS (GJJSTD20200001), the Innovation Program for Quantum Science and Technology (grant number 2021ZD0302200), the Anhui Initiative in Quantum Information Technologies (grant number AHY050000), and the Fundamental Research Funds for the Central Universities (grant number WK3540000010).
Author information
Authors and Affiliations
Contributions
J.D., Y.W. and K.X. supervised the project. Y.W. and K.X. conceived the idea. Y.W., K.X. and J.Z. designed the experiment. J.Z. performed the data-writing experiments. J.Z., J.S., J.G., Y.Y. and K.X. performed the data-reading experiments. J.Z. and W.J. analysed the data. M.W. prepared the sample. Y.W., K.X., J.Z., W.J., J.S., F.S. and J.D. wrote the paper. All authors discussed the results and commented on the paper.
Corresponding authors
Ethics declarations
Competing interests
The authors declare no competing interests.
Peer review
Peer review information
Nature Photonics thanks Carlos A. Rios Ocampo, Ye Zhou and the other, anonymous, reviewer(s) for their contribution to the peer review of this work.
Additional information
Publisher’s note Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.
Supplementary information
Supplementary Information
Supplementary Figs. 1–12 and Table 1.
Supplementary Video 1
Data restored from a diamond storage medium of The Horse in Motion (the first film in the world; Eadweard Muybridge, 1887).
Rights and permissions
Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.
About this article
Cite this article
Zhou, J., Su, J., Guan, J. et al. Terabit-scale high-fidelity diamond data storage. Nat. Photon. 18, 1327–1334 (2024). https://doi.org/10.1038/s41566-024-01573-1
Received:
Accepted:
Published:
Issue date:
DOI: https://doi.org/10.1038/s41566-024-01573-1