Introduction

The spatiotemporal variation of stable water isotope ratios in modern precipitation (δ18Op) shows clear patterns that strongly correlate with several environmental variables1,2. Dansgaard1 was the first to analyze δ18Op data comprehensively, identifying empirical relationships between δ18Op variations with several environmental factors across space, notably surface temperature and precipitation amount. Two well-known effects were observed: the “temperature effect”, where δ18Op becomes more enriched with higher temperatures, and the “amount effect”, where δ18Op is depleted with increased precipitation1,2,3. Both effects are thought to be influenced by the Rayleigh distillation. These effects have also been used to infer climatic changes over various timescales, from seasonal to orbital cycles4,5,6,7. However, climatic interpretations of δ18Op across different timescales are often studied separately without a unified framework, leaving it a great challenge to connect long-term climate changes from paleoclimate records with present short-term observations, especially in the East Asian Monsoon (EAM) region.

Present observations reveal contrasting seasonal δ18Op patterns in northern and southern China. In northern China, the “temperature effect” dominates, while in southern China, the “amount effect” is more prominent4,8,9,10. However, these seasonal relationships are insufficient to explain longer-term climate changes. In proxy records and climate model simulations, δ18Op shows variability from interannual to millennial and orbital timescales, which can sometimes decouple from local temperature in northern China11,12 or local precipitation amount in southern China9,13,14. Furthermore, δ18Op exhibits coherent changes across the entire EAM region on interannual15,16,17, millennial18,19,20, and orbital timescales21,22,23, despite the differing seasonal cycles between southern and northern China (Fig. 1a, b).

Fig. 1: EOF analysis of the seasonal cycle of δ18Op over the EAM region and its surroundings.
figure 1

a The leading EOF mode (EOF1) of observed δ18Op. b The EOF1 of modeled δ18Op. c The leading principal components (PC1) of observed δ18Op. d The PC1 of modeled δ18Op. e Seasonal cycle of observed (red) and simulated (blue) δ18Op in northern China (N. China). f Seasonal cycle of observed (red) and simulated (blue) δ18Op in southern China (S. China). The percentage values in the top right of (a, b) represent the variance explained by EOF1. In (a, b), the upper and bottom black boxes mark the regions of N. China (37°N to 43°N, 108°E to 120°E) and S. China (22°N to 35°N, 108°E to 120°E), respectively. The dark gray lines outline the part of the Tibetan Plateau boundary. Detailed information regarding the observed δ18Op is provided in Supplementary Table 1. The modeled δ18Op is derived from the final 20 years of a 40-year PI water tagging experiment.

The complexity of interpreting δ18Op across different timescales is partly due to the influence of remote moisture sources and transport patterns, which can exert a much greater influence on δ18Op than local temperature or precipitation alone24. In the EAM region, the seasonal variation in moisture sources and the meridional shift of moisture transport patterns, both driven by the monsoon system, significantly complicate the climatic interpretation of δ18Op. As a result, several other factors, such as changes in precipitation and moisture sources4,15,25,26,27,28,29,30,31, enroute depletion and upstream rainout/convection12,13,17,32,33,34,35,36,37,38,39,40,41,42,43, monsoon intensity44,45, and precipitation seasonality23,35,46,47,48,49,50, have been proposed to explain δ18Op variations. However, these factors are often interrelated, making it challenging to isolate them. For example, changes in summer monsoon moisture sources are often coincide with enhanced upstream convection. Despite the EAM’s influence on both northern and southern China, it remains unclear how these monsoon-related factors contribute to the contrasting seasonal δ18Op cycles in the two regions while also explaining the coherent δ18Op changes on longer timescales.

To address these issues, we quantitatively analyze δ18Op variations in northern and southern China across seasonal, millennial, and orbital timescales using a unified framework in a state-of-the-art isotope-enabled earth system model. This unified framework reveals that the main distinction between the δ18Op variations in seasonal and longer timescale lies in the additional impact of precipitation seasonality in the latter. Otherwise, both are controlled by the same processes in the water cycle, including changes in moisture sources and a series of source-to-enroute-to-condensation processes. Our results show that change in moisture sources and upstream enroute depletion are the two primary factors controlling δ18Op variability in the EAM region, with their importance varying across different timescales. Change in moisture source dominate δ18Op variability on seasonal and orbital timescales, while meltwater-induced enroute depletion is the main driver on millennial timescales. The contrasting seasonal cycles of the δ18Op between northern and southern China are mainly due to seasonal changes in moisture source from remote regions, where the contributed δ18Op values are very depleted, with minimal contribution from local change of temperature or precipitation amount.

Results and discussion

Model-data comparison

Our pre-industrial (PI) simulation in iCAM5.3 reproduces the major feature of the observed seasonal δ18Op cycle in the EAM region. It shows a clear contrast between the “temperature effect” in northern China and the “amount effect” in southern China, as shown by the leading EOFs (Fig. 1; Supplementary Fig. 1; see Methods, Part 1). Additionally, our model accurately reproduces the spatial pattern of seasonal δ18Op variations in the EAM region. Specifically, both the observation and simulation show that the δ18Op enrichment in summer gradually become more pronounced with latitude in the northern part of the EAM region, while δ18Op depletion in summer is most pronounced in southwestern China (Fig. 1a, b). The direct model-data comparison shows good agreement between the simulated and observed δ18Op in North China (r = 0.77, p < 0.01) and South China (r = 0.90, p < 0.01) (Fig. 1e, f).

Moisture source (\({{\mathbf{\Delta }}}_{{{\bf{dP}}}_{{\bf{ori}}}}\)) dominants the seasonal δ18Op anomaly over the EAM region

The seasonal variation of δ18Op (anomaly from the annual mean) is influenced by moisture from different source regions (see Methods, Part 2). In northern China, although most precipitation comes from local East Asia continent (EAS) throughout the year (Supplementary Fig. 2a, e), this has little impact on the seasonal cycle of δ18Op (Fig. 2a). In contrast, the remote North Atlantic Ocean (AO), with much more depleted δ18Op (Supplementary Fig. 2c), plays a crucial role in producing the apparent “temperature effect” in northern China (Fig. 2a). To understand how each source region contributes to the seasonal cycle of δ18Op, we decompose the δ18Op anomaly into two components: \({\Delta {{\updelta }}}^{18}{{\rm{O}}}_{{\rm{p}}}={\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}+{\Delta }_{{\rm{d}}{{\updelta }}}\), where \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\) represents the precipitation weight change from the source region and Δ represents the isotope change from the source region (see Methods, Part 3). This decomposition illustrates that the AO determines the seasonal δ18Op anomalies in northern China through the \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\) component (Fig. 2b, c). This is because, in comparison with local EAS enriched δ18Op, the AO’s contribution to EAM δ18Op is severely depleted (~ −5‰ vs −30‰, Supplementary Fig. 2c), as moisture travels long distances across the Eurasian Continent, undergoing upstream rainout. In winter, the AO is a major oceanic moisture source for northern China, accounting for over 20% of precipitation (Supplementary Fig. 2a), leading to δ18Op depletion. In summer, as the AO’s contribution diminishes (Supplementary Fig. 2a) due to the northward migration of the westerly jet and the increased source from the nearby EAS (where the δ18Op is enriched ~ −6‰, Supplementary Fig. 2c), the δ18Op anomaly returns to positive. This seasonal change in the AO moisture contribution causes δ18Op to be negative in winter and positive in summer (Fig. 2a, b). It should be noted that the Δ component from the Pacific Ocean (PO) contributes to the “temperature effect” in northern China (Fig. 2a, c). However, the offsetting effects of the Δ and \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\) from the PO result in a negligible seasonal variation in δ18Op change induced by the PO (Fig. 2a–c). Consequently, the seasonal δ18Op anomaly in northern China is primarily driven by the \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\) component from the AO (Fig. 2a–c). We emphasize the significant role of the AO in winter precipitation in northern China, which has not been widely recognized in previous studies using other approaches like the Lagrangian method51,52. The Lagrangian method infers moisture sources based on the evaporation-precipitation difference assumptions51,52, whereas our water tagging method can directly trace moisture sources where evaporation occurs and unaffected by precipitation events18,53. Additionally, the Lagrangian method is restricted by several other assumptions and limitations, notably the exclusion of important processes like convection, turbulence, and numerical diffusion52. In essence, for Lagrangian methods to be reliable, they require high-frequency observational data and an integration period longer than 10 days for the calculations54. In contrast, the water-tagging approach accounts for complex feedbacks (e.g., cloud microphysics) and offers a comprehensive view of moisture contributions and isotopic evolution under varying climate conditions15,18. We assert that the water tagging method implemented in the iCAM5.3 model is reliable, as it accurately reproduces the seasonal cycle of δ18Op in North China (Fig. 1f).

Fig. 2: Seasonal δ18Op variations and its decomposition in N. China and S. China.
figure 2

a Seasonal δ18Op anomaly (bold black line) and its source decomposition (non-black lines) in N. China. b Contribution of moisture source change to the δ18Op anomaly (\({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\), bold black line) and the source decomposition of \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\) (non-black lines) in N. China. c Contribution of isotope change from source regions to the δ18Op anomaly (Δ, bold black line) and the source decomposition of Δ (non-black lines) in N. China. d Same as (a) but for S. China. e Same as (b) but for S. China. f Same as c but for S. China. In each region, \({{\rm{\delta }}}^{18}{{\rm{O}}}_{{\rm{p}}}={\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}+{\Delta }_{\text{d}{\rm{\delta }}}\). PO the Pacific Ocean, IO the Indian Ocean, AO the Atlantic Ocean, EAS East Asia Continent, EC the Eurasian Continent, Other, the remaining other tagging regions. The bold black line in each panel represents the total δ18Op anomaly, \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\), or Δ for each study regions.

In contrast, the \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\) from the remote Indian Ocean (IO) is the major factor driving the apparent “amount effect” in southern China (Fig. 2d–f). Southern China is influenced by two major moisture sources, the IO and PO (Supplementary Fig. 2b). The IO has more depleted δ18Op (~ −15‰ annually) due to its longer distance to reach southern China (Supplementary Fig. 2d). In winter, the IO’s contribution is small, and the δ18Op in southern China is dominated by the relatively enriched PO contribution (~ −8‰ annually). However, in summer, the IO’s contribution increases significantly and becomes comparable to that of the PO (Supplementary Fig. 2b). As a result, in southern China, there is a negative δ18Op anomaly in summer and a positive anomaly in winter (Fig. 2d). The importance of the IO for southern China aligns with previous study that has investigated δ18Op variations between summer and winter seasons15. Overall, the Δ component does not influence the seasonal δ18Op anomaly in southern China (Fig. 2d, f).

Our analysis reveals a consistent mechanism behind the contrasting seasonal δ18Op variations in northern China and southern China. These variations are primarily dictated by changes from the remote moisture sources of the AO and IO (\({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\), Fig. 2b, e), rather than by local temperature and precipitation amount. Additionally, \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\) consistently serves as the main factor driving the seasonal variations of δ18Op in the EAM region under climate conditions that differ significantly from the PI climate (Supplementary Fig. 3; Supplementary Fig. 4). However, the differences in the seasonal amplitude of δ18Op across climate conditions are not necessarily driven by \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\). For example, in northern China, the increase in the seasonal amplitude of δ18Op during periods of enhanced summer insolation (Pmin) is primarily due to \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Enroute}}}}\) rather than \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\) (Supplementary Fig. 3a, e).

Enroute depletion \(({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Enroute}}}})\) dominants the seasonal change of isotope value Δ

Although the isotope value change Δ is not the dominant factor in the seasonal cycle of δ18Op, we briefly discuss it here for comparison with δ18Op variability on longer timescales later. We decompose the seasonal Δ change into three sub-processes associated with the changes over the source region, the enroute process, and the condensation over the sink region: \({\Delta }_{{\rm{d}}{{\updelta }}}={{\Delta }_{{\rm{d}}{{\updelta }}}}_{{\rm{Source}}}+{\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Enroute}}}}+{\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Condensation}}}}\) (see Methods, Part 3). Our decomposition analysis reveals that the seasonal Δ in both northern China and southern China is mainly driven by changes in the enroute depletion process \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Enroute}}}}\). For northern China, the seasonal anomaly of Δ is contributed mainly by the enroute process, especially from the PO (Fig. 2c; Supplementary Fig. 5a–c). A further analysis shows this enroute contribution from the PO is dominated by that from the subtropical North Pacific (SNP) (Supplementary Fig. 6). The seasonal changes in SNP \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Enroute}}}}\) are influenced by the north-south movement of the low-latitude circulation. From winter to summer, the North Pacific Subtropical High migrates northward, and the southern branch of its anticyclonic circulation transports moisture from the SNP to northern China via a shorter path in summer than winter (Supplementary Fig. 7). As a result, the values of water vapor (δ18Ov) arriving in North China are enriched in summer than winter (~ −20‰ \({\rm{vs}}\) −60‰, Supplementary Fig. 8a). This causes the enrichment in summer and depletion in winter of the PO \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Enroute}}}}\) (Supplementary Fig. 5b). Relatively, the seasonal changes in δ18Ov arriving in southern China from SNP are less pronounced (Supplementary Fig. 8b). The longer summer moisture transport path from the IO may explain why SNP δ18Ov peaks in spring rather than summer in southern China (−15‰ vs −16.6‰, Supplementary Fig. 7a, b; Supplementary Fig. 8b).

Competition between moisture source \(({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}})\) and enroute depletion \(({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Enroute}}}})\) determining δ18Op on longer timescales

We now further examine the mechanisms underlying δ18Op variations in northern and southern China on longer timescales, comparing them with the seasonal cycle. Analogous to the seasonal cycle study, δ18Op changes can be better understood as the difference between two time periods using a decomposition. This study advances previous work by developing a refined decomposition method that separates the precipitation seasonality component from the moisture source component (see Methods, Part 4). This approach is particularly valuable, as previous studies have highlighted the potential influence of precipitation seasonality on δ18Op in East Asia23,35,46,47,48,49,50. In our method, the change of δ18Op can be decomposed into three components: the change of precipitation seasonality \({\Delta }_{{{\rm{dP}}}_{{\rm{sea}}}}\), the change of moisture source \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\), and the change of isotope values Δ. The Δ can be further decomposed into three processes: the source change \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Source}}}}\), enroute change \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Enroute}}}}\), and condensation change \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Condensation}}}}\) (see Methods, Part 4). The decomposition analysis shows that the precipitation seasonality \({\Delta }_{{{\rm{dP}}}_{{\rm{Sea}}}}\) is not important for δ18Op changes in the EAM region on millennial and orbital timescales, unlike high-latitude regions such as Greenland55,56. Instead, δ18Op changes are primarily determined by the competition between the changes of moisture source\(\,{\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\) and the changes in isotope values via the enroute process \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Enroute}}}}\) (Fig. 3).

Fig. 3: δ18Op variations and its decomposition on millennial and orbital timescales in N. China and S. China.
figure 3

a The δ18Op difference between HS1 and LGM across the pan-Asian monsoon region. b The δ18Op difference between HS1 and LGM and its decomposition in N. China. c The δ18Op difference between HS1 and LGM and its decomposition in S. China. d The δ18Op difference between Pmin and Pmax across the pan-Asian monsoon region. e The δ18Op difference between Pmin and Pmax and its decomposition in N. China. f The δ18Op difference between Pmin and Pmax and its decomposition in S. China. In this figure, δ18Op represents the precipitation-weighted annual δ18Op. In (a, d), solid circles represent observed cave speleothem δ18O records (Supplementary Table 2). Note that our study focuses on the western part of S. China (22°N to 35°N, 108°E to 114°E) on millennial and orbital timescales, where model results are consistent with observations on orbital timescales. The dark gray lines outline the Tibetan Plateau boundary. In (b, c, e, f), \({\Delta }_{{{\rm{\delta }}}^{18}{{\rm{O}}}_{{\rm{p}}}}={\Delta }_{{{\rm{dP}}}_{{\rm{Sea}}}}+{\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}+{\Delta }_{{\rm{d}}{\rm{\delta }}}\), and \({\Delta }_{{\rm{d}}{\rm{\delta }}}={\Delta }_{{{\rm{d}}{\rm{\delta }}}_{{\rm{Source}}}}+{\Delta }_{{{\rm{d}}{\rm{\delta }}}_{{\rm{Enroute}}}}+{\Delta }_{{{\rm{d}}{\rm{\delta }}}_{{\rm{Condensation}}}}\). PO the Pacific Ocean, IO the Indian Ocean, AO the Atlantic Ocean, EAS East Asia Continent, EC the Eurasian Continent, Other, the remaining other tagging regions. The Sum in each panel represents the total \({\Delta }_{{{\rm{\delta }}}^{18}{{\rm{O}}}_{{\rm{p}}}}\), \({\Delta }_{{{\rm{dP}}}_{{\rm{Sea}}}}\), \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\), \({\Delta }_{{{\rm{d}}{\rm{\delta }}}_{{\rm{Source}}}}\), \({\Delta }_{{{\rm{d}}{\rm{\delta }}}_{{\rm{Enroute}}}}\), or \({\Delta }_{{{\rm{d}}{\rm{\delta }}}_{{\rm{Condensation}}}}\) of six tagging domains.

On millennial timescales, we examine the δ18Op change from the Last Glacial Maximum (LGM) to Heinrich Stadial 1 (HS1). Both observational and model data show a spatially coherent positive δ18Op change across the pan Asian monsoon region in the HS1–LGM difference (Fig. 3a), aligning with previous studies18,53. In contrast, the annual precipitation anomaly exhibits a heterogenous response: significant increase in southern China and a decrease across the Indian monsoon region (Supplementary Fig. 9a). Therefore, δ18Op and rainfall anomalies are both positive in southern China, which does not align with the classical “amount effect”. Our decomposition analysis shows that positive δ18Op variations in both northern and southern China are primarily result from the enroute process \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Enroute}}}}\), which alters the isotope values in Δ (Fig. 3b, c). There is minimal contribution from \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\) or \({\Delta }_{{{\rm{dP}}}_{{\rm{sea}}}}\) (Fig. 3b,c). The dominant process is the \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Enroute}}}}\) change associated with the IO, rather than the PO, which dominates the \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Enroute}}}}\) changes on seasonal timescales (Supplementary Fig. 5b, e). Mechanistically, during HS1, the weakening of the Indian summer monsoon shortens the moisture transport distance from the Indian Ocean to EAM region (Supplementary Fig. 10a, b; Supplementary Fig. 11). This shortened distance results in a positive δ18Op variation across the EAM region due to reduced enroute isotopic depletion18,53. This mechanism differs significantly from the seasonal cycle, which is dominated by seasonal change of moisture source\({\,\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\) in the EAM region, as discussed earlier (Fig. 2b, e). Additionally, the \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Source}}}}\) and \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Condensation}}}}\) also contribute to the positive δ18Op variations, especially in northern China, due to reduced upstream rainout (Supplementary Fig. 9a) and enhanced local EAS contribution (Fig. 3b, c, refs. 18,53).

On orbital timescales, we investigate the δ18Op responses to two different precessional forcing: one with minimum precession (Pmin) and the other with maximum precession (Pmax). Our model simulations, along with previous observations, reveal a spatially coherent negative δ18Op variation across the Indian monsoon region to northern China during the transition from reduced (Pmax) to intensified (Pmin) summer insolation (Fig. 3d). This finding is consistent with results from previous modeling studies15,57,58. In contrast, the precipitation amount response to orbital forcing shows a north-south dipole pattern, with increasing precipitation in northern China and decreasing precipitation in southern China (Supplementary Fig. 9b). Therefore, the δ18Op anomaly in northern China aligns with the “amount effect”, but this is not the case in southern China, consistent with previous work12. The negative δ18Op response is primarily caused by the changes of moisture source \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\) in both northern and southern China (Fig. 3e, f). Mechanistically, intensified summer insolation during Pmin increases the transport of moisture from the remote PO and IO (Supplementary Fig. 10c), both of which contribute highly depleted isotope values to northern China (Fig. 3e, f). This lead to significant δ18Op depletion, as indicated by the negative \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\) (Fig. 3e, f). In southern China, the increased moisture from the remote PO is partially offset by the reduced moisture from the IO, resulting in less significant δ18Op depletion in \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\) (Fig. 3f; Supplementary Fig. 10d). Although the enroute process \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Enroute}}}}\) contributes the most to depletion in southern China, this contribution is largely offset by the condensation process \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Condensation}}}}\), leading to a negligible total contribution from the isotope value response Δ. Therefore, the dominant impact comes from the \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\) (Fig. 3f). Previous studies have suggested that the orbital-scale δ18Op variation in southern China is primarily influenced by the IO, based on seasonal timescales findings15. However, our study reveals the PO’s primary influence on East Asian δ18Op on orbital timescales, contrasting with the seasonal and millennial scales, which are dominated by the IO. This suggest that a simplistic comparison between seasonal and precessional timescales warrants additional scrutiny and discussion. Previous studies have shown that orbital-scale δ18Op variations in the Indian monsoon region are also linked to changes in moisture source \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\) 57. This implies a consistent mechanism for δ18Op variation across the Asian monsoon region on orbital timescales: intensified summer insolation strengthens the monsoon, driving more remote moisture to the region and resulting in a uniform δ18Op depletion across the entire Asian monsoon region. This consistent mechanism is further supported by a recent model study across the Asian monsoon region58.

Our decomposition analysis reveals that the δ18Op variations across the EAM region are primarily driven by enroute depletion \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Enroute}}}}\) on millennial timescales, while changes in moisture source \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\) on orbital timescales. Unlike the season cycle, the AO plays a negligible role in influencing the δ18Op variations in northern China on millennial and orbital timescales. This difference arises because annual δ18Op in northern China is dominated by the δ18Op change during summer monsoon season (Supplementary Fig. 1e), while the AO plays a stronger role only in winter (Supplementary Fig. 1a). Instead, in summer, both northern and southern China experience significant precipitation from moisture sources in the IO and PO (Supplementary Fig. 1e, f). As a result, their annual δ18Op exhibit synchronous responses to the influences of the IO or PO influences on millennial and orbital timescales, mediated by enroute depletion \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Enroute}}}}\) and moisture source \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\) (Fig. 3b, c, e, f). This explains why consistent δ18Op variations are observed on millennial and orbital timescales in the EAM region, but are absent on the seasonal timescales.

The framework we developed emphasizes the distinction in δ18Op variations across seasonal and longer timescales, highlighting that longer timescales are additionally influenced by precipitation seasonality. When precipitation seasonality is not significant for a specific region, the δ18Op variations on different timescales in this region can be explained through our framework, which isolates and quantifies the relative contributions of different water cycle processes. This refined δ18Op decomposition method in our study can be generalized to other monsoon systems, such as the South Asian57 and African monsoons59, as well as to various paleoclimate archives, including ice cores56, tree rings, and lake sediments. The broad application of this method will greatly enhance our understanding of the climatic significance of δ18Op at different timescales across different regions.

Conclusions

The contrasting δ18Op response across the EAM region on seasonal timescales and the coherent δ18Op response on millennial and orbital timescales can be understood through a unified framework as caused by different mechanisms, notably the competition between the change of moisture sources and the enroute depletion. The seasonal contrast in δ18Op between northern and southern China is primarily caused by the shifts in moisture sources: the very depleted δ18Op from the remote AO in winter for northern China and from the remote IO in summer for southern China (Fig. 4a). On millennial timescales, the coherent δ18Op response across the entire EAM region results from similar isotope enrichment from the major moisture source of the IO, via the enroute process, along with reduced upstream precipitation linked to a weakening summer monsoon in response to meltwater forcing (Fig. 4b). On orbital timescales, the coherent δ18Op response is mainly caused by a stronger summer monsoon, which transports more depleted moisture from the PO or IO moisture to the EAM region (Fig. 4c). In none of the cases, the change of δ18Op is directly related to the change of local temperature and precipitation amount. Our study highlights that the correlation between δ18Op and local meteorological factors on a seasonal scale should not be directly applied to interpret longer-term isotopic variability in paleoclimate proxies, even qualitatively. Instead, long-term δ18Op variations in East Asia are primarily influenced by changes in moisture source and enroute processes, two key components of the summer monsoon system associated with seasonal precipitation reversals and meridional shifts in low-latitude circulation, respectively60.

Fig. 4: Schematic diagrams illustrating δ18Op variations across timescales in the EAM region.
figure 4

a Seasonal timescale. In summer, the monsoon carries remote IO moisture to S. China, depleting δ18Op in this region. In winter, westerly winds bring remote AO moisture to N. China, depleting δ18Op here. b Millennial timescales. During HS1, a weakened Indian summer monsoon increases transport of nearby IO moisture (e.g., the Bay of Bengal) to the EAM region. Reduced enroute depletion enriches δ18Op across the EAM region. c Orbital timescales. During Pmin, intensified insolation enhances remote PO moisture transport to the EAM region, depleting δ18Op across the EAM region. Notably, the remote IO also contributes to the depleted δ18Op in N. China but not in S. China due to reduced IO contribution there. Blue shading in each panel represents δ18Op depletion while red shading represents δ18Op enrichment. PO the Pacific Ocean, IO the Indian Ocean, AO the Atlantic Ocean. HS1 the Heinrich Stadial 1 (15.5 ka BP). LGM the Last Glacial Maximum (20 ka BP). Pmin Precessional minimum (127 ka BP). Pmax Precessional maximum (116 ka BP).

Observational records suggest that δ18Op variations in the EAM region on decadal- to centennial-scale do not exhibit a robust coherent or north-south dipole patterns15,61,62,63,64,65. This inconsistency may indicate the important influence of local factors, independent of the monsoon system, on δ18O variations on these timescales. Such local factors fall outside the scope of this study, which focuses on the monsoon-related mechanisms driving δ18Op variability across the EAM region. Additionally, a systematic, multi-model investigation into the effects of moisture source and enroute depletion on δ18Op variations across different timescales in the EAM region would provide a more comprehensive and robust understanding of how summer monsoon evolution is reflected in oxygen isotope records.

Methods

Part 1: Precipitation stable isotope data

We used observational monthly δ18Op data from 24 stations located in the East Asian monsoon (EAM) region and its surrounding areas, sourced from the Global Network of Isotopes in Precipitation (GNIP). The stations were selected based on the availability of complete monthly data after multiyear averaging (Supplementary Table 1).

Part 2: Water tagging experiments

Recently, researchers have utilized water tagging methods in numerical models to examine changes in δ18Op in the EAM region15,18,31. The tagging experiment is designed to trace the life cycle of water isotopes. H216O or H218O is traced from the tagging region once it evaporates from the surface (source region) and follows the hydrological cycle in the model to the region where it rains out (sink region). We performed five snapshot water tagging experiments during the pre-industrial (PI), Heinrich Stadial 1 (HS1, 15.5 ka BP), Last Glacial Maximum (LGM, 20 ka BP), precessional minimum (Pmin, 127 ka BP), and precessional maximum (Pmax, 116 ka BP) periods using the isotope-enabled Community Atmosphere Model (iCAM5.3), the atmospheric model in iCESM1.3. We use the “FV2” version of the iCESM1.3, which employs a finite-volume dynamical core at a nominal resolution of 2°66. The iCAM5.3 has a horizontal resolution of 1.9° in latitude and 2.5° in longitude, and a vertical resolution of 30 levels. The isotopic ratios, related fluxes, and isotope fractionation are simulated across all components of the hydrological cycle. The tagging experiments for the PI, HS1, and LGM periods were driven by sea ice distribution, sea surface temperature, and sea surface δ18O data from the iCESM1.3 experiment, which is an isotope-enabled full forcing transient climate experiment including icesheet, orbital, greenhouse gas, and meltwater forcing. Detailed experiment setup descriptions can be obtained from refs. 18,56. The forcing for the two water tagging experiments, named Pmin and Pmax, are directly derived from a 100-fold accelerated single-orbit forced transient simulation of the past 300 ka58. In this transient experiment, all boundary conditions are kept fixed in the PI period, with only changes made to the Earth’s orbital parameters. The direct model-data comparison demonstrates that the model can effectively simulate the δ18Op variations in the East Asian monsoon (EAM) region during the last deglaciation, including the LGM and HS1 periods18. Furthermore, the model also accurately captures the δ18Op variations in the EAM region over the past 300,000 years, particularly during the precession cycle58.

Of the five water tagging experiments, the PI experiment is utilized to analyze the seasonal δ18Op variations in the EAM region. Millennial-scale abrupt climate changes, characterized by rapid transitions between cold stadial and warm interstadial states, are most prevalent during glacial periods67,68. HS events, driven by extreme ice-rafting, represent the coldest of these stadials53 and are recorded in speleothem δ18O records in the EAM regions69. In this study, the modeled millennial-scale δ18Op changes are primarily attributed to meltwater forcing18. Therefore, we focused on the HS1-LGM period of the last deglaciation to analyze millennial-scale δ18Op variations, as this interval was characterized by relatively small changes in ice sheets, greenhouse gases, and orbital parameters, allowing us to better isolate the impact of meltwater forcing. The pervasive millennial-scale abrupt climate changes during glacial-interglacial cycles70 are often linked to changes in the Atlantic Meridional Overturning Circulation (AMOC) induced by meltwater forcing71,72. Therefore, while the HS1-LGM transition provides a valuable case study of deglacial millennial-scale climate change, it also offers insights into the mechanisms driving similar δ18Op variations during other abrupt climate events, including warm interglacial periods. While obliquity-induced changes in insolation are considered to impact East Asian seasonality and monsoons at orbital scales73, the monsoon’s response to obliquity forcing is weaker than its response to precession forcing74. For δ18O variations in this study, observations show that the most prominent cycle in speleothem δ18O records in the EAM region is the ~20,000-year precession cycle69. Our simulations also reveal a clear precession cycle in δ18Op for both South and North China, with no indication of a ~ 40,000-year obliquity cycle (Supplementary Fig. 12). A previous study demonstrated that even after removing the precessional component, the variance within the precessional band in the detrended (suborbital) speleothem δ18O signal still exceeds that within the obliquity band, indicating a minor role for obliquity69. Therefore, the Pmin and Pmax experiments are used for analyzing variations on orbital timescales. The simulation result shows a subtle increase in δ18Op values in southeastern China during Pmin when insolation intensifies (Fig. 3d). This result contradicts the speleothem δ18O records reported in previous studies conducted at Hulu Cave (32.50°N, 119.17°E)75,76. To address this discrepancy, we conducted a decomposition analysis specifically targeting the millennial and orbital variations in δ18Op in southwestern China (22°N to 35°N, 108°E to 114°E), where simulation results align with observations (Fig. 3d). In addition, the Pmin and Pmax experiments exclude changes in ice sheets, greenhouse gases, meltwater forcing, and seawater isotopes, which may explain why the simulated δ18Op amplitudes are smaller than the observed variations (Fig. 3d). However, they effectively capture the general δ18Op changes across the southwestern China and northern China driven by precession-cycle insolation (Fig. 3d). This makes these experiments well-suited for investigating the mechanisms driving δ18Op changes in the EAM region on precession timescale, which is the primary focus of this study. This study does not analyze time scales ranging from a decade to a century, based on two main considerations. First, on these time scales, the δ18O records in the EAM region do not show consistent spatial patterns. Specifically, the δ18O variations in southern and northern China differ significantly19; even within southern China, there are large differences in δ18O records between different sites77. This makes it difficult to extract a clear regional δ18O periodic signal on these time scales, and it becomes even harder to analyze its underlying mechanisms. On the other hand, the model’s ability to simulate these time scales requires further verification. Previous results indicate that the iCESM model can simulate large-scale drought conditions from the Medieval Climate Anomaly (MCA) to the Little Ice Age (LIA), but it fails to capture the temporal evolution of the climate recorded in proxy over the Common Era78. A recent model-data comparisons over the past millennium using multiple isotope-enabled climate models underscore the difficulty of reliably validating model simulations on decadal to centennial scales using speleothem isotope records due to the lower temporal resolution of speleothem records, karst mixing effects, and uncertainties in volcanic forcing reconstructions79. Thus, applying decomposition approach to investigate the δ18Op variability across these timescales remains a task for future research.

We employ 25 tags globally and each tag utilizes either oceanic evaporation or land evapotranspiration (Supplementary Fig. 13). This tagging methods are different from previous modern studies that mainly focus on the effects of several main moisture source on δ18Op variations in the EAM region15,31. In our work, the total monthly precipitation amount (Pm) and precipitation water isotope ratio (δ18Op, m) for a specific region can be calculated using the following equations:

$${{\rm{P}}}_{{\rm{m}}}=\mathop{\sum }\limits_{{\rm{i}}=1}^{25}{{\rm{P}}}_{{\rm{i}},{\rm{m}}},\,{\rm{m}}=1,\,2,\,3,...,\,12$$
(1a)
$${{{{\updelta }}}^{18}{\rm{O}}}_{{\rm{p}},{\rm{m}}}=\mathop{\sum }\limits_{{\rm{i}}=1}^{25}{{{{\updelta }}}^{18}{\rm{O}}}_{{\rm{pi}},{\rm{m}}}\left(\frac{{{\rm{P}}}_{{\rm{i}},{\rm{m}}}}{{{\rm{P}}}_{{\rm{m}}}}\right),\,{\rm{m}}=1,\,2,\,3,...,\,12$$
(1b)

where Pi, m (or δ18Opi, m) refers to the precipitation amount (or δ18O) contribution of tagging region i in a given month m.

Part 3: Decomposing seasonal δ18Op variations

The seasonal \({{{\updelta }}}^{18}{{\rm{O}}}_{\text{p},\text{m}}\) anomaly \((\Delta {{{\updelta }}}^{18}{{\rm{O}}}_{\text{p},\text{m}})\) is its difference from the annual mean δ18Op

$${{{{\updelta }}}^{18}{\rm{O}}}_{{\rm{p}},{\rm{a}}}=\frac{\mathop{\sum }\nolimits_{{\rm{j}}=1}^{12}\mathop{\sum }\nolimits_{{\rm{i}}=1}^{25}{{{{\updelta }}}^{18}{\rm{O}}}_{{\rm{pi}},{\rm{j}}}\left(\frac{{{\rm{P}}}_{{\rm{i}},{\rm{j}}}}{{{\rm{P}}}_{{\rm{j}}}}\right)}{12},$$
(2)

as

$$\Delta {{{\updelta }}}^{18}{{\rm{O}}}_{\text{p},\text{m}}={{{\updelta }}}^{18}{{\rm{O}}}_{\text{p},\text{m}}-{{{\updelta }}}^{18}{{\rm{O}}}_{\text{p},\text{a}},\, {\rm{m}}=1,\,2,\,3,...,\,12$$
(3a)

This seasonal change \(\Delta {{{\updelta }}}^{18}{{\rm{O}}}_{\text{p},\text{m}}\) in the sink region reflects the contributions from all source regions. Using Eqs. (1b) and (2), this seasonal \(\Delta {{{\updelta }}}^{18}{{\rm{O}}}_{\text{p},\text{m}}\) can be decomposed into two parts. The first part is the contribution to the precipitation weight change from different source regions, or simply moisture source change \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\), and the second part associated with the change of the δ18Op value from different source regions, or simply isotope change Δ (Supplementary Fig. 14a).

$$\Delta {{{\updelta }}}^{18}{{\rm{O}}}_{\text{p},\text{m}}={\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}+{\Delta }_{\text{d}{{\updelta }}},\ {\rm{m}}=1,\,2,\,3,...,\,12$$
(3b)

with each part contributed by that from all source regions as

$${\Delta }_{{\rm{dP}}_{\rm{Ori}}}={\sum }_{{\rm{i}}=1}^{25}{\Delta }_{{\rm{dP}}_{\rm{Ori}},{\rm{i}}}, \ {\Delta }_{{\rm{dP}}_{\rm{Ori}},{\rm{i}}}=\frac{{\sum }_{{\rm{j}}=1}^{12}{\frac{1}{2}}\left({{\updelta }}^{18}{{\rm{O}}_{\rm{p}}}_{{\text{i}},{\text{j}}}+{{\updelta }}^{18}{{\rm{O}}_{\rm{p}}}_{{\text{i}},{\text{m}}}\right){\left(\frac{{\rm{P}}_{{\text{i}},{\text{m}}}}{{\rm{P}}_{\text{m}}}-\frac{{\rm{P}}_{{\text{i}},{\text{j}}}}{{\rm{P}}_{\text{j}}}\right)}}{12}$$
(3c)
$${\Delta }_{\text{d}{{\updelta }}}={\sum }_{{\rm{i}}=1}^{25}{\Delta }_{{\rm{d}}{{\updelta }},{\rm{i}}}, \ {\Delta }_{{\rm{d}}{{\updelta }},{\rm{i}}}=\frac{{\sum }_{{\rm{j}}=1}^{12}\frac{1}{2}(\frac{{{\rm{P}}}_{\text{i},\text{j}}}{{{\rm{P}}}_{\text{j}}}+\frac{{{\rm{P}}}_{\text{i},\text{m}}}{{{\rm{P}}}_{\text{m}}})({{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{p}}}}_{\text{i},\text{m}}-{{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{p}}}}_{\text{i},\text{j}})}{12}$$
(3d)

The isotope change, from say, region i, Δ(dδ,i) can be further decomposed along its trajectory to three processes: source process \({\Delta }_{{{\rm{d}}{{\updelta }},{\rm{i}}}_{{\rm{Source}}}}\), enroute process \({\Delta }_{{{\rm{d}}{{\updelta }},{\rm{i}}}_{{\rm{Enroute}}}}\), and condensation process \({\Delta }_{{{\rm{d}}{{\updelta }},{\rm{i}}}_{{\rm{Condensation}}}}\)57. Hence, the Δ(dδ,i) term in equation (3 d) can be further decomposed using vapor water isotope \({{{\updelta }}}^{18}{{\rm{O}}}_{{\rm{v}}}\) into three components (Supplementary Fig. 14a):

$${\Delta }_{\text{d}{{\updelta }},\text{i}}={\Delta }_{{{\rm{d}}{{\updelta }},{\rm{i}}}_{{\rm{Source}}}}+{\Delta }_{{{\rm{d}}{{\updelta }},{\rm{i}}}_{{\rm{Enroute}}}}+{\Delta }_{{{\rm{d}}{{\updelta }},{\rm{i}}}_{{\rm{Condensation}}}},$$
(4a)

where

$${\Delta }_{{{\rm{d}}{{\updelta }},{\rm{i}}}_{{\rm{Source}}}}=\mathop{\sum}\limits_{{\rm{j}}=1}^{12}\frac{1}{2}\left(\frac{{{\rm{P}}}_{\text{i},\text{j}}}{{{\rm{P}}}_{\text{j}}}+\frac{{{\rm{P}}}_{\text{i},\text{m}}}{{{\rm{P}}}_{\text{m}}}\right)\Delta \left({{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{vi}}}}_{{\rm{Source}}}\right),$$
(4b)
$$\Delta \left({{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{vi}}}}_{{\rm{Source}}}\right)={{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{vi}},{\rm{m}}}}_{{\rm{Source}}}-{{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{vi}},{\rm{j}}}}_{{\rm{Source}}},$$
(4c)
$${\Delta }_{{{\rm{d}}{{\updelta }},{\rm{i}}}_{{\rm{Enroute}}}}=\mathop{\sum}\limits_{{\rm{j}}=1}^{12}\frac{1}{2}\left(\frac{{{\rm{P}}}_{\text{i},\text{j}}}{{{\rm{P}}}_{\text{j}}}+\frac{{{\rm{P}}}_{\text{i},\text{m}}}{{{\rm{P}}}_{\text{m}}}\right)\Delta \left({{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{vi}}}}_{{\rm{Sink}}}-{{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{vi}}}}_{{\rm{Source}}}\right),$$
(4d)
$$\Delta \left({{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{vi}}}}_{{\rm{Sink}}}-{{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{vi}}}}_{{\rm{Source}}}\right) = \left({{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{vi}},{\rm{m}}}}_{{\rm{Sink}}}-{{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{vi}},{\rm{j}}}}_{{\rm{Sink}}}\right)\\ -\left({{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{vi}},{\rm{m}}}}_{{\rm{Source}}}-{{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{vi}},{\rm{j}}}}_{{\rm{Source}}}\right),$$
(4e)
$$\,{\Delta }_{{{\rm{d}}{{\updelta }},{\rm{i}}}_{{\rm{Condensation}}}}=\mathop{\sum}\limits_{{\rm{j}}=1}^{12}\frac{1}{2}(\frac{{{\rm{P}}}_{\text{i},\text{j}}}{{{\rm{P}}}_{\text{j}}}+\frac{{{\rm{P}}}_{\text{i},\text{m}}}{{{\rm{P}}}_{\text{m}}})\Delta \left({{{\updelta }}}^{18}{{\rm{O}}}_{{\rm{pi}}}-{{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{vi}}}}_{{\rm{Sink}}}\right),$$
(4f)
$$\Delta \left({{{\updelta }}}^{18}{{\rm{O}}}_{{\rm{pi}}}-{{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{vi}}}}_{{\rm{Sink}}}\right)= \left({{{\updelta }}}^{18}{{\rm{O}}}_{{\rm{pi}},{\rm{m}}}-{{{\updelta }}}^{18}{{\rm{O}}}_{{\rm{pi}},{\rm{j}}}\right)\\ -\left({{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{vi}},{\rm{m}}}}_{{\rm{Sink}}}-{{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{vi}},{\rm{j}}}}_{{\rm{Sink}}}\right),$$
(4g)

In Eqs. (4b)–(4g), m represents a specific month of interest, whereas j is a monthly index that iterates from 1 to 12, used to derive the annual average of δ18Op. Finally, the seasonal δ18Op anomalies (\(\Delta {{{\updelta }}}^{18}{{\rm{O}}}_{\text{p},\text{m}}\)) are ultimately decomposed into four components: \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\), \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Source}}}}\), \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Enroute}}}}\), and \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Condensation}}}}\) (Supplementary Fig. 14a).

Part 4: Decomposing δ18Op difference between two periods

We present a refined decomposition method for investigating δ18Op variations on longer timescales. This method decomposes annual δ18Op variations caused by precipitation weight change (ΔdP) into two distinct components: (1) δ18Op variations driven by changes in precipitation seasonality (\({\Delta }_{{{\rm{dP}}}_{{\rm{Sea}}}}\)), and (2) δ18Op variations reflecting changes in moisture source (\({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\)). This approach is different from previous studies that combined these two components into a single moisture source component15,18,57. Previous studies have suggested a potential influence of precipitation seasonality on δ18Op in this region23,35,46,47,48,49,50. By isolating these components, our improved methodology offers a clearer picture of the mechanisms influencing δ18Op variations in East Asia. Specifically, the annual δ18Op difference (\(\Delta {{{\updelta }}}^{18}{{\rm{O}}}_{\text{p},\text{a}}\)) between two periods “1” and “2” can be decomposed into the changes of precipitation seasonality (\({\Delta }_{{{\rm{dP}}}_{{\rm{S}}{\rm{ea}}}}\)) and δ18Op seasonality (\({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Sea}}}}\)) (Supplementary Fig. 14b).

$$\Delta {{{\updelta }}}^{18}{{\rm{O}}}_{\rm{p},\rm{a}}= {{{\updelta }}}^{18}{{\rm{O}}}_{\rm{p}1,\rm{a}}-{{{\updelta }}}^{18}{{\rm{O}}}_{\rm{p}2,\rm{a}}=\mathop{\sum}\limits_{{\rm{m}}=1}^{12}\left({{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{p}}1}}_{\rm{m}}\frac{{{\rm{P}}1}_{\rm{m}}}{{{\rm{P}}1}_{{\rm{a}}}}\right)\\ -\mathop{\sum}\limits_{{\rm{m}}=1}^{12}\left({{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{p}}2}}_{\rm{m}}\frac{{{\rm{P}}2}_{\rm{m}}}{{{\rm{P}}2}_{{\rm{a}}}}\right)={\underbrace{\mathop{\sum }\limits_{{\rm{m}}=1}^{12}\left(\left(\frac{{{\rm{P}}1}_{\rm{m}}}{{{\rm{P}}1}_{{\rm{a}}}}-\frac{{{\rm{P}}2}_{\rm{m}}}{{{\rm{P}}2}_{{\rm{a}}}}\right)\left(\frac{{{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{p}}1}}_{\rm{m}}+{{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{p}}2}}_{\rm{m}}}{2}\right)\right)}_{{{{\updelta }}}_{{{\rm{dP}}}_{{\rm{Sea}}}}\,}}\\ +{\underbrace{\mathop{\sum}\limits_{{\rm{m}}=1}^{12}\left(\left({{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{p}}1}}_{\rm{m}}-{{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{p}}2}}_{\rm{m}}\right)\left(\frac{\frac{{{\rm{P}}1}_{\rm{m}}}{{{\rm{P}}1}_{{\rm{a}}}}+\frac{{{\rm{P}}2}_{\rm{m}}}{{{\rm{P}}2}_{{\rm{a}}}}}{2}\right)\right)}_{{\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Sea}}}}\,}}$$
(5a)

where

$$\frac{{{\rm{P}}1}_{\rm{m}}}{{{\rm{P}}1}_{{\rm{a}}}}=\mathop{\sum }\limits_{{\rm{i}}=1}^{25}\frac{{{\rm{P}}1}_{\rm{m},\rm{i}}}{{{\rm{P}}1}_{{\rm{a}}}},$$
(5b)
$$\frac{{{\rm{P}}2}_{\rm{m}}}{{{\rm{P}}2}_{{\rm{a}}}}=\mathop{\sum }\limits_{{\rm{i}}=1}^{25}\frac{{{\rm{P}}2}_{\rm{m},\rm{i}}}{{{\rm{P}}2}_{{\rm{a}}}},$$
(5c)
$${\delta }^{18}{{{\rm{O}}}_{{\rm{p}}1}}_{\rm{m}}=\mathop{\sum }\limits_{{\rm{i}}=1}^{25}{\delta }^{18}{{{\rm{O}}}_{{\rm{p}}1}}_{\rm{m},\rm{i}}\frac{{{\rm{P}}1}_{\rm{m},\rm{i}}}{{{\rm{P}}1}_{{\rm{m}}}},$$
(5d)
$${\delta }^{18}{{{\rm{O}}}_{{\rm{p}}2}}_{\rm{m}}=\mathop{\sum }\limits_{{\rm{i}}=1}^{25}{\delta }^{18}{{{\rm{O}}}_{{\rm{p}}2}}_{\rm{m},\rm{i}}\frac{{{\rm{P}}2}_{\rm{m},\rm{i}}}{{{\rm{P}}2}_{{\rm{m}}}},$$
(5e)

Following the decomposition of seasonal δ18Op variations in eqs. (3a–d), water isotope seasonality change \({\Delta }_{{{\rm{d}}\delta }_{{\rm{Sea}}}}\) can be further decomposed into \({\Delta }_{{{\rm{d}}\delta }_{{\rm{Sea}}\_{\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}}}\) and \({\Delta }_{{{\rm{d}}\delta }_{{\rm{Sea}}{{\_}}{\Delta }_{{\rm{d}}\delta }}}\) (Supplementary Fig. 14b):

$${\Delta }_{{{\rm{d}}\delta }_{{\rm{Sea}}}}= \mathop{\sum}\limits_{{\rm{m}}=1}^{12}\left(\left({\delta }^{18}{{{\rm{O}}}_{{\rm{p}}1}}_{\rm{m}}-{\delta }^{18}{{{\rm{O}}}_{{\rm{p}}2}}_{\rm{m}}\right)\left(\frac{\frac{{{\rm{P}}1}_{\rm{m}}}{{{\rm{P}}1}_{{\rm{a}}}}+\frac{{{\rm{P}}2}_{\rm{m}}}{{{\rm{P}}2}_{{\rm{a}}}}}{2}\right)\right),\\ = \mathop{\sum}\limits_{{\rm{m}}=1}^{12}\left(\left(\mathop{\sum }\limits_{{\rm{i}}=1}^{25}{\delta }^{18}{{{\rm{O}}}_{{\rm{p}}1}}_{\rm{m},\rm{i}}\frac{{{\rm{P}}1}_{\rm{m},\rm{i}}}{{{\rm{P}}1}_{{\rm{m}}}}-\mathop{\sum }\limits_{{\rm{i}}=1}^{25}{\delta }^{18}{{{\rm{O}}}_{{\rm{p}}2}}_{\rm{m},\rm{i}}\frac{{{\rm{P}}2}_{\rm{m},\rm{i}}}{{{\rm{P}}2}_{{\rm{m}}}}\right)\left(\frac{\frac{{{\rm{P}}1}_{\rm{m}}}{{{\rm{P}}1}_{{\rm{a}}}}+\frac{{{\rm{P}}2}_{\rm{m}}}{{{\rm{P}}2}_{{\rm{a}}}}}{2}\right)\right),\\ = {\underbrace{\sum _{{\rm{m}}=1}^{12}\left(\mathop{\sum }\limits_{{\rm{i}}=1}^{25}\left(\left(\frac{{{\rm{P}}1}_{\rm{m},\rm{i}}}{{{\rm{P}}1}_{{\rm{m}}}}-\frac{{{\rm{P}}2}_{\rm{m},\rm{i}}}{{{\rm{P}}2}_{{\rm{m}}}}\right)\left(\frac{{\delta }^{18}{{{\rm{O}}}_{{\rm{p}}1}}_{\rm{m},\rm{i}}+{\delta }^{18}{{{\rm{O}}}_{{\rm{p}}2}}_{\rm{m},\rm{i}}}{2}\right)\right)\frac{(\frac{{{\rm{P}}1}_{\rm{m}}}{{{\rm{P}}1}_{{\rm{a}}}}+\frac{{{\rm{P}}2}_{\rm{m}}}{{{\rm{P}}2}_{{\rm{a}}}})}{2}\right)}_{{\Delta }_{{{\rm{d}}\delta }_{{\rm{Sea}}\_{\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}}}\,}}\\ + {\underbrace{\sum _{{\rm{m}}=1}^{12}\left(\mathop{\sum }\limits_{{\rm{i}}=1}^{25}\left(\left({\delta }^{18}{{{\rm{O}}}_{{\rm{p}}1}}_{\rm{m},\rm{i}}-{\delta }^{18}{{{\rm{O}}}_{{\rm{p}}2}}_{\rm{m},\rm{i}}\right)\left(\frac{\frac{{{\rm{P}}1}_{\rm{m},\rm{i}}}{{{\rm{P}}1}_{{\rm{m}}}}+\frac{{{\rm{P}}2}_{\rm{m},\rm{i}}}{{{\rm{P}}2}_{{\rm{m}}}}}{2}\right)\right)\frac{(\frac{{{\rm{P}}1}_{\rm{m}}}{{{\rm{P}}1}_{{\rm{a}}}}+\frac{{{\rm{P}}2}_{\rm{m}}}{{{\rm{P}}2}_{{\rm{a}}}})}{2}\right)}_{{\Delta }_{{{\rm{d}}\delta }_{{\rm{Sea}}\_{\Delta }_{{\rm{d}}\delta }}}\,}},$$
(6)

Following the seasonal decomposition in Eq. (4a–g), \({\Delta }_{{{\rm{d}}\delta }_{{\rm{Sea}}{{\_}}{\Delta }_{{\rm{d}}{{\updelta }}}}}\) can be further decomposed into the processes associated with the source \({\Delta }_{{{\rm{d}}\delta }_{{{\rm{Sea}}}_{-}{\Delta }_{{{\rm{d}}\delta }_{{\rm{Source}}}}}}\), enroute \({\Delta }_{{{\rm{d}}\delta }_{{{\rm{Sea}}}_{-}{\Delta }_{{{\rm{d}}\delta }_{{\rm{Enroute}}}}}}\) and condensation \({\Delta }_{{{\rm{d}}\delta }_{{{\rm{Sea}}}_{-}{\Delta }_{{{\rm{d}}\delta }_{{\rm{Condensation}}}}}}\) as (Supplementary Fig. 14b)

$${\Delta }_{{{\rm{d}}\delta }_{{{\rm{Sea}}}_{-}{\Delta }_{{\rm{d}}\delta }}}= {\underbrace{\mathop{\sum }\limits_{{\rm{m}}=1}^{12}\left(\mathop{\sum }\limits_{{\rm{n}}=1}^{25}\left(\widetilde{\Delta }\left({\delta }^{18}{{{\rm{O}}}_{{\rm{v}}}}_{{\rm{source}}}\right)\left(\frac{\frac{{{\rm{P}}1}_{\rm{m},\rm{j}}}{{{\rm{P}}1}_{{\rm{m}}}}+\frac{{{\rm{P}}2}_{\rm{m},\rm{j}}}{{{\rm{P}}2}_{{\rm{m}}}}}{2}\right)\right)\frac{(\frac{{{\rm{P}}1}_{\rm{m}}}{{{\rm{P}}1}_{{\rm{a}}}}+\frac{{{\rm{P}}2}_{\rm{m}}}{{{\rm{P}}2}_{{\rm{a}}}})}{2}\right)}_{{\Delta }_{{{\rm{d}}\delta }_{{{\rm{Sea}}}_{-}{\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Source}}}}}}\,}}\\ +{\underbrace{\mathop{\sum }\limits_{{\rm{m}}=1}^{12}\left(\mathop{\sum }\limits_{{\rm{n}}=1}^{25}\left(\widetilde{\Delta }\left({{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{v}}}}_{{\rm{sink}}}-{{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{v}}}}_{{\rm{source}}}\right)\left(\frac{\frac{{{\rm{P}}1}_{\rm{m},\rm{j}}}{{{\rm{P}}1}_{{\rm{m}}}}+\frac{{{\rm{P}}2}_{\rm{m},\rm{j}}}{{{\rm{P}}2}_{{\rm{m}}}}}{2}\right)\right)\frac{\left(\frac{{{\rm{P}}1}_{\rm{m}}}{{{\rm{P}}1}_{{\rm{a}}}}+\frac{{{\rm{P}}2}_{\rm{m}}}{{{\rm{P}}2}_{{\rm{a}}}}\right)}{2}\right)}_{{\Delta }_{{{\rm{d}}{{\updelta }}}_{{{\rm{Sea}}}_{-}{\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Enroute}}}}}}\,}}\\ +{\underbrace{\mathop{\sum }\limits_{{\rm{m}}=1}^{12}\left(\mathop{\sum }\limits_{{\rm{n}}=1}^{25}\left(\,\widetilde{\Delta }\left({{{\updelta }}}^{18}{{\rm{O}}}_{{\rm{p}}}-{{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{v}}}}_{{\rm{sink}}}\right)\left(\frac{\frac{{{\rm{P}}1}_{\rm{m},\rm{j}}}{{{\rm{P}}1}_{{\rm{m}}}}+\frac{{{\rm{P}}2}_{\rm{m},\rm{j}}}{{{\rm{P}}2}_{{\rm{m}}}}}{2}\right)\right)\frac{\left(\frac{{{\rm{P}}1}_{\rm{m}}}{{{\rm{P}}1}_{{\rm{a}}}}+\frac{{{\rm{P}}2}_{\rm{m}}}{{{\rm{P}}2}_{{\rm{a}}}}\right)}{2}\right)}_{{\Delta }_{{{\rm{d}}{{\updelta }}}_{{{\rm{Sea}}}_{-}{\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Condensation}}}}}}}}$$
(7a)

where

$$\widetilde{\Delta }\left({{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{v}}}}_{{\rm{source}}}\right)={{{\updelta }}}^{18}{{{\rm{O}}}_{{{\rm{v}}1}_{{\rm{m}},{\rm{j}}}}}_{{\rm{source}}}-{{{\updelta }}}^{18}{{{\rm{O}}}_{{{\rm{v}}2}_{{\rm{m}},{\rm{j}}}}}_{{\rm{source}}}$$
(7b)
$$\widetilde{\Delta }\left({{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{v}}}}_{{\rm{sink}}}-{{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{v}}}}_{{\rm{source}}}\right) = \left({{{\updelta }}}^{18}{{{\rm{O}}}_{{{\rm{v}}1}_{{\rm{m}},{\rm{j}}}}}_{{\rm{sink}}}-{{{\updelta }}}^{18}{{{\rm{O}}}_{{{\rm{v}}2}_{{\rm{m}},{\rm{j}}}}}_{{\rm{sink}}}\right)\\ -\left({{{\updelta }}}^{18}{{{\rm{O}}}_{{{\rm{v}}1}_{{\rm{m}},{\rm{j}}}}}_{{\rm{source}}}-{{{\updelta }}}^{18}{{{\rm{O}}}_{{{\rm{v}}2}_{{\rm{m}},{\rm{j}}}}}_{{\rm{source}}}\right)$$
(7c)
$$\widetilde{\Delta }\left({{{\updelta }}}^{18}{{\rm{O}}}_{{\rm{p}}}-{{{\updelta }}}^{18}{{{\rm{O}}}_{{\rm{v}}}}_{{\rm{sink}}}\right) = \left({{{\updelta }}}^{18}{{\rm{O}}}_{{{\rm{p}}1}_{{\rm{m}},{\rm{j}}}}-{{{\updelta }}}^{18}{{\rm{O}}}_{{{\rm{p}}2}_{{\rm{m}},{\rm{j}}}}\right)\\ -\left({{{\updelta }}}^{18}{{{\rm{O}}}_{{{\rm{v}}1}_{{\rm{m}},{\rm{j}}}}}_{{\rm{sink}}}-{{{\updelta }}}^{18}{{{\rm{O}}}_{{{\rm{v}}2}_{{\rm{m}},{\rm{j}}}}}_{{\rm{sink}}}\right)$$
(7d)

Therefore, the \(\Delta {{{\updelta }}}^{18}{{\rm{O}}}_{\rm{p},\rm{a}}\) is decomposed into five components as follows: \({\Delta }_{{{\rm{dP}}}_{{\rm{Sea}}}}\), \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{{\rm{Sea}}}_{-}{\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}}}\), \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{{\rm{Sea}}}_{-}{\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Source}}}}}}\), \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{{\rm{Sea}}}_{-}{\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Enroute}}}}}}\), and \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{{\rm{Sea}}}_{-}{\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Condensation}}}}}}\). To simplify subscript labels, we use the same names for the last four components as the decomposition names of seasonal δ18Op variations, i.e., \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\), \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Source}}}}\), \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Enroute}}}}\), and \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Condensation}}}}\). The interpretation of the anomaly is the difference between two time periods, similar to the case of seasonal cycle where the anomaly is the difference between two months. Finally, the annual δ18Op anomalies (\(\Delta {{{\updelta }}}^{18}{{\rm{O}}}_{\rm{p},\rm{a}}\)) are ultimately decomposed into five components: \({\Delta }_{{{\rm{dP}}}_{{\rm{Sea}}}}\), \({\Delta }_{{{\rm{dP}}}_{{\rm{Ori}}}}\), \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Source}}}}\), \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Enroute}}}}\), and \({\Delta }_{{{\rm{d}}{{\updelta }}}_{{\rm{Condensation}}}}\) (Supplementary Fig. 14b).

For our purpose of analysis of EAM region here, we group the 25 source regions into six domains, the Pacific Ocean (PO), the Indian Ocean (IO), the Atlantic Ocean (AO), the local East Asia continent (EAS), the non-local Eurasian Continent (EC), and the remaining other source regions (Other). It should be noted that the EC includes Europe (EUR), Central Asia (CAS), and North Asia (NAS).