Abstract
Macroscopic order appears as the collective behaviour of many interacting particles. Prime examples are superfluidity in helium1, atomic Bose–Einstein condensation2, s-wave3 and d -wave superconductivity4 and metal–insulator transitions5. Such physical properties are tightly linked to spin and charge degrees of freedom and are greatly enriched by orbital structures6. Moreover, high-orbital states of bosons exhibit exotic orders distinct from the orders with real-valued bosonic ground states7. Recently, a wide range of related phenomena have been studied using atom condensates in optical lattices8,9,10, but the experimental observation of high-orbital orders has been limited to momentum space11,12. Here we establish microcavity exciton–polariton condensates as a promising alternative for exploring high-orbital orders. We observe the formation of d -orbital condensates on a square lattice and characterize their coherence properties in terms of population distributions both in real and momentum space.
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References
Leggett, A. J. Quantum Liquids: Bose Condensation and Cooper Pairing in Condensed-Matter Systems (Oxford Univ. Press, 2006).
Pitaevskii, L. P. & Stringari, S. Bose–Einstein Condensation (Clarendon, 2003).
Tinkham, M. Introduction to Superconductivity (McGraw-Hill, 1996).
Van Harlingen, D. J. Phase-sensitive tests of the symmetry of the pairing state in the high-temperature superconductors—evidence for d x 2 − y 2 symmetry. Rev. Mod. Phys. 67, 515–535 (1995).
Imada, M., Fujimori, A. & Tokura, Y. Metal–insulator transitions. Rev. Mod. Phys. 70, 1039–1263 (1998).
Tokura, Y. & Nagaosa, N. Orbital physics in transition-metal oxides. Science 288, 462–468 (2000).
Wu, C. Unconventional Bose–Einstein condensations beyond the ‘no-node’ theorem. Mod. Phys. Lett. B 23, 1–24 (2009).
Greiner, M. et al. Quantum phase transition from a superfluid to a Mott insulator in a gas of ultracold atoms. Nature 415, 39–44 (2002).
Paredes, B. et al. Tonks–Girardeau gas of ultracold atoms in an optical lattice. Nature 429, 277–281 (2004).
Chin, J. K. et al. Evidence for superfluidity of ultracold fermions in an optical lattice. Nature 443, 961–964 (2006).
Müller, T., Fölling, S., Widera, A. & Bloch, I. State preparation and dynamics of ultracold atoms in higher lattice orbitals. Phys. Rev. Lett. 99, 200405 (2007).
Köhl, M., Moritz, H., Stöferle, T., Günter, K. & Esslinger, T. Fermionic atoms in a three dimensional optical lattice: Observing Fermi surfaces, dynamics, and interactions. Phys. Rev. Lett. 94, 080403 (2005).
Kavokin, A. & Malpuech, G. Cavity Polaritons (Academic, 2003).
Deng, H. et al. Condensation of semiconductor microcavity exciton polaritons. Science 298, 199–202 (2002).
Kasprzak, J. et al. Bose–Einstein condensation of exciton polaritons. Nature 443, 409–414 (2006).
Balili, R. et al. Bose–Einstein condensation of microcavity polaritons in a trap. Science 316, 1007–1010 (2007).
Bajoni, D. et al. Polariton laser using single micropillar GaAs–GaAlAs semiconductor cavities. Phys. Rev. Lett. 100, 047401 (2008).
Lai, C. W. et al. Coherent zero-state and π-state in an exciton–polariton condensate array. Nature 450, 529–533 (2007).
Salamon, M. B. & Jaime, M. The physics of manganites: Structure and transport. Rev. Mod. Phys 73, 583–628 (2001).
Ishida, K., Nakai, Y. & Hosono, H. To what extent iron-pnictide new superconductors have been clarified: A progress report. J. Phys. Soc. Jpn 78, 062001 (2009).
Mazin, I. I. & Schmalian, J. Pairing symmetry and pairing state in ferropnictides: Theoretical overview. Physica C 469, 614–627 (2009).
Feynman, R. P. Statistical Mechanics: A Set of Lectures (Addison-Wesley, 1972).
Wirth, G., Ölschläger, M & Hemmerich, A. Evidence for orbital superfluidity in the P -band of a bipartite optical square lattice. Nature Phys. 7, 147–153 (2010).
Sanvitto, D. et al. Exciton–polariton condensation in a natural two-dimensional trap. Phys. Rev. B 80, 045301 (2009).
Maragkou, M. et al. Spontaneous nonground state polariton condensation in pillar microcavities. Phys. Rev. B 81, 081307 (2010).
Kim, N. Y. et al. GaAs microcavity exciton–polaritons in a trap. Phys. Status. Solidi B 245, 1076–1079 (2008).
Ashcroft, N. W. & Mermin, N. D. Solid State Physics (Brooks Cole, 1989).
Acknowledgements
We acknowledge Special Coordination Funds for Promoting Science and Technology in Japan, Navy/SPAWAR Grant N66001-09-1-2024, MEXT, the Japan Society for the Promotion of Science (JSPS) through its Funding Program for World-Leading Innovative R&D on Science and Technology (FIRST Program), and State of Bavaria. C.W. is supported by the NSF under grant no. DMR-0804775.
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Y.Y. and N.Y.K. conceived this study. A.L. and S.H. grew the wafer. K.K processed the device. N.Y.K. built an optical set-up, and N.Y.K., K.K. and N.M. carried out experiments. N.Y.K. and Y.Y. analysed experimental data and C.W. carried out band-structure calculations. N.Y.K. and Y.Y. wrote the manuscript. All authors discussed the results and commented on the manuscript.
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Kim, N., Kusudo, K., Wu, C. et al. Dynamical d-wave condensation of exciton–polaritons in a two-dimensional square-lattice potential. Nature Phys 7, 681–686 (2011). https://doi.org/10.1038/nphys2012
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DOI: https://doi.org/10.1038/nphys2012
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