Abstract
Ultrafast electron diffractive imaging of nanoscale objects such as biological molecules1,2 and defects in solid-state devices3 provides crucial information on structure and dynamic processes: for example, determination of the form and function of membrane proteins, vital for many key goals in modern biological science, including rational drug design4. High brightness and high coherence are required to achieve the necessary spatial and temporal resolution, but have been limited by the thermal nature of conventional electron sources and by divergence due to repulsive interactions between the electrons, known as the Coulomb explosion. It has been shown that, if the electrons are shaped into ellipsoidal bunches with uniform density5, the Coulomb explosion can be reversed using conventional optics, to deliver the maximum possible brightness at the target6,7. Here we demonstrate arbitrary and real-time control of the shape of cold electron bunches extracted from laser-cooled atoms. The ability to dynamically shape the electron source itself and to observe this shape in the propagated electron bunch provides a remarkable experimental demonstration of the intrinsically high spatial coherence of a cold-atom electron source, and the potential for alleviation of electron-source brightness limitations due to Coulomb explosion6.
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Acknowledgements
We thank E. J. D. Vredenbregt and O. J. Luiten for discussions and advice. This work was supported by the Australian Research Council Federation Fellowship scheme and Australian Research Council Discovery Project DP1096025.
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A.J.M. and D.V.S. contributed equally to this work; they executed the experiments and acquired and analysed the data; S.D.S. contributed to the analysis of electron coherence; D.V.S., M.J. and S.C.B. designed and constructed the apparatus; K.A.N. contributed to the theoretical analysis; A.J.M., D.V.S., K.A.N. and R.E.S. wrote the manuscript; R.E.S. conceived and directed the project.
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McCulloch, A., Sheludko, D., Saliba, S. et al. Arbitrarily shaped high-coherence electron bunches from cold atoms. Nature Phys 7, 785–788 (2011). https://doi.org/10.1038/nphys2052
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DOI: https://doi.org/10.1038/nphys2052
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