Fig. 3: Simulations of time evolution of reactants’ distribution, P(x, t).
From: Effects of nonequilibrium fluctuations on ultrafast short-range electron transfer dynamics
The simulations are performed with different solvation timescales τD, while values of other parameters used are the same as those in Fig. 2. The bold red line represents the curve of −k(x) without scaling. Within each graph, the upper panel displays the time evolution of P(x, t), while the lower panel displays the evolution of the reaction rate’s distribution, −k(x)P(x, t). a τD = 0.1 ps. b τD = 10 ps. c τD = 3 ns.
