Fig. 1: Illustrative of top-down and bottom-up crystallization.

Conventional downward crystallization by a anti-solvent dripping in 3D PVSKs, b direct spin-coating in 2D PVSKs and c upward crystallization by ISC method in 2D PVSKs.

Conventional downward crystallization by a anti-solvent dripping in 3D PVSKs, b direct spin-coating in 2D PVSKs and c upward crystallization by ISC method in 2D PVSKs.