Fig. 3: Dynamicity, self-healability and reprocessability.

Normalized stress relaxation of (a) PTU1 and (b) PTU11 as a function of temperature. The insets show the temperature variations of the characteristic relaxation time, τ*, fitted according to Arrhenius equation. Storage shear modulus, G’, and loss shear modulus, G”, versus frequency of (c) PTU1 and (d) PTU11 recorded at different temperatures, respectively. Healed version of bisect PTU1 subjected to (e) a lateral load of 200 g in the single cantilever mode, and (f) a 5 kg weight in the parallel direction (35 × 2 × 1.2 mm). g Photos showing molding of pulverized PTU1 into square sheet and dog-bone-shaped specimens via hot pressing (100 °C, 4 MPa, 4 h). h Typical tensile stress-strain curves of the virgin and repaired PTUs. i Typical tensile stress-strain curves of the recycled PTU1.