Introduction

The concept of quantum steering can be traced back to the renowned debate on the completeness of quantum mechanics initiated by Einstein, Podolsky, and Rosen in 19351, along with the subsequent responses from Schrödinger2. Quantum steering refers to the ability of one party (Alice) in a composite quantum system to influence the quantum state of another party (Bob) through local measurements. This phenomenon implies a distinct form of non-local correlations that are found to exist between quantum entanglement and Bell non-locality3,4,5.

Recently, a lot of efforts have been made to characterize and understand quantum steering by means of local hidden state (LHS) models and steering inequalities. In seminal works3,6, Wiseman et al. established the steering thresholds for Werner states and isotropic states under projective measurements by constructing LHS models (c.f. also refs. 7,8). Subsequent advances by Nguyen and Gühne determined the new thresholds for the restricted case of dichotomic measurements performed by Alice9. Very recently, people found the Wiseman et al.’s threshold condition remains valid for positive operator-valued measurements (POVMs) in qubit systems10,11, which challenges the presumed advantage of POVMs in quantum steering scenario. Moreover, similar to Bell non-locality, quantum steering can be identified as well by the violation of some inequalities. This provides a practical way to detect the quantum steering in experiments. To this aim, various steering inequalities have been proposed, including the well-known Reid criteria12, linear steering inequalities13,14, and steering inequalities based on various uncertainty relations15,16,17,18,19,20,21,22, among others (see reviews5,23,24). Due to the equivalence between quantum steering and incompatibility of measurements25, the results of measurement incompatibility can also be employed to characterize quantum steering26. In recent years, high-dimensional quantum steering has garnered significant attention due to its enhanced robustness against noise and loss27,28,29,30,31, while limited inequalities are established, merely applicable to qubit system or systems with specific measurement settings, such as mutually unbiased bases (MUBs).

Over the past few decades, majorization theory has found widespread applications across various aspects of quantum information science32,33,34,35,36,37,38,39,40,41,42,43. Of particular significance is the majorization lattice44,45,46,47, which establishes an algebraic structure for the set of probability distributions, providing a framework that is naturally congruent with the probabilistic descriptions inherent to quantum theory. Recently, majorization theory has been applied to quantum steering22,48,49 in lower-dimensional systems.

In this paper, we present a systematic approach to the detection of quantum steering based on the probability majorization lattice. Notably, this method is applicable to any measurement setting and any dimension, by which the quantum correlation information encoded in joint probabilities can then be fully extracted through tailored aggregation operations. This leads to lossless information extraction in contrast to conventional methods relying on functions of probability distributions, such as entropy and variance. To illustrate the efficacy of our approach, we derive steering inequalities for two-qubit systems, as well as for arbitrary-dimensional Werner states and isotropic states. In the MUBs scenario, our approach not only yields stronger steering inequalities compared to existing ones, but also indicates that previous high-dimensional steering inequalities can be systematically obtained in a series of approximations. In the following we present first the preliminary preparation for later use, then the derivation of our central theorem, and representative examples confronting to the yet known results.

Results

Preliminaries

Majorization theory establishes a partial ordering relation between any two vectors \(\vec{x},\vec{y}\in {{\mathbb{R}}}^{n}\) with \({\sum }_{i=1}^{n}{x}_{i}={\sum }_{i=1}^{n}{y}_{i}\), denoted \(\vec{x}\prec \vec{y}\), i.e. \(\vec{x}\) is majorized by \(\vec{y}\), if and only if50

$$\mathop{\sum }\limits_{i=1}^{k}{x}_{i}^{\downarrow }\le \mathop{\sum }\limits_{i=1}^{k}{y}_{i}^{\downarrow },k=1,\cdots \,,n-1.$$
(1)

Here, the superscript denotes the components of \(\vec{x}\) and \(\vec{y}\) in decreasing order. For n-dimensional probability vectors with components in decreasing order, we can define

$${{\mathcal{P}}}_{n}\equiv \left\{{({p}_{1},\cdots \,,{p}_{n})}^{{\rm{T}}}| {p}_{i}\ge {p}_{i+1}\ge 0,\mathop{\sum }\limits_{i=1}^{n}{p}_{i}=\mathrm{const}.\right\}.$$
(2)

The set \({{\mathcal{P}}}_{n}\), equipped with the majorization relation defined in Eq. (1), forms a lattice44 (see51 for a thorough discussion). In mathematics, a lattice is defined as a quadruple, and a probability majorization lattice can be represented as \(\langle {{\mathcal{P}}}_{n},\prec ,\vee ,\wedge \rangle\), where for \(\forall \vec{p},\vec{q}\in {{\mathcal{P}}}_{n}\) there is a unique infimum \(\vec{p}\wedge \vec{q}\) and a unique supremum \(\vec{p}\vee \vec{q}\). It is proved that the probability majorization lattice is a complete lattice and we have45,46,47

Lemma 1

A probability majorization lattice is a complete lattice, meaning that for every subset \(S\subseteq {{\mathcal{P}}}_{n}\), both the supremum \({\bigvee }S\in {{\mathcal{P}}}_{n}\) and the infimum \({\bigwedge }S\in {{\mathcal{P}}}_{n}\) exist.

Probability majorization lattice provides an elegant formalism to establish state-independent uncertainty relation (UR). For any observables A, B in a d-dimensional Hilbert space \({\mathcal{H}}\), one can define the measurement distribution set as

$${{\mathcal{P}}}_{A,B}=\left\{{\vec{p}}_{A}\odot {\vec{p}}_{B}| {\vec{p}}_{A}\in {{\mathcal{P}}}_{A},{\vec{p}}_{B}\in {{\mathcal{P}}}_{B}\right\}.$$
(3)

Here, \({{\mathcal{P}}}_{A}\) and \({{\mathcal{P}}}_{B}\) are respectively the sets of probability vectors corresponding to the measurements A and B, such as \({{\mathcal{P}}}_{A}=\{{(p({a}_{1}| A),\cdots \,,p({a}_{d}| A))}^{T}| \rho \in {\mathcal{D}}({\mathcal{H}})\}\) with the set of density matrices \({\mathcal{D}}({\mathcal{H}})\) for d-dimensional Hilbert space \({\mathcal{H}}\); denotes any binary operation that preserve the majorization relation, including direct sum, direct product, and vector sum, i.e. { , , + }. In light of Lemma 1, a probability majorization lattice is a complete lattice and there exists a supremum for the subset \({{\mathcal{P}}}_{A,B}\subset {{\mathcal{P}}}_{n}\), which formulates the majorization-based state-independent UR:

$$\forall \vec{\chi }\in {{\mathcal{P}}}_{A,B},\vec{\chi }\prec \vec{\omega }(A,B),$$
(4)

where \(\vec{\omega }(A,B)=\bigvee {{\mathcal{P}}}_{A,B}\). Clearly, the statements above can be generalized to the scenario involving N measurements. Note that the bound \(\vec{\omega }(A,B)\) with binary operations { , } has been extensively studied in refs. 37,38,39,40,41,42,43,48. Let Iμ [d] be a subset of [d], where [d] be the set of all integers from 1 to d. For binary operation , we have \(\vec{\omega }({\mathcal{B}})=({\Omega }_{1},{\Omega }_{2}-{\Omega }_{1},\cdots \,,{\Omega }_{Nd}-{\Omega }_{N(d-1)},0,\cdots \,,0)\), where ΩL for N measurements \({\mathcal{B}}=({B}_{1},\cdots \,,{B}_{N})\) is defined as

$${\Omega }_{L}\equiv \mathop{\max }\limits_{\begin{array}{l}{I}_{1},\cdots \,,{I}_{N}\\ {\sum }_{\mu =1}^{N}| {I}_{\mu }| =L\end{array}}\mathop{\max }\limits_{\rho }{\text{T}}{\rm{r}}\left[\rho \left(\mathop{\sum }\limits_{\mu =1}^{L}\mathop{\sum }\limits_{i\in {I}_{\mu }}| {b}_{i}^{(\mu )}\rangle \langle {b}_{i}^{(\mu )}| \right)\right]$$
(5)
$$=\mathop{\max }\limits_{\begin{array}{l}{I}_{1},\cdots \,,{I}_{N}\\ {\sum }_{\mu =1}^{N}| {I}_{\mu }| =L\end{array}}\left|\left|\mathop{\sum }\limits_{\mu =1}^{L}\mathop{\sum }\limits_{i\in {I}_{\mu }}| {b}_{i}^{(\mu )}\rangle \langle {b}_{i}^{(\mu )}| \right|\right|.$$
(6)

Here, denotes the operator norm and \(| {b}_{i}^{(\mu )}\rangle \langle {b}_{i}^{(\mu )}|\) is μ-th projector of measurement base Bμ (see Methods for more details).

Probability majorization lattice and quantum steering

Assuming that Alice and Bob each possess one of the two subsystems of a bipartite state and measure on bases A and B respectively, in projective measurement, quantum theory predicts the joint probability

$$p({a}_{i},{b}_{j}| A,B;\rho )=Tr[{\Pi }_{ij}\rho ]$$
(7)

with projectors \({\Pi }_{ij}=| {a}_{i}\rangle \langle {a}_{i}| \otimes | {b}_{j}\rangle \langle {b}_{j}|\). Considering of all alternative measurements, a bipartite quantum state corresponds to the infinite set of joint probability p(ai, bjA, B; ρ), i.e.

$$\rho \to {\mathcal{P}}=\{p({a}_{i},{b}_{j}| A,B;\rho )| \forall A,B\}.$$
(8)

If the LHS description does not exist, i.e. \(p({a}_{i},{b}_{j}| A,B;\rho )\ne {\sum }_{\xi }\wp ({a}_{i}| A,\xi )Tr[{\Pi }_{j}^{B}{\rho }_{\xi }^{B}]{\wp }_{\xi }\) for certain measurements A and B, Alice can then demonstrably steer Bob’s state, hence exhibiting the quantum steering3. Here, {ξ, ξ}, (aiA, ξ) and \({\rho }_{\xi }^{B}\) denote the possible hidden variables, Alice’s measurement distribution and Bob’s local state, respectively.

In practical experiments, only a finite number of measurement settings can be implemented. We define the set of the joint distributions of non-steerable states in N-measurement scenario as follows:

$${P}_{\mathrm{ns}}^{N}=\left\{\mathop{\mathop{\bigodot}\limits^{N}}\limits_{\mu =1}\vec{p}{({A}_{\mu }\otimes {B}_{\mu })}_{\rho }|\rho \in {D}_{\mathrm{ns}}\right\}.$$
(9)

Here, \({{\mathcal{D}}}_{ns}\) signifies the set of non-steerable states. Clearly, \({{\mathcal{P}}}_{ns}^{N}\) sets up a subset of the probability majorization lattice \({{\mathcal{P}}}_{n}\). Moreover, by Lemma 1, there exists a supremum over all non-steerable states, from which the steerability condition follows:

Lemma 2

Given the orthonormal complete base sets \({\mathcal{A}}=({A}_{1},\cdots \,,{A}_{N})\) and \({\mathcal{B}}=({B}_{1},\cdots \,,{B}_{N})\) for Hilbert spaces \({{\mathcal{H}}}_{A}\) and \({{\mathcal{H}}}_{B}\), the violation of the following majorization inequality

$$\mathop{\bigodot }\limits_{\mu =1}^{N}\vec{p}{({A}_{\mu }\otimes {B}_{\mu })}_{\rho }\prec \vec{\delta }({\mathcal{A}},{\mathcal{B}}),\vec{\delta }({\mathcal{A}},{\mathcal{B}})=\bigvee {{\mathcal{P}}}_{ns}^{N}$$
(10)

signifies the steerability of the quantum state ρ.

Although Lemma 2 establishes a direct connection between quantum steering and probability majorization lattice, calculating the supremum \(\vec{\delta }({\mathcal{A}},{\mathcal{B}})\) presents an intractable challenge. It can be shown that in the quantum steering scenario, the supremum \(\vec{\delta }({\mathcal{A}},{\mathcal{B}})\) can be replaced by the majorization UR bound \(\vec{\omega }({\mathcal{B}})\), thereby formulating an operational steering detection framework. To this end, we employ the concept of aggregating a probability distribution48,52,53,54. Given probability vectors \(\vec{p}\in {{\mathcal{P}}}_{n}\) and \(\vec{q}\in {{\mathcal{P}}}_{m}\), \(\vec{q}\) is referred as an aggregation of \(\vec{p}\) if there is a partition \({\mathcal{I}}\) of {1, , n} into disjoint sets I1, , Im such that \({q}_{j}={\sum }_{i\in {I}_{j}}{p}_{i}\), for j = 1, , m. The vector \(\vec{q}\) can then be denoted as \(\vec{q}={\mathcal{I}}(\vec{p})\) and we have the following theorem (proof shown in Supplementary Note 1):

Theorem 1

Given orthonormal complete base sets \({\mathcal{A}}=({A}_{1},\cdots \,,{A}_{N})\) and \({\mathcal{B}}=({B}_{1},\cdots \,,{B}_{N})\) for Hilbert spaces \({{\mathcal{H}}}_{A}\) and \({{\mathcal{H}}}_{B}\), the violation of the following majorization inequality

$$\mathop{\bigodot }\limits_{\mu =1}^{N}{\mathcal{I}}(\vec{p}{({\mathcal{J}}({A}_{\mu })\otimes {\mathcal{E}}({B}_{\mu }))}_{\rho })\prec \vec{\omega }({\mathcal{B}})$$
(11)

signifies the steerability of quantum state ρ (from Alice to Bob). Here, \(\vec{\omega }({\mathcal{B}})\) is the majorization UR bound of \({\mathcal{B}}=({B}_{1},\cdots \,,{B}_{N})\) for binary operations { , , + } and \({\mathcal{I}}(\vec{p}{({A}_{\mu }\otimes {B}_{\mu })}_{\rho })\) denotes all aggregations of \(\vec{p}{({A}_{\mu }\otimes {B}_{\mu })}_{\rho }\) with partitions \({\mathcal{I}}\) satisfying \({\mathcal{I}}(\vec{p}\otimes \vec{q})\prec \vec{q}\); \({\mathcal{E}}\) denotes the local transformations preserving the majorization UR bound \(\vec{\omega }({\mathcal{B}})\), i.e., \(\vec{\omega }({\mathcal{E}}({\mathcal{B}}))=\vec{\omega }({\mathcal{B}})\); \({\mathcal{J}}\) represents any local transformation of measurement Alice performs.

Theorem 1 provides a criterion for quantum steering that is applicable to arbitrary finite dimension and measurement settings. It offers a novel perspective that quantum correlation information embedded in the joint probability can be extracted through appropriate aggregation operations of joint probability distributions. Next, to exhibit the capacity of the above theorem in steering detection, we first develop some steering inequalities from it and then apply the inequalities to some typical states.

Witnessing quantum steering via the majorization formalism

For illustration, we herein focus on the binary operation and present some practical steering inequalities. Employing the Bloch representation, a bipartite state is expressed in the form of

$$\begin{array}{rcl}\rho & = & \frac{1}{{d}^{2}}{\mathbb{1}}\otimes {\mathbb{1}}+\frac{1}{2d}\vec{u}\cdot \vec{\pi }\otimes {\mathbb{1}}+\frac{1}{2d}{\mathbb{1}}\otimes \vec{v}\cdot \vec{\pi }\\ & & +\frac{1}{4}\mathop{\sum }\limits_{\mu ,\nu }{{\mathcal{T}}}_{\mu \nu }{\pi }_{\mu }\otimes {\pi }_{\nu }.\end{array}$$
(12)

Here, the coefficient matrix entries are \({u}_{\mu }=Tr[{\rho }_{A}{\pi }_{\mu }]\), \({v}_{\mu }=Tr[{\rho }_{B}{\pi }_{\mu }]\) and \({{\mathcal{T}}}_{\mu \nu }=Tr[\rho {\pi }_{\mu }\otimes {\pi }_{\nu }]\) with generators \({\{{\pi }_{\mu }\}}_{\mu =1}^{{d}^{2}-1}\) of \({\mathfrak{su}}(d)\) Lie algebra. Let us consider the partition \({\mathcal{I}}=\{{I}_{1},\cdots \,,{I}_{d}\}\) of {(1, 1), , (1, n), , (i, j), , (d, d)} with elements

$${I}_{k}=\{(i,j)| j\equiv (i+k-1)\,(mod\,\,d),1\le i,j\le d\},$$
(13)

where k = 1, , d. It has been proved that the partition \({\mathcal{I}}=\{{I}_{1},\cdots \,,{I}_{d}\}\) satisfies \({\mathcal{I}}(\vec{p}\otimes \vec{q})\prec \vec{q}\), which is equivalent to the degenerate case of Lemma 1 in ref. 35. The partition \({\mathcal{I}}\) results in an aggregation \(\vec{\Upsilon }\) of p(ai, bjA, B; ρ) with components

$$\begin{array}{rcl}{\Upsilon }_{k}(A,B;\rho ) & = & \mathop{\sum }\limits_{(i,j)\in {I}_{k}}p({a}_{i},{b}_{j}| A,B;\rho )\\ & = & \frac{1}{d}+\frac{1}{4}\mathop{\sum }\limits_{(i,j)\in {I}_{k}}({\vec{a}}_{i},{\mathcal{T}}{\vec{b}}_{j}),\end{array}$$
(14)

where \({\vec{a}}_{i}({\vec{b}}_{j})\) is Bloch vectors of projectors. Based upon Theorem 1, we obtain the following majorization steering inequality:

$$\mathop{\bigoplus}\limits_{\mu =1}^{N}\vec{\Upsilon }({\mathcal{J}}({A}_{\mu }),{\mathcal{E}}({B}_{\mu });\rho )\prec \vec{\omega }({\mathcal{B}}),$$
(15)

which yields a family of aggregation \(\vec{\Upsilon }\) steering inequalities

$${{\mathcal{S}}}_{L}\equiv \frac{1}{L}\mathop{\sum }\limits_{k=1}^{L}{\left[\mathop{\bigoplus}\limits_{\mu}^{N}{\vec{\Upsilon}}_{\mu }\right]}_{k}^{\downarrow }\le {\overline{\Omega }}_{L},L=2,\cdots \,,Nd.$$
(16)

Here, \({[\cdot ]}_{k}^{\downarrow }\) denotes the largest k-th component of a vector and \({\overline{\Omega }}_{L}=\frac{{\Omega }_{L}}{L}\) with \({\Omega }_{L}={\sum }_{k=1}^{L}{[\vec{\omega }({\mathcal{B}})]}_{k}^{\downarrow }\). Similarly to the qubit situation13, we define the quantity \({{\mathcal{S}}}_{L}\) as the steering parameter for N measurement settings in arbitrary dimensional Hilbert space. The calculation of ΩL is a typical combinatorial optimization problem (COP). We derive three computational simple upper bounds ΛL, ΘL and ΓL for ΩL in the Supplementary Note 2. Especially, we have upper bounds for ΩL in the case of MUBs:

$$\{\begin{array}{l}{\Theta }_{L}=1+\frac{L-1}{\sqrt{d}},\\ {\Gamma }_{L}=\frac{L+\sqrt{(d-1)(dL-\Phi (L))}}{d},\end{array}$$
(17)

where \(\Phi (L)=N{\lfloor \frac{L}{N}\rfloor }^{2}+(L-N\lfloor \frac{L}{N}\rfloor )(2\lfloor \frac{L}{N}\rfloor +1)\) with the floor function and 1 ≤ L ≤ N(d − 1). Note that the upper bounds in Eq. (17) satisfy ΓLΘL for a complete set of MUBs (see Supplementary Note 2 for proofs and details). Note that the authors of ref. 26 defined the exact same quantity ΩL and obtained the same upper bound ΘL in terms of measurement incompatibility.

Applications

Next, we formulate quantum steering inequalities in two-qubit systems, arbitrary-dimensional Werner states, isotropic states and general scenario, with detailed calculations given in Supplementary Note 3.

Two qubits system

Given spin observables \({A}_{\mu }={\vec{a}}_{\mu }\cdot \vec{\sigma }\) and \({B}_{\mu }={\vec{b}}_{\mu }\cdot \vec{\sigma }\) with Pauli matrices vector \(\vec{\sigma }\), we have the aggregated joint probability for a two-qubit system

$${\Upsilon }_{\pm }=\frac{1}{2}\left[1\pm (\vec{t}\circ {\vec{a}}_{\mu })\cdot {\vec{b}}_{\mu }\right].$$
(18)

Here, \(\vec{t}=({t}_{1},{t}_{2},{t}_{3})\) is the singular value vector of \({\mathcal{T}}\); denotes Hadamard product. Considering the two-qubit Werner state \({\rho }_{W}=(1-w){\mathbb{1}}/4+w| {\psi }_{-}\rangle \langle {\psi }_{-}|\) with \(| {\psi }_{-}\rangle =\frac{1}{\sqrt{2}}(| 01\rangle -| 10\rangle )\) and setting \({\vec{a}}_{\mu }={\vec{b}}_{\mu }\), we have \({\Upsilon }_{\pm }=\frac{1\pm w}{2}\) and

$${{\mathcal{S}}}_{N}=\frac{1+w}{2},$$
(19)

which yields a steering threshold for the two-qubit Werner state: \({w}^{* }=2{\overline{\Omega }}_{N}-1\). Throughout this paper, we define the steering threshold as the minimum value of the state parameter (e.g., the visibility \({w}\) for Werner states) sufficient to violate the steering inequalities under a given measurement setting. Notably, this result is equivalent to the linear steering inequality established by Saunders et al.13. Furthermore, when measurements are conducted over the entire hemisphere of the Bloch sphere, there exists a limit of \({\mathrm{lim}}_{N\to \infty }\frac{{\Omega }_{N}}{N}=\frac{3}{4}\), which leads to a threshold of 1/2.

Isotropic state and Werner state in dimension d

Without loss of generality, one can set \({A}_{\mu }={\vec{a}}_{\mu }\cdot \vec{\pi }\) and \({B}_{\mu }={\vec{b}}_{\mu }\cdot \vec{\pi }\) with μ = 1, , N, where \({\vec{a}}_{\mu },{\vec{b}}_{\mu }\) are (d2 − 1) dimensional real vectors. For isotropic states and Werner states, we have the aggregated joint probabilities

$${\Upsilon }_{k}^{{\rm{I}}{\rm{S}}{\rm{O}}}=\left\{\begin{array}{l}\frac{1+(d-1)w}{d},k=1,\\ \frac{1-w}{d},k=2,\cdots \,,d,\end{array}\right.$$
(20)
$${\Upsilon }_{k}^{{\rm{W}}}=\left\{\begin{array}{l}\frac{1-\eta }{d},k=1,\\ \frac{d-1+\eta }{d(d-1)},k=2,\cdots \,,d.\end{array}\right.$$
(21)

and steering parameters

$${{\mathcal{S}}}_{N}^{ISO}=\frac{1+(d-1)w}{d},{{\mathcal{S}}}_{N(d-1)}^{W}=\frac{d-1+\eta }{d(d-1)}.$$
(22)

Here, w and η [0, 1] are noise parameters for the isotropic and Werner state, respectively. By Eq. (16), we obtain the steering thresholds for isotropic and Werner states, respectively

$${w}^{* }=(d{\overline{\Omega }}_{N}-1)/(d-1),$$
(23)
$${\eta }^{* }=(d-1)(d{\overline{\Omega }}_{N(d-1)}-1).$$
(24)

For the case of two measurement settings, we obtain \({\overline{\Omega }}_{2}=(1+c)/2\) with \(c={\max }_{i,j}| \langle {a}_{i}| {b}_{j}\rangle |\) representing the maximal overlap of the two bases. The steering threshold is then \({w}^{* }=\frac{d(1+c)-2}{2(d-1)}\), which implies that the results in refs. 29,55,56 are the special cases corresponding to pairs of MUBs. A notable correspondence exists between the steering thresholds derived from the majorization lattice framework and those obtained from the measurement incompatibility perspective26,57,58. This relationship becomes apparent when reformulating Eq. (23) ang (24) in terms of ΩN and ΩN(d−1), as shown in Table 1. Remarkably, for the isotropic states, our result coincides exactly with the noise robustness derived from the perspective of measurement incompatibility57,58.

Table 1 Comparison of steering thresholds derived from the majorization lattice framework and the measurement incompatibility perspective

Utilizing upper bounds derived in Eq. (17), we obtain approximate steering thresholds for isotropic states and Werner states, as summarized in Table 2. These bounds provide an excellent approximation for isotropic state steering scenario involving MUBs, which significantly simplifies the analysis of steering in high-dimensional system. Note, the thresholds in refs. 20,27,31 are compatible with the upper bounds of \({\overline{\Theta }}_{N}\) and \({\overline{\Gamma }}_{N}\), respectively, which indicates that those previous results are not optimal ones for isotropic state. As illustrated in Fig. 1, we compute the optimal steering thresholds for various isotropic states with MUBs dimensions, from d = 2 to 8 for illustration, and compare these thresholds with those from \({\overline{\Gamma }}_{N},{\overline{\Theta }}_{N}\), as well as the critical values from LHS model3,7,8.

Fig. 1: The steering thresholds of the isotropic states for different dimensions d, in case of a complete set of MUBs.
Fig. 1: The steering thresholds of the isotropic states for different dimensions d, in case of a complete set of MUBs.
Full size image

The red and green lines represent the steering threshold derived from the approximate upper bounds \({\overline{\Theta }}_{N}\) and \({\overline{\Gamma }}_{N}\), respectively. The cyan line indicates the optimal steering threshold from \({\overline{\Omega }}_{N}\), while the magenta line represents the critical value of isotropic states derived from the LHS model3,7,8. Note that, due to the existence problem of 6-dimensional MUBs, the threshold for d = 6 is calculated using only three MUBs.

Table 2 Steering thresholds of isotropic (w*) and Werner (η*) states derived from upper bounds \({\overline{\Gamma }}_{N}\) and \({\overline{\Theta }}_{N}\)

It is noteworthy that for d > 2, the steering threshold of Werner states in Table 2 exceeds 1, i.e. η*≥1, which indicates that MUBs fail to witness the steerability of Werner states in high dimensions. Intuitively, this follows from \({\eta }^{* }=1-\frac{d}{N}(N-{\Omega }_{N(d-1)})\), where ΩN(d−1) is close to N for MUBs. Conversely, non-MUB measurements with ΩN(d−1) < N are expected to perform better. It is worth noting that Nguyen et al. showed that MUBs can never detect steering for Werner states in odd prime-power dimensions, a limitation that appears to hold asymptotically for even prime-power dimensions (e.g. η* = 0.9174 for d = 4)58. These findings highlight an intriguing fact that while MUBs effectively capture the steerability of isotropic states, they perform poorly for witnessing the steerability of Werner states in high dimensions.

Notice that the new approach enables the investigation of optimal measurement settings for quantum steering. Consequently, we are tasked with addressing the optimization problem

$$\begin{array}{rcl} & \min & {\overline{\Omega }}_{N}\\ & s.t. & {\mathcal{B}}=({B}_{1},\cdots \,,{B}_{N}),\forall {B}_{\mu }={B}_{\mu }^{\dagger }.\end{array}$$
(25)

In Fig. 2, we examine the optimal settings for qutrit isotropic and Werner states using the Cross-Entropy Method (CEM)59,60, a powerful technique for solving complex continuous optimization problems and machine learning tasks. As shown in Fig. 2a, b, we compute the steering thresholds for qutrit isotropic states in N = 2 to 13 measurement settings and for qutrit Werner states in N = 2 to 8 measurement settings. Our results indicate that MUBs remain optimal for N = 2, 3, 4 in isotropic scenario. Notably, Bavaresco et al. obtained smaller upper bounds for projective measurements using semidefinite programming (SDP) and search algorithms61, resulting in a small gap between their results and our lower bounds. A plausible explanation is that both the CEM and the search algorithms are heuristic optimization methods, which do not guarantee finding the global optimum. To certify the steerability of qutrit Werner states, the optimal measurement settings always be non-MUBs. Lower thresholds are achieved as the number of measurement settings N increases. We conjecture that the critical values 5/12 and 2/3 can be attained in the limit as N for both qutrit isotropic and Werner states, respectively, similarly to the scenario in two-qubit Werner states.

Fig. 2: The steering threshold value of the qutrit isotropic and Werner states for N measurement settings.
Fig. 2: The steering threshold value of the qutrit isotropic and Werner states for N measurement settings.
Full size image

Here, we plot the steering threshold of qutrit isotropic states (a) and Werner states (b) obtained from the Cross-Entropy Method (CEM) for N = 2 to 13 and N = 2 to 8, respectively. The red points represent the critical values 5/12 and 2/3 of qutrit isotropic and Werner states from LHS model3,7,8. a Qutrit isotropic states. b Qutrit Werner states.

General scenario

Here, we formulate the steering detection in a general scenario where Alice’s measurements are related to Bob’s measurements via unitary or anti-unitary transformations, i.e., \({A}_{\mu }={\mathcal{J}}({B}_{\mu })\). This leads to the following steering inequality:

$$\mathop{\bigoplus}\limits_{\mu =1}^{N}\vec{\Upsilon }({\mathcal{J}}({B}_{\mu }),{B}_{\mu };\rho )\prec \vec{\omega }({\mathcal{B}}).$$
(26)

Since the joint probability distributions \(\vec{\Upsilon }\) depend on the choice of \({\mathcal{J}}\), there exists an optimal alignment between Alice’s and Bob’s measurements for steering detection. The optimal alignment mechanism necessarily minimizes the entropy of the aggregated joint probability distributions. Therefore, the optimal \({\mathcal{J}}\) can be obtained by solving the optimization problem:

$$\begin{array}{rcl} & \min & H\left(\mathop{\bigoplus}\limits_{\mu =1}^{N}\vec{\Upsilon }({\mathcal{J}}({B}_{\mu }),{B}_{\mu };\rho )\right)\\ & s.t. & {\mathcal{J}}\,is\,unitary\,or\,anti-unitary,\end{array}$$
(27)

where H( ) denotes the Shannon entropy.

We now apply the above procedure to detect steerability in a general scenario. Consider the following family of qutrit states:

$$\rho (\lambda ,\theta ,\phi )=\lambda | \psi (\theta ,\phi )\rangle \langle \psi (\theta ,\phi )| +(1-\lambda )\frac{{\mathbb{1}}}{9},$$
(28)

where \(| \psi (\theta ,\phi )\rangle =\cos \theta \sin \phi | 00\rangle +\sin \theta \sin \phi | 11\rangle +\cos \phi | 22\rangle\), with λ [0, 1], θ [0, π/4] and ϕ [0, π/2]. This state reduces to the isotropic state when θ = π/4 and \(\phi =\arctan \sqrt{2}\). We consider the measurement setting \({\mathcal{B}}=({B}_{1},{B}_{2},U{B}_{3}{U}^{\dagger },U{B}_{4}{U}^{\dagger })\) with \(U={e}^{i\delta {J}_{z}}\), where B1, B2, B3, B4 are MUBs and Jz is the z component of the angular momentum operator. In Fig. 3, we plot the Lorenz curves of Eq. (26) for ρ(λ, θ, ϕ) with Schmidt rank 1 (θ = 0, ϕ = π/2), rank 2 (θ = π/4, ϕ = π/2), and rank 3 (θ = ϕ = π/3, \(\theta =\pi /4,\phi =\arctan \sqrt{2}\)) for both MUBs (Fig. 3a) and non-MUBs (Fig. 3b) cases. The Lorenz curve of a probability distribution vector \(\vec{p}\) is defined as \({f}_{\vec{p}}(k)\equiv {\sum }_{i=1}^{k}{p}_{i}^{\downarrow }\) with \({f}_{\vec{p}}(0)=0\). Note that Lorenz curves have been previously applied to investigate optimal uncertainty relations42. Genuine high-dimensional steering has attracted extensive attention recently62,63,64. These studies show that high-dimensional entanglement, as quantified by the Schmidt number, can lead to a stronger form of steering that is provably impossible to obtain via entanglement in lower dimensions. The results in Fig. 3 and Table 3 indicate that states with higher Schmidt rank reveal stronger robustness to noise (corresponding to a larger shaded area above the majorization bound curve). Conversely, lower Schmidt rank states (e.g., θ = π/4, ϕ = π/2) exhibit more pronounced sensitivity to noise and the choice of measurement settings.

Fig. 3: Lorenz curves for ρ(λ, θ, ϕ) with Schmidt rank 1(θ = 0, ϕ = π/2), 2(θ = π/4, ϕ = π/2) and \(3(\theta =\phi =\pi /3,\theta =\pi /4,\phi =\arctan \sqrt{2})\) for MUBs and non-MUBs cases.
Fig. 3: Lorenz curves for ρ(λ, θ, ϕ) with Schmidt rank 1(θ = 0, ϕ = π/2), 2(θ = π/4, ϕ = π/2) and 
                          $$3(\theta =\phi =\pi /3,\theta =\pi /4,\phi =\arctan \sqrt{2})$$
                          
                            
                              3
                              (
                              θ
                              =
                              ϕ
                              =
                              π
                              /
                              3
                              ,
                              θ
                              =
                              π
                              /
                              4
                              ,
                              ϕ
                              =
                              arctan
                              
                                
                                  2
                                
                              
                              )
                            
                          
                         for MUBs and non-MUBs cases.
Full size image

The black solid line represents the majorization bound \(\vec{\omega }({\mathcal{B}})\). The shadow region above the majorization bound curve indicates the steerable region detected by Eq. (26). a Steering of state ρ(λ, θ, ϕ) with MUBs. b Steering of state ρ(λ, θ, ϕ) with non-MUBs.

Table 3 Noise threshold λ* of \(| \psi (\theta ,\phi )\rangle\) for MUBs (δ = 0) and non-MUBs (δ = π/3) cases

Discussion

In this paper, we have established a connection between quantum steering and the probability majorization lattice, leading to a novel framework for detecting quantum steering. This framework is applicable to arbitrary finite dimensions and measurement settings. By introducing the concept of aggregating probability distributions, we have formulated a family of aggregation-based steering inequalities and applied them to the two-qubit systems, arbitrary-dimensional Werner and isotropic states and general scenarios.

From the perspective of information theory, our approach facilitates the extraction of quantum correlation information embedded in the joint probability without loss, utilizing appropriate aggregation operations that differ from those based on entropies and variances. In the context of mutually unbiased bases (MUBs), our approach not only reproduces known steering inequalities as approximate cases but also provides improved thresholds and new insights into the optimal measurement settings for detecting quantum steerability.

For high-dimensional Werner states, non-MUB measurements outperform MUBs in witnessing steerability. We investigate the optimal N-measurement settings for qutrit isotropic and Werner states using the Cross-Entropy Method (CEM), revealing that MUBs remain optimal for N = 2, 3, 4 for isotropic states, while non-MUBs are required for qutrit Werner states. Our framework can also be employed to explore quantum steering in more general scenarios by optimizing the alignment between Alice’s and Bob’s measurements. We illustrate this by examining a family of non-symmetric qutrit states.

High-dimensional quantum systems have garnered significant attentions in quantum information processing due to their enhanced resilience to noise, reduced susceptibility to loss, and greater information capacity. These advantages render them particularly valuable for applications in quantum communication65,66,67, quantum cryptography68, and superdense coding69. Hopefully, the majorization-based framework for quantum steering may enlighten our understanding of quantum correlation and facilitate practical applications across these areas.

Methods

Ω L of N measurement bases

Given N orthonormal and complete bases \({\{{| b\rangle }_{i}^{(\mu )}\}}_{i=1}^{d}\) for μ = 1, 2, , N, we define the index set I = {1, 2, , d} and the subsets I1, I2, , IN I, where Iμ denotes the index set of the μ-th basis Aμ. Assuming we choose L base vectors from the N bases, with each basis selecting Iμ vectors, we can define L projectors \(\{| {x}_{j}\rangle \langle {x}_{j}| \}\), \(j=1,2,\cdots \,,L={\sum }_{\mu =1}^{N}| {I}_{\mu }|\) as follows:

$$| {x}_{{i}_{1}}\rangle =| {a}_{i}^{(1)}\rangle ,\exists i\in {I}_{1},{i}_{1}=1,\cdots \,,| {I}_{1}| ,$$
(29)
$$\begin{array}{rcl}| {x}_{{i}_{2}}\rangle & = & | {a}_{i}^{(2)}\rangle ,\exists i\in {I}_{2},{i}_{2}=| {I}_{1}| +1,\cdots \,,| {I}_{1}| +| {I}_{2}| ,\\ & \vdots & \end{array}$$
(30)
$$| {x}_{{i}_{N}}\rangle =| {a}_{i}^{(N)}\rangle ,\exists i\in {I}_{N},{i}_{N}=\mathop{\sum }\limits_{\mu =1}^{N-1}| {I}_{\mu }| +1,\cdots \,,L=\mathop{\sum }\limits_{\mu =1}^{N}| {I}_{\mu }| .$$
(31)

Then, we can reformulate ΩL as

$${\Omega }_{L}\equiv \mathop{\max }\limits_{\begin{array}{l}{I}_{1},\cdots \,,{I}_{N}\\ {\sum }_{\mu =1}^{N}| {I}_{\mu }| =L\end{array}}\mathop{\max }\limits_{\rho }{\rm{T}}{\rm{r}}\left[{\rm{\rho }}\left(\mathop{\sum }\limits_{{\rm{j}}=1}^{{\rm{L}}}| {{\rm{x}}}_{{\rm{j}}}\rangle \langle {{\rm{x}}}_{{\rm{j}}}| \right)\right]$$
(32)
$$=\mathop{\max }\limits_{\begin{array}{l}{I}_{1},\cdots \,,{I}_{N}\\ {\sum }_{\mu =1}^{N}| {I}_{\mu }| =L\end{array}}\left|\left|\mathop{\sum }\limits_{j=1}^{L}| {x}_{j}\rangle \langle {x}_{j}|\right |\right|.$$
(33)

Here, denotes the operator norm, i.e. the largest singular value of the operator. Especially, if L > d(N − 1) we have ΩL = N (the maximal value possible), which occurs if I1 = = IN−1 = I and IN = {l}, \(\rho =| {a}_{l}^{(N)}\rangle \langle {a}_{l}^{(N)}|\). The solution of ΩL is a typical combinatorial optimization problem (COP), which has a discrete set of feasible solutions with a size of \((\begin{array}{c}Nd\\ L\end{array})\). Next, we provide a few equivalent expressions of ΩL for N measurements.

Bloch representation of Ω L

Let \(\{{\vec{x}}_{j}\}\) be Bloch vectors of \(\{| {x}_{j}\rangle \}\). Under Bloch representation, the projectors are in form of \(| {x}_{j}\rangle \langle {x}_{j}| =\frac{1}{d}{\mathbb{1}}+\frac{1}{2}{\vec{x}}_{j}\cdot \vec{\pi }\). Thus, we have

$${\Omega }_{L}=\mathop{\max }\limits_{\begin{array}{l}{I}_{1},\cdots \,,{I}_{N}\\ {\sum }_{\mu =1}^{N}| {I}_{\mu }| =L\end{array}}\mathop{\max }\limits_{\rho }{\rm{T}}{\rm{r}}\left[{\rm{\rho }}\left(\mathop{\sum }\limits_{{\rm{j}}=1}^{{\rm{L}}}| {{\rm{x}}}_{{\rm{j}}}\rangle \langle {{\rm{x}}}_{{\rm{j}}}| \right)\right]$$
(34)
$$=\mathop{\max }\limits_{\begin{array}{l}{I}_{1},\cdots \,,{I}_{N}\\ {\sum }_{\mu =1}^{N}| {I}_{\mu }| =L\end{array}}\mathop{\max }\limits_{\rho }{\rm{T}}{\rm{r}}\left[{\rm{\rho }}\left(\frac{L}{d}{\mathbb{1}}+{\vec{{\rm{o}}}}_{{\rm{L}}}\cdot \vec{{\rm{\pi }}}\right)\right]$$
(35)
$$=\frac{L}{d}+\mathop{\max }\limits_{\begin{array}{c}{I}_{1},\cdots \,,{I}_{N}\\ {\sum }_{\mu =1}^{N}| {I}_{\mu }| =L\end{array}}\parallel {\vec{o}}_{L}\cdot \vec{\pi }\parallel .$$
(36)

Here, \({\vec{o}}_{L}=\frac{1}{2}{\sum }_{j=1}^{L}{\vec{x}}_{j}\). Clearly, a concise expression can be derived for the qubit system

$${\Omega }_{L}=\frac{L}{2}+\mathop{\max }\limits_{\begin{array}{c}{I}_{1},\cdots \,,{I}_{N}\\ {\sum }_{\mu =1}^{N}| {I}_{\mu }| =L\end{array}}| {\vec{o}}_{L}| .$$
(37)

Transition matrix representation

Here, we formulate ΩL via the transition matrices between measurement bases.

$${\Omega }_{L}=\mathop{\max }\limits_{\begin{array}{l}{I}_{1},\cdots \,,{I}_{N}\\ {\sum }_{\mu =1}^{N}| {I}_{\mu }| =L\end{array}}\mathop{\max }\limits_{\rho }{\rm{T}}{\rm{r}}\left[{\rm{\rho }}\left(\mathop{\sum }\limits_{{\rm{j}}=1}^{{\rm{L}}}| {{\rm{x}}}_{{\rm{j}}}\rangle \langle {{\rm{x}}}_{{\rm{j}}}| \right)\right],$$
(38)
$$=\mathop{\max }\limits_{\begin{array}{c}{I}_{1},\cdots \,,{I}_{N}\\ {\sum }_{\mu =1}^{N}| {I}_{\mu }| =L\end{array}}\mathop{\max }\limits_{| \psi \rangle }\mathop{\sum }\limits_{j=1}^{L}| \langle {x}_{j}| \psi \rangle {| }^{2},$$
(39)
$$=\mathop{\max }\limits_{\begin{array}{c}{I}_{1},\cdots \,,{I}_{N}\\ {\sum }_{\mu =1}^{N}| {I}_{\mu }| =L\end{array}}\mathop{\max }\limits_{| \psi \rangle }\langle \psi | {X}^{\dagger }X| \psi \rangle ,$$
(40)
$$=\mathop{\max }\limits_{\begin{array}{c}{I}_{1},\cdots \,,{I}_{N}\\ {\sum }_{\mu =1}^{N}| {I}_{\mu }| =L\end{array}}{\lambda }_{\max }({\mathcal{X}}).$$
(41)

Here, we have employed the property of operator norm in the last line and \({\lambda }_{\max }({\mathcal{X}})\) denotes the largest eigenvalue of the operator \({\mathcal{X}}=X{X}^{\dagger }\) and \(X=(| {x}_{1}\rangle ,| {x}_{2}\rangle ,\cdots \,,| {x}_{k}\rangle )\). The operator \({\mathcal{X}}\) is defined as

$${\mathcal{X}}=X{X}^{\dagger }=\left[\begin{array}{cccc}{{\mathbb{1}}}_{| {I}_{1}| } & {U}_{(1,2)}[{I}_{1},{I}_{2}] & \cdots & {U}_{(1,N)}[{I}_{1},{I}_{N}]\\ {U}_{(2,1)}^{\dagger }[{I}_{2},{I}_{1}] & {{\mathbb{1}}}_{| {I}_{2}| } & \cdots & {U}_{(2,N)}[{I}_{2},{I}_{N}]\\ \vdots & \vdots & \ddots & \vdots \\ {U}_{(N,1)}^{\dagger }[{I}_{N},{I}_{1}] & {U}_{(N,2)}^{\dagger }[{I}_{N},{I}_{2}] & \cdots & {{\mathbb{1}}}_{| {I}_{N}| }\end{array}\right],$$
(42)

where \({{\mathbb{1}}}_{| {I}_{\mu }| }\) is the identity matrix of size Iμ × Iμ and U(i, j)[Iμ, Iν] is the submatrix of entries that lie in the rows of the transition matrix \({U}_{(i,j)}={\{\langle {a}_{i}^{(\mu )}| {a}_{j}^{(\nu )}\rangle \}}_{i,j=1}^{d}\) indexed by Iμ and the columns indexed by Iν, i.e. \({U}_{(i,j)}[{I}_{\mu },{I}_{\nu }]={\{\langle {a}_{i}^{(\mu )}| {a}_{j}^{(\nu )}\rangle \}}_{i\in {I}_{\mu },j\in {I}_{\nu }}\).

Two measurement bases scenario

When the involved measurement bases are two orthonormal complete bases, i.e., N = 2, we have

$${\mathcal{X}}=\left[\begin{array}{cc}{{\mathbb{1}}}_{| {I}_{1}| } & U[{I}_{1},{I}_{2}]\\ {U}^{\dagger }[{I}_{2},{I}_{1}] & {{\mathbb{1}}}_{| {I}_{2}| }\end{array}\right]={{\mathbb{1}}}_{| {I}_{1}| +| {I}_{2}| }+\left[\begin{array}{cc}0 & U[{I}_{1},{I}_{2}]\\ {U}^{\dagger }[{I}_{2},{I}_{1}] & 0\end{array}\right]$$
(43)

In light of Theorem 7.3.3 in ref. 70, we have \({\lambda }_{\max }({\mathcal{X}})=1+{\sigma }_{\max }(U[{I}_{1},{I}_{2}])\), and thus

$${\Omega }_{L}=1+\mathop{\max }\limits_{\begin{array}{c}{I}_{1},{I}_{2}\\ | {I}_{1}| +| {I}_{2}| =L\end{array}}{\sigma }_{\max }(U[{I}_{1},{I}_{2}]),L\le d,$$
(44)
$${\Omega }_{L}=2,L > d.$$
(45)

Here, \({\sigma }_{\max }(\cdot )\) denotes the maximal singular value and \(U[{I}_{1},{I}_{2}]={\{{u}_{ij}\}}_{i\in {I}_{1},j\in {I}_{2}}\) for \({u}_{ij}=\langle {a}_{i}^{(1)}| {a}_{j}^{(2)}\rangle\). If I1 = 1 or I2 = 1, we have \({\sigma }_{\max }(U[{I}_{1},{I}_{2}])=\sqrt{{\sum }_{j\in {I}_{n}}| {u}_{ij}{| }^{2}}\) or \({\sigma }_{\max }(U[{I}_{m},{I}_{1}])=\sqrt{{\sum }_{i\in {I}_{m}}| {u}_{ij}{| }^{2}}\). So, the first three terms have the analytical expressions

$${\Omega }_{1}=1,{\Omega }_{2}=1+\mathop{\max \limits_{i,j}\left.\left|\left\langle {a}_{i}^{(1)}\right|{{a}_{j}^{(2)}}\right\rangle \right|},$$
(46)
$${\Omega }_{3}=1+\mathop{\max }\limits_{\begin{array}{l}i={i}^{{\prime} },j\,\ne \,{j}^{{\prime} }\\ j={j}^{{\prime} },i\,\ne \,{i}^{{\prime} }\end{array}}\sqrt{| \langle {a}_{i}^{(1)}| {a}_{j}^{(2)}\rangle {| }^{2}+| \langle {a}_{{i}^{{\prime} }}^{(1)}| {a}_{{j}^{{\prime} }}^{(2)}\rangle {| }^{2}}.$$
(47)

Mutually unbiased bases

For a pair of mutually unbiased bases (MUBs), the transition matrix U between them is a discrete Fourier transformation (DFT) matrix, i.e.

$$U=\frac{1}{\sqrt{d}}\left[\begin{array}{ccccc}1 & 1 & 1 & \cdots & 1\\ 1 & \omega & {\omega }^{2} & \cdots & {\omega }^{d-1}\\ 1 & {\omega }^{2} & {\omega }^{4} & \cdots & {\omega }^{2(d-1)}\\ 1 & {\omega }^{3} & {\omega }^{6} & \cdots & {\omega }^{3(d-1)}\\ \vdots & \vdots & \vdots & \ddots & \vdots \\ 1 & {\omega }^{d-1} & {\omega }^{2(d-1)} & \cdots & {\omega }^{(d-1)(d-1)}\end{array}\right],$$
(48)

where ω = e2πi/d is a d-th root of unity. For a pair of d-dimensional MUBs, we conjecture the following expression. It is noted that the matrix U is only one possible example of pairs of MUBs. sThere exist inequivalent pairs of MUBs57,71.

Conjecture

$${\Omega }_{L}=1+\mathop{\max }\limits_{\begin{array}{c}{I}_{m},{I}_{n}\\ | {I}_{m}| =\lfloor \frac{L}{2}\rfloor ,| {I}_{n}| =\lceil \frac{L}{2}\rceil \end{array}}{\sigma }_{\max }(U[{I}_{m},{I}_{n}]),L\le d.$$
(49)

Here, and denote the floor and the ceiling functions, respectively.