Abstract
Measurement of the ground-state spin polarization of quantum systems offers great potential for the discovery and characterization of correlated electronic states. However, spin polarization measurements have mainly involved optical1,2,3 and NMR4,5 techniques that perturb the delicate ground states and, for quantum Hall systems, have provided conflicting results1,4,6. Here we present spin-resolved pulsed tunnelling (SRPT) that precisely determines the phase diagram of the ground-state spin polarization as a function of magnetic field and Landau level (LL) filling factor (ν) with negligible perturbation to the system. Our phase diagram shows a variety of polarized, unpolarized and topological spin states in the lowest (N = 0) LL, which can largely be described by a weakly interacting composite fermion (CF) model7. However, the phase diagram shows unexpected behaviour in the N = 1 LL. We observe fully polarized ν = 5/2 and 8/3 states but a partially depolarized ν = 7/3 state. This behaviour deviates from the conventional theoretical picture7,8 of weakly interacting fractional quasiparticles, but instead suggests unusual electronic correlations and the possibility of new non-Abelian phases9,10,11. The results establish SRPT as a powerful technique for investigating correlated electron phenomena.
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Source data are provided with this paper. All other data that support the plots within this paper and other findings of this study are available from the corresponding author upon reasonable request.
References
Stern, M. et al. Optical probing of the spin polarization of the ν = 5/2 quantum Hall state. Phys. Rev. Lett. 105, 096801 (2010).
Hayakawa, J., Muraki, K. & Yusa, G. Real-space imaging of fractional quantum Hall liquids. Nat. Nanotechnol. 8, 31–35 (2013).
Kukushkin, I. V., Klitzing, K. V. & Eberl, K. Spin polarization of composite fermions: measurements of the Fermi energy. Phys. Rev. Lett. 82, 3665–3668 (1999).
Tiemann, L., Gamez, G., Kumada, N. & Muraki, K. Unraveling the spin polarization of the Ν = 5/2 fractional quantum Hall state. Science 335, 828–831 (2012).
Barrett, S. E., Dabbagh, G., Pfeiffer, L. N., West, K. W. & Tycko, R. Optically pumped NMR evidence for finite-size skyrmions in GaAs quantum wells near Landau level filling ν = 1. Phys. Rev. Lett. 74, 5112–5115 (1995).
Kukushkin, I. V., Klitzing, K. V. & Eberl, K. Spin polarization of two-dimensional electrons in different fractional states and around filling factor ν = 1. Phys. Rev. B 55, 10607–10612 (1997).
Jain, J. K. Composite Fermions (Cambridge Univ. Press, 2007).
Laughlin, R. B. Anomalous quantum Hall effect: an incompressible quantum fluid with fractionally charged excitations. Phys. Rev. Lett. 50, 1395–1398 (1983).
Bonderson, P. & Slingerland, J. K. Fractional quantum Hall hierarchy and the second Landau level. Phys. Rev. B 78, 125323 (2008).
Balram, A. C., Jain, J. K. & Barkeshli, M. Zn superconductivity of composite bosons and the 7/3 fractional quantum Hall effect. Phys. Rev. Res. 2, 013349 (2020).
Peterson, M. R. et al. Abelian and non-Abelian states in ν = 2/3 bilayer fractional quantum Hall systems. Phys. Rev. B 92, 035103 (2015).
Smet, J. H. et al. Gate-voltage control of spin interactions between electrons and nuclei in a semiconductor. Nature 415, 281 (2002).
Dial, O. E., Ashoori, R. C., Pfeiffer, L. N. & West, K. W. High-resolution spectroscopy of two-dimensional electron systems. Nature 448, 176–179 (2007).
Ezawa, Z. F. & Tsitsishvili, G. Quantum Hall ferromagnets. Rep. Prog. Phys. 72, 086502 (2009).
MacDonald, A. H., Oji, H. C. A. & Liu, K. L. Thermodynamic properties of an interacting two-dimensional electron gas in a strong magnetic field. Phys. Rev. B 34, 2681–2689 (1986).
Chaudhary, G., Efimkin, D. K. & MacDonald, A. H. Tunneling density of states, correlation energy, and spin polarization in the fractional quantum Hall regime. Phys. Rev. B 100, 085107 (2019).
Park, K. & Jain, J. K. Phase diagram of the spin polarization of composite fermions and a new effective mass. Phys. Rev. Lett. 80, 4237–4240 (1998).
Archer, A. C. & Jain, J. K. Phase diagram of the two-component fractional quantum Hall effect. Phys. Rev. Lett. 110, 246801 (2013).
Sondhi, S. L., Karlhede, A., Kivelson, S. A. & Rezayi, E. H. Skyrmions and the crossover from the integer to fractional quantum Hall effect at small Zeeman energies. Phys. Rev. B 47, 16419–16426 (1993).
Balram, A. C., Wurstbauer, U., Wójs, A., Pinczuk, A. & Jain, J. K. Fractionally charged skyrmions in fractional quantum Hall effect. Nat. Commun. 6, 8981 (2015).
Fertig, H. A. et al. Hartree–Fock theory of skyrmions in quantum Hall ferromagnets. Phys. Rev. B 55, 10671–10680 (1997).
Nayak, C., Simon, S. H., Stern, A., Freedman, M. & Das Sarma, S. Non-Abelian anyons and topological quantum computation. Rev. Mod. Phys. 80, 1083–1159 (2008).
Eisenstein, J. P. et al. Collapse of the even-denominator fractional quantum Hall effect in tilted fields. Phys. Rev. Lett. 61, 997–1000 (1988).
Pan, W. et al. Competing quantum Hall phases in the second Landau level in the low-density limit. Phys. Rev. B 89, 241302 (2014).
Kleinbaum, E., Kumar, A., Pfeiffer, L. N., West, K. W. & Csáthy, G. A. Gap reversal at filling factors 3+1/3 and 3+1/5: towards novel topological order in the fractional quantum Hall regime. Phys. Rev. Lett. 114, 076801 (2015).
Pan, W., Baldwin, K. W., West, K. W., Pfeiffer, L. N. & Tsui, D. C. Spin transition in the ν = 8/3 fractional quantum Hall effect. Phys. Rev. Lett. 108, 216804 (2012).
Haldane, D. F. in The Quantum Hall Effect (ed. Prange, R. E.) 303–352 (Springer, 1987).
MacDonald, A. H. Introduction to the physics of the quantum Hall regime. Preprint at http://arxiv.org/abs/cond-mat/9410047 (1994).
Jain, J. K., Kamilla, R. K., Park, K. & Scarola, V. W. Interacting composite fermions. Solid State Commun. 117, 117–122 (2001).
d’Ambrumenil, N. & Reynolds, A. M. Fractional quantum Hall states in higher Landau levels. J. Phys. C 21, 119–132 (1988).
MacDonald, A. H. & Girvin, S. M. Collective excitations of fractional Hall states and Wigner crystallization in higher Landau levels. Phys. Rev. B 33, 4009–4013 (1986).
Chakraborty, T. & Pietiläinen, P. Temperature dependence of spin polarizations at higher Landau levels. Phys. Rev. Lett. 83, 5559–5562 (1999).
Koulakov, A. A., Fogler, M. M. & Shklovskii, B. I. Charge density wave in two-dimensional electron liquid in weak magnetic field. Phys. Rev. Lett. 76, 499 (1996).
Samkharadze, N. et al. Observation of a transition from a topologically ordered to a spontaneously broken symmetry phase. Nat. Phys. 12, 191–195 (2016).
Schreiber, K. A. et al. Electron–electron interactions and the paired-to-nematic quantum phase transition in the second Landau level. Nat. Commun. 9, 1–7 (2018).
Acknowledgements
We thank J. K. Jain and A. H. MacDonald for discussions. This work is supported by the Basic Energy Sciences Program of the Office of Science of the US Department of Energy through contract no. FG02-08ER46514 and by the Gordon and Betty Moore Foundation through grant GBMF2931. The work at Princeton University was funded by the Gordon and Betty Moore Foundation through the EPiQS (Emergent Phenomena in Quantum Systems) initiative grant GBMF4420 and by the National Science Foundation MRSEC (Materials Research Science and Engineering Centers) grant DMR-1420541.
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H.M.Y. and R.C.A. conceived the experiments. L.P., K.W.B. and K.W. contributed in the epitaxial growth of the sample. H.M.Y. carried out the measurements. H.M.Y. and R.C.A. performed data analysis and prepared the manuscript. R.C.A. supervised the project.
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Supplementary Information
Supplementary Figs. 1–10, Supplementary Discussion
Source data
Source Data Fig. 1
Raw tunnelling current spectra.
Source Data Fig. 2
Spin polarization 1D plot.
Source Data Fig. 3
Spin polarization 2D plot.
Source Data Fig. 4
Spin polarization 2D plot.
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Yoo, H.M., Baldwin, K.W., West, K. et al. Spin phase diagram of the interacting quantum Hall liquid. Nat. Phys. 16, 1022–1027 (2020). https://doi.org/10.1038/s41567-020-0946-1
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DOI: https://doi.org/10.1038/s41567-020-0946-1
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