Abstract
Vehicle emissions produce an important share of a city’s air pollution, with a substantial impact on the environment and human health. Traditional emission estimation methods use remote sensing stations, missing the full driving cycle of vehicles, or focus on a few vehicles. We have used GPS traces and a microscopic model to analyse the emissions of four air pollutants from thousands of private vehicles in three European cities. We found that the emissions across the vehicles and roads are well approximated by heavy-tailed distributions and thus discovered the existence of gross polluters, vehicles responsible for the greatest quantity of emissions, and grossly polluted roads, which suffer the greatest amount of emissions. Our simulations show that emissions reduction policies targeting gross polluters are far more effective than those limiting circulation based on an uninformed choice of vehicles. Our study contributes to shaping the discussion on how to measure emissions with digital data.
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Data availability
The data that support the findings of this study are not publicly available due to privacy restrictions and were used under licence for the current study. Aggregated source data for figures are available from the authors upon reasonable request.
Code availability
The Python code to reproduce the analyses in the study from public GPS data (taxi trips) is publicly available in GitHub (https://github.com/matteoboh/mobility_emissions) and the Zenodo repository66.
References
Venter, Z. S., Aunan, K., Chowdhury, S. & Lelieveld, J. COVID-19 lockdowns cause global air pollution declines. Proc. Natl Acad. Sci. USA 117, 18984–18990 (2020).
Le Quéré, C. et al. Temporary reduction in daily global CO2 emissions during the COVID-19 forced confinement. Nat. Clim. Change 10, 647–653 (2020).
He, G., Pan, Y. & Tanaka, T. The short-term impacts of COVID-19 lockdown on urban air pollution in China. Nat. Sustain. 3, 1005–1011 (2020).
Liu, Z. et al. Near-real-time monitoring of global CO2 emissions reveals the effects of the COVID-19 pandemic. Nat. Commun. 11, 5172 (2020).
Forster, P. et al. Current and future global climate impacts resulting from COVID-19. Nat. Clim. Change 10, 913–919 (2020).
IPCC Climate Change 2014: Mitigation of Climate Change (eds Edenhofer et al.) 599–670 (Cambridge Univ. Press, 2014).
Ritchie, H. Sector by Sector: Where Do Global Greenhouse Gas Emissions Come From? (Our World in Data, 2020); https://ourworldindata.org/ghg-emissions-by-sector
United Nations General Assembly Transforming Our World: The 2030 Agenda for Sustainable Development (United Nations, 2015).
deSouza, P. et al. Air quality monitoring using mobile low-cost sensors mounted on trash-trucks: methods development and lessons learned. Sustaina. Cities Soc. 60, 102239 (2020).
Chong, H. S., Kwon, S., Lim, Y. & Lee, J. Real-world fuel consumption, gaseous pollutants, and CO2 emission of light-duty diesel vehicles. Sustain. Cities Soc. 53, 101925 (2020).
Luján, J. M., Bermúdez, V., Dolz, V. & Monsalve-Serrano, J. An assessment of the real-world driving gaseous emissions from a Euro 6 light-duty diesel vehicle using a portable emissions measurement system (PEMS). Atmos. Environ. 174, 112–121 (2018).
Chatterton, T., Barnes, J., Wilson, R. E., Anable, J. & Cairns, S. Use of a novel dataset to explore spatial and social variations in car type, size, usage and emissions. Transp. Res. D 39, 151–164 (2015).
i Diao, M. & Ferreira, J. Jr. Vehicle miles traveled and the built environment: evidence from vehicle safety inspection data. Environ. Plan. A. 46, 2991–3009 (2014).
Kancharla, S. R. & Ramadurai, G. Incorporating driving cycle based fuel consumption estimation in green vehicle routing problems. Sustain. Cities Soc. 40, 214–221 (2018).
Choudhary, A. & Gokhale, S. Urban real-world driving traffic emissions during interruption and congestion. Transp. Res. D 43, 59–70 (2016).
Ferreira, J. C., de Almeida, J. & da Silva, A. R. The impact of driving styles on fuel consumption: a data-warehouse-and-data-mining-based discovery process. IEEE Trans. Intell. Transp. Syst. 16, 2653–2662 (2015).
Zheng, F., Li, J., van Zuylen, H. & Lu, C. Influence of driver characteristics on emissions and fuel consumption. In 20th EURO Working Group on Transportation Meeting (eds Esztergár-Kiss, D. et al.) 624–631 (Elsevier, 2017).
Pappalardo, L., Rinzivillo, S., Qu, Z., Pedreschi, D. & Giannotti, F. Understanding the patterns of car travel. Eur. Phys. J. Spec. Top. 215, 61–73 (2013).
Pappalardo, L. et al. Returners and explorers dichotomy in human mobility. Nat. Commun. 6, 8166 (2015).
Gallotti, R., Bazzani, A. & Rambaldi, S. Towards a statistical physics of human mobility. Int. J. Mod. Phys. C 23, 1250061 (2012).
Luca, M., Barlacchi, G., Lepri, B. & Pappalardo, L. A survey on deep learning for human mobility. ACM Comput. Surv. 55, 1–44 (2021).
Barbosa, H. et al. Human mobility: models and applications. Phys. Rep. 734, 1–74 (2018).
Çolak, S., Lima, A. & González, M. C. Understanding congested travel in urban areas. Nat. Commun. 7, 10793 (2016).
Lwin, H. & Naing, T. Estimation of road traffic congestion using GPS data. Int. J. Adv. Res. Comput. Commun. Eng. 4, 1–5 (2015).
Stipancic, J., Miranda-Moreno, L., Labbe, A. & Saunier, N. Measuring and visualizing space–time congestion patterns in an urban road network using large-scale smartphone-collected GPS data. Transp. Lett. 11, 391–401 (2019).
Camargo, C. Q., Bright, J., McNeill, G., Raman, S. & Hale, S. A. Estimating traffic disruption patterns with volunteered geographic information. Sci. Rep. 10, 1271 (2020).
Jenn, A. Emissions benefits of electric vehicles in Uber and Lyft ride-hailing services. Nat. Energy 5, 520–525 (2020).
Liang, X. et al. Air quality and health benefits from fleet electrification in China. Nat. Sustain. 2, 962–971 (2019).
Rolnick, D. et al. Tackling climate change with machine learning. ACM Comput. Surv. 55, 1–96 (2019).
Nyhan, M. et al. Predicting vehicular emissions in high spatial resolution using pervasively measured transportation data and microscopic emissions model. Atmos. Environ. 140, 352–363 (2016).
Liu, J., Han, K., Chen, X. M. & Ong, G. P. Spatial-temporal inference of urban traffic emissions based on taxi trajectories and multi-source urban data. Transp. Res. C 106, 145–165 (2019).
Reznik, A., Kissinger, M. & Alfasi, N. Real-data-based high-resolution GHG emissions accounting of urban residents private transportation. Int. J. Sustain. Transp. 13, 235–244 (2019).
Wang, X., Grengs, J. & Kostyniuk, L. Using a GPS data set to examine the effects of the built environment along commuting routes on travel outcomes. J. Urban Plan. Dev. 140, 04014009 (2014).
Cervero, R. & Kockelman, K. Travel demand and the 3Ds: density, diversity, and design. Transp. Res. D 2, 199–219 (1997).
Gately, C. K., Hutyra, L. R., Peterson, S. & Sue Wing, I. Urban emissions hotspots: quantifying vehicle congestion and air pollution using mobile phone GPS data. Environ. Pollut. 229, 496–504 (2017).
Chen, J. et al. Mining urban sustainable performance: GPS data-based spatio-temporal analysis on on-road braking emission. J. Clean. Prod. 270, 122489 (2020).
Sui, Y. et al. GPS data in urban online ride-hailing: a comparative analysis on fuel consumption and emissions. J. Clean. Prod. 227, 495–505 (2019).
Yu, Q. et al. Mobile phone GPS data in urban customized bus: dynamic line design and emission reduction potentials analysis. J. Clean. Prod. 272, 122471 (2020).
Rahman, M. N. & Idris, A. O. Tribute: trip-based urban transportation emissions model for municipalities. Int. J. Sustain. Transp. 11, 540–552 (2017).
Zhu, S., Kim, I. & Choi, K. High-resolution simulation-based analysis of leading vehicle acceleration profiles at signalized intersections for emission modeling. Int. J. Sustain. Transp. 15, 375–385 (2020).
Aziz, H. M. A. & Ukkusuri, S. V. A novel approach to estimate emissions from large transportation networks: hierarchical clustering-based link-driving-schedules for EPA-MOVES using dynamic time warping measures. Int. J. Sustain. Transp. 12, 192–204 (2018).
Guenther, P., Bishop, G., Peterson, J. & Stedman, D. Emissions from 200 000 vehicles: a remote sensing study. Sci. Total Environ. 146–147, 297–302 (1994).
Brand, C. & Boardman, B. Taming of the few—the unequal distribution of greenhouse gas emissions from personal travel in the UK. Energy Policy 36, 224–238 (2008).
Huang, Y. et al. Remote sensing of on-road vehicle emissions: mechanism, applications and a case study from Hong Kong. Atmos. Environ. 182, 58–74 (2018).
Huang, Y. et al. Re-evaluating effectiveness of vehicle emission control programmes targeting high-emitters. Nat. Sustain. 3, 904–907 (2020).
Batty, M. et al. Smart cities of the future. Eur. Phys. J. Spec. Top. 214, 481–518 (2012).
Kitchin, R. The real-time city? Big data and smart urbanism. GeoJournal 79, 1–14 (2014).
Voukelatou, V. et al. Measuring objective and subjective well-being: dimensions and data sources. Int. J. Data Sci. Anal. 11, 279–309 (2020).
OpenStreetMap contributors https://www.openstreetmap.org (2017); planet dump, retrieved from https://planet.osm.org
González, M. C., Hidalgo, C. A. & Barabási, A.-L. Understanding individual human mobility patterns. Nature 453, 779–782 (2008).
Pappalardo, L., Simini, F., Barlacchi, G. & Pellungrini, R. scikit-mobility: a Python library for the analysis, generation and risk assessment of mobility data. Preprint at http://arxiv.org/abs/1907.07062 (2019).
Song, C., Qu, Z., Blumm, N. & Barabási, A.-L. Limits of predictability in human mobility. Science 327, 1018–1021 (2010).
Eagle, N. & Pentland, A. S. Eigenbehaviors: identifying structure in routine. Behav. Ecol. Sociobiol. 63, 1057–1066 (2009).
Pappalardo, L. et al. An analytical framework to nowcast well-being using mobile phone data. Int. J. Data Sci. Anal. 2, 75–92 (2016).
Hastie, T. & Tibshirani, R. Generalized additive models. Stat. Sci. 1, 297–310 (1986).
Lelo, K., Monni, S. & Tomassi, F. Socio-spatial inequalities and urban transformation. The case of Rome districts. Socioecon. Plan. Sci. 68, 100696 (2019).
Richards, F. J. A flexible growth function for empirical use. J. Exp. Bot. 10, 290–300 (1959).
Fekedulegn, D. & Colbert, J. Parameter estimation of nonlinear growth models in forestry. Silva Fenn. 33, 653 (1999).
Vyas, L. & Butakhieo, N. The impact of working from home during COVID-19 on work and life domains: an exploratory study on Hong Kong. Policy Des. Pract. 4, 59–76 (2021).
Nagel, L. The influence of the COVID-19 pandemic on the digital transformation of work. Int. J. Sociol. Soc. Policy 40, 861–875 (2020).
Travel in London: Report 12 (Transport for London, 2019); http://content.tfl.gov.uk/travel-in-london-report-12.pdf
Fuschiotto, A. et al. Rapporto Mobilità 2019 (Dipartimento Mobilità e Trasporti Roma Capitale, 2019); https://romamobilita.it/it/media/pubblicazioni/rapporto-mobilita-2019
Boeing, G. OSMnx: new methods for acquiring, constructing, analyzing, and visualizing complex street networks. Comput. Environ. Urban Syst. 65, 126–139 (2017).
White, C. E., Bernstein, D. & Kornhauser, A. L. Some map matching algorithms for personal navigation assistants. Transp. Res. C 8, 91–108 (2000).
Pappalardo, L., Ferres, L., Sacasa, M., Cattuto, C. & Bravo, L. Evaluation of home detection algorithms on mobile phone data using individual-level ground truth. EPJ Data Sci. 10, 29 (2021).
Bohm, M., Nanni, M. & Pappalardo, L. matteoboh/mobility emissions: code release for Nature Sustainability paper https://doi.org/10.5281/zenodo.6124225 (2022).
Acknowledgements
This work was partially funded by the Horizon 2020 projects Track & Know (grant agreement no. 780754, M.N.), SoBigData++ (grant agreement no. 871042, M.B.) and HumanE-AI-Net (grant agreement no. 952026, L.P.). We thank G. Cornacchia, V. Voukelatou, M. Luca and G. Mauro for their useful suggestions, D. Fadda for his precious support in data visualization and F. Totti for his inspiration.
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M.B. designed the study, performed the data pre-processing and cleaning, developed the code for and performed the statistical analyses, experiments and simulations, created the plots, contributed to the interpretation of the results and wrote the paper. M.N. provided the data, contributed to the work methodology and interpretation of the results, and revised the paper. L.P. developed the concept and designed the study, contributed to the work methodology and interpretation of the results, wrote the paper and coordinated the study. All authors read, edited and approved the final version of the paper.
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Extended data
Extended Data Fig. 1 Step-by-step procedure for the computation of emissions and results analyses.
The left column describes the steps followed starting from the data, passing through the data processing, and ending with the analyses performed. The central column shows a schema of what happens in each step. The right column shows some numbers and results in support of the central column. The heatmap in step 1 is plotted with the Python library scikit-mobility51. The small road network in step 7 is plotted with the Python library OSMnx63. Car icons from the Noun Project (thenounproject.com).
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Supplementary Figs. 1–32, Tables 1–13, Notes 1–8 and references.
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Böhm, M., Nanni, M. & Pappalardo, L. Gross polluters and vehicle emissions reduction. Nat Sustain 5, 699–707 (2022). https://doi.org/10.1038/s41893-022-00903-x
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DOI: https://doi.org/10.1038/s41893-022-00903-x
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