Table 1 Refined AF1 commensurate magnetic structure at 200 K

From: Evidence of high-temperature magnetic spiral in YBaCuFeO5 single-crystal by spherical neutron polarimetry

AF1 collinear phase with conjugated magnetic domains (D1, D2)

m1B)

m2B)

θc (deg)

ϕc (deg)

φ‘c (deg)

Dom. pop.

D1/D2 (%)

Agreement factors

Unpolarized neutrons (D10)

 1.284 (3)

2.188 (7)

91.0 (9)

46 (19)

179.8 (6)

53.7/46.3 (1.6)

χ2 = 2.87; RF = 4.82; \({{\rm{R}}}_{{\rm{F}}}^{2}\) = 9.25

Spherical Neutron Polarimetry (D3)

 –

90.8 (1)

43 (8)

180

53.1/46.9 (0.5)

χ2 = 3.22

  1. The two independent results correspond to the fitting of (i) the neutron-integrated magnetic intensities collected in D10 (unpolarized neutrons) and (ii) the fitting of the neutron polarization matrices (SNP) measured in D3. The spherical neutron polarization matrices are more sensitive than the integrated intensities to the orientation of the spins in the ab plane. The refined domain population is also shown.